Ripple formation on Nickel irradiated with radially polarized femtosecond beams

We report on the morphological effects induced by the inhomogeneous absorption of radially polarized femtosecond laser irradiation of nickel (Ni) in sub-ablation conditions. A theoretical prediction of the morphology profile is performed and the role of surface plasmon excitation in the production of self-formed periodic ripples structures is evaluated. Results indicate a smaller periodicity of the ripples profile compared to that attained under linearly polarized irradiation conditions. A combined hydrodynamical and thermoelastic model is presented in laser beam conditions that lead to material melting. The simulation results are presented to be in good agreement with the experimental findings. The ability to control the size of the morphological changes via modulating the beam polarization may provide an additional route for controlling and optimizing the outcome of laser micro-processingComment: 4 pages, 4 figures, 4 appendix page

Control of the damage threshold of Si via a SiO2 coating upon irradiation with Mid-IR femtosecond laser pulses

A key issue in the use of high-power mid-infrared (Mid-IR) laser sources for a plethora of applications is the investigation of the exciting laser driven physical phenomena taking place in materials coated with dielectric films. Here, we present a theoretical investigation of the ultrafast processes and thermal response upon excitation of two-layered complexes consisting of fused silica thin films placed on silicon substrates with ultrashort pulsed lasers in the Mid-IR spectral regime. Through the development of a theoretical model, we demonstrate that the control of the underlying ultrafast phenomena and the damage threshold (DT) of the substrate are achieved via an appropriate modulation of the thickness of the SiO2 film. It is shown that a decrease of DT by up to 27% compared to the absence of coating is feasible emphasising the impact of coatings of a lower refractive index than the substrate. Besides this, it is demonstrated that no absorption of energy occurs within the SiO2 layer, therefore the dynamics of the reflectivity of the two-layered complex is directly associated with the electron excitation in the substrate. These remarkable predictions can be employed for the development of new optical coatings and components for nonlinear optics and photonics for a large range of Mid-IR laser-based applications.Comment: To appear In Physical Review