Diffusion of Nonequilibrium Quasiparticles in a Cuprate Superconductor

We report a transport study of nonequilibrium quasiparticles in a high-Tc cuprate superconductor using the transient grating technique. Low-intensity laser excitation (at photon energy 1.5 eV) was used to introduce a spatially periodic density of quasiparticles into a high-quality untwinned single crystal of YBa2Cu3O6.5. Probing the evolution of the initial density through space and time yielded the quasiparticle diffusion coefficient, and both inelastic and elastic scattering rates. The technique reported here is potentially applicable to precision measurement of quasiparticle dynamics, not only in cuprate superconductors, but in other electronic systems as well.Comment: 5 pages, 4 figure

Semiconducting-to-metallic photoconductivity crossover and temperature-dependent Drude weight in graphene

We investigated the transient photoconductivity of graphene at various gate-tuned carrier densities by optical-pump terahertz-probe spectroscopy. We demonstrated that graphene exhibits semiconducting positive photoconductivity near zero carrier density, which crosses over to metallic negative photoconductivity at high carrier density. Our observations are accounted for by considering the interplay between photo-induced changes of both the Drude weight and the carrier scattering rate. Notably, we observed multiple sign changes in the temporal photoconductivity dynamics at low carrier density. This behavior reflects the non-monotonic temperature dependence of the Drude weight, a unique property of massless Dirac fermions

Photoinduced Changes of Reflectivity in Single Crystals of YBa2Cu3O6.5 (Ortho II)

We report measurements of the photoinduced change in reflectivity of an untwinned single crystal of YBa2Cu3O6.5 in the ortho II structure. The decay rate of the transient change in reflectivity is found to decrease rapidly with decreasing temperature and, below Tc, with decreasing laser intensity. We interpret the decay as a process of thermalization of antinodal quasiparticles, whose rate is determined by an inelastic scattering rate of quasiparticle pairs.Comment: 4 pages, 4 figure

Amplitude dynamics of charge density wave in LaTe3_3: theoretical description of pump-probe experiments

We formulate a dynamical model to describe a photo-induced charge density wave (CDW) quench transition and apply it to recent multi-probe experiments on LaTe$_3$ [A. Zong et al., Nat. Phys. 15, 27 (2019)]. Our approach relies on coupled time-dependent Ginzburg-Landau equations tracking two order parameters that represent the modulations of the electronic density and the ionic positions. We aim at describing the amplitude of the order parameters under the assumption that they are homogeneous in space. This description is supplemented by a three-temperature model, which treats separately the electronic temperature, temperature of the lattice phonons with stronger couplings to the electronic subsystem, and temperature of all other phonons. The broad scope of available data for LaTe$_3$ and similar materials as well as the synergy between different time-resolved spectroscopies allow us to extract model parameters. The resulting calculations are in good agreement with ultra-fast electron diffraction experiments, reproducing qualitative and quantitative features of the CDW amplitude evolution during the initial few picoseconds after photoexcitation.Comment: 21 pages, 14 figures; this version is almost identical to the published version; comparing to the earlier arXiv submission, current version contains a new figure (Fig.10), and a broader discussion of theoretical results and approximation

Spatially modulated magnetic structure of EuS due to the tetragonal domain structure of SrTiO3_3

The combination of ferromagnets with topological superconductors or insulators allows for new phases of matter that support excitations such as chiral edge modes and Majorana fermions. EuS, a wide-band-gap ferromagnetic insulator with a Curie temperature around 16 K, and SrTiO$_3$ (STO), an important substrate for engineering heterostructures, may support these phases. We present scanning superconducting quantum interference device (SQUID) measurements of EuS grown epitaxially on STO that reveal micron-scale variations in ferromagnetism and paramagnetism. These variations are oriented along the STO crystal axes and only change their configuration upon thermal cycling above the STO cubic-to-tetragonal structural transition temperature at 105 K, indicating that the observed magnetic features are due to coupling between EuS and the STO tetragonal structure. We speculate that the STO tetragonal distortions may strain the EuS, altering the magnetic anisotropy on a micron-scale. This result demonstrates that local variation in the induced magnetic order from EuS grown on STO needs to be considered when engineering new phases of matter that require spatially homogeneous exchange

