Deflection of Rotating Symmetric Molecules by Inhomogeneous Fields

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle. Scattering of the prolate/oblate molecules is analyzed in detail, and it is shown that the process can be efficiently controlled by means of short and strong femtosecond laser pulses. In particular, the angular dispersion of the deflected molecules may be dramatically reduced by laser-induced molecular pre-alignment. We first study the problem by using a simple classical model, and then find similar results by means of more sophisticated methods, including the formalism of adiabatic invariants and direct numerical simulation of the Euler-Lagrange equations of motion. The suggested control scheme opens new ways for many applications involving molecular focusing, guiding, and trapping by optical and static fields

Deflection of field-free aligned molecules

We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like features in the distribution of the scattering angle. Moreover, by pre-shaping molecular angular distribution with the help of short and strong femtosecond laser pulses, one may efficiently control the scattering process, manipulate the average deflection angle and its distribution, and reduce substantially the angular dispersion of the deflected molecules. This opens new ways for many applications involving molecular focusing, guiding and trapping by optical and static fields.Comment: 4 pages, 4 figure

Enhanced Molecular Orientation Induced by Molecular Anti-Alignment

We explore the role of laser induced anti-alignment in enhancing molecular orientation. A field-free enhanced orientation via anti-alignment scheme is presented, which combines a linearly polarized femtosecond laser pulse with a half-cycle pulse. The laser pulse induces transient anti-alignment in the plane orthogonal to the field polarization, while the half-cycle pulse leads to the orientation. We identify two qualitatively different enhancement mechanisms depending on the pulse order, and optimize their effects using classical and quantum models both at zero and non-zero temperature

Splitting in the Excitation Spectrum of A Bose-Einstein Condensate Undergoing Strong Rabi Oscillations

We report on a measurement of splitting in the excitation spectrum of a condensate driven by an optical travelling wave. Experimental results are compared to a numerical solution of the Gross Pitaevskii equation, and analyzed by a simple two level model and by the more complete band theory, treating the driving beams as an optical lattice. In this picture, the splitting is a manifestation of the energy gap between neighboring bands that opens on the boundary of the Brillouin zone.Comment: 5 pages, 5 figure

Echo spectroscopy of bulk Bogoliubov excitations in trapped Bose-Einstein condensates

We propose and demonstrate an echo method to reduce the inhomogeneous linewidth of Bogoliubov excitations, in a harmonically-trapped Bose-Einstein condensate. Our proposal includes the transfer of excitations with momentum +q to -q using a double two photon Bragg process, in which a substantial reduction of the inhomogeneous broadening is calculated. Furthermore, we predict an enhancement in the method's efficiency for low momentum due to many-body effects. The echo can also be implemented by using a four photon process, as is demonstrated experimentally.Comment: 4 pages, 5 figure

Decoherence and dephasing in strongly driven colliding Bose-Einstein condensates

We report on a series of measurements of decoherence and wavepacket dephasing between two colliding, strongly coupled, identical Bose-Einstein condensates. We measure, in the strong excitation regime, a suppression of the mean-field shift, compared to the shift which is observed for a weak excitation. This suppression is explained by applying the Gross-Pitaevskii energy functional. By selectively counting only the non-decohered fraction in a time of flight image we observe oscillations for which both inhomogeneous and Doppler broadening are suppressed, in quantitative agreement with a full Gross-Pitaevskii equation simulation. If no post selection is used, the decoherence rate due to collisions can be extracted, and is in agreement with the local density average calculated rate.Comment: 4 pages, 5 figure

Electric Deflection of Rotating Molecules

We provide a theory of the deflection of polar and non-polar rotating molecules by inhomogeneous static electric field. Rainbow-like features in the angular distribution of the scattered molecules are analyzed in detail. Furthermore, we demonstrate that one may efficiently control the deflection process with the help of short and strong femtosecond laser pulses. In particular the deflection process may by turned-off by a proper excitation, and the angular dispersion of the deflected molecules can be substantially reduced. We study the problem both classically and quantum mechanically, taking into account the effects of strong deflecting field on the molecular rotations. In both treatments we arrive at the same conclusions. The suggested control scheme paves the way for many applications involving molecular focusing, guiding, and trapping by inhomogeneous fields