Analysis of a Parallel Machine Scheduling Problem with Sequence Dependent Setup Times and Job Availability Intervals

In this study, we propose constraint programming (CP) model and logic-based Benders algorithms in order to make the best decisions for scheduling non-identical jobs with availability intervals and sequence dependent setup times on unrelated parallel machines in a fixed planning horizon. In this problem, each job has a profit, cost and must be assigned to at most one machine in such a way that total profit is maximized. In addition, the total cost has to be less than or equal to a budget level. Computational tests are performed on a real-life case study prepared in collaboration with the U.S. Army Corps of Engineers (USACE). Our initial investigations show that the pure CP model is very efficient in obtaining good quality feasible solutions but, fails to report the optimal solution for the majority of the problem instances. On the other hand, the two logic-based Benders decomposition algorithms are able to obtain near optimal solutions for 86 instances out of 90 examinees. For the remaining instances, they provide a feasible solution. Further investigations show the high quality of the solutions obtained by the pure CP model

Real time observation of cuprates structural dynamics by Ultrafast Electron Crystallography

The phonon-mediated attractive interaction between carriers leads to the Cooper pair formation in conventional superconductors. Despite decades of research, the glue holding Cooper pairs in high-temperature superconducting cuprates is still controversial, and the same is true as for the relative involvement of structural and electronic degrees of freedom. Ultrafast electron crystallography (UEC) offers, through observation of spatio-temporally resolved diffraction, the means for determining structural dynamics and the possible role of electron-lattice interaction. A polarized femtosecond (fs) laser pulse excites the charge carriers, which relax through electron-electron and electron-phonon coupling, and the consequential structural distortion is followed diffracting fs electron pulses. In this review, the recent findings obtained on cuprates are summarized. In particular, we discuss the strength and symmetry of the directional electron-phonon coupling in Bi2Sr2CaCu2O8+\delta (BSCCO), as well as the c-axis structural instability induced by near-infrared pulses in La2CuO4 (LCO). The theoretical implications of these results are discussed with focus on the possibility of charge stripes being significant in accounting for the polarization anisotropy of BSCCO, and cohesion energy (Madelung) calculations being descriptive of the c-axis instability in LCO

4D visualization of embryonic, structural crystallization by single-pulse microscopy

In many physical and biological systems the transition from an amorphous to ordered native structure involves complex energy landscapes, and understanding such transformations requires not only their thermodynamics but also the structural dynamics during the process. Here, we extend our 4D visualization method with electron imaging to include the study of irreversible processes with a single pulse in the same ultrafast electron microscope (UEM) as used before in the single-electron mode for the study of reversible processes. With this augmentation, we report on the transformation of amorphous to crystalline structure with silicon as an example. A single heating pulse was used to initiate crystallization from the amorphous phase while a single packet of electrons imaged selectively in space the transformation as the structure continuously changes with time. From the evolution of crystallinity in real time and the changes in morphology, for nanosecond and femtosecond pulse heating, we describe two types of processes, one that occurs at early time and involves a nondiffusive motion and another that takes place on a longer time scale. Similar mechanisms of two distinct time scales may perhaps be important in biomolecular folding

Invariant quantum discord in qubit-qutrit systems under local dephasing

We investigate the dynamics of quantum discord and entanglement for a class of mixed qubit-qutrit states assuming that only the qutrit is under the action of a dephasing channel. We demonstrate that even though the entanglement in the qubit-qutrit state disappears in a finite time interval, partial coherence left in the system enables quantum discord to remain invariant throughout the whole time evolution