Sterically stabilized lock and key colloids: A self-consistent field theory study

A self-consistent field theory study of lock and key type interactions between sterically stabilized colloids in polymer solution is performed. Both the key particle and the lock cavity are assumed to have cylindrical shape, and their surfaces are uniformly grafted with polymer chains. The lock-key potential of mean force is computed for various model parameters, such as length of free and grafted chains, lock and key size matching, free chain volume fraction, grafting density, and various enthalpic interactions present in the system. The lock-key interaction is found to be highly tunable, which is important in the rapidly developing field of particle self-assembly

Incoherent excitation and switching of spin states in exciton-polariton condensates

We investigate, theoretically and numerically, the spin dynamics of a two-component exciton-polariton condensate created and sustained by non-resonant spin-polarized optical pumping of a semiconductor microcavity. Using the open-dissipative mean-field model, we show that the existence of well defined phase-locked steady states of the condensate may lead to efficient switching and control of spin (polarization) states with a non-resonant excitation. Spatially inhomogeneous pulsed excitations can cause symmetry breaking in the pseudo-spin structure of the condensate and lead to formation of non-trivial spin textures. Our model is universally applicable to two weakly coupled polariton condensates, and therefore can also describe the behaviour of condensate populations and phases in 'double-well' type potentials

Hysteresis in the de Haas-van Alphen Effect

A hysteresis loop is observed for the first time in the de Haas-van Alphen (dHvA) effect of beryllium at low temperatures and quantizing magnetic field applied parallel to the hexagonal axis of the single crystal. The irreversible behavior of the magnetization occurs at the paramagnetic part of the dHvA period in conditions of Condon domain formation arising by strong enough dHvA amplitude. The resulting extremely nonlinear response to a very small modulation field offers the possibility to find in a simple way the Condon domain phase diagram. From a harmonic analysis, the shape and size of the hysteresis loop is constructed.Comment: 4 pages, 5 figures, submitted to PR

Direct Observation of Condon Domains in Silver by Hall Probes

Using a set of micro Hall probes for the detection of the local induction, the inhomogeneous Condon domain structure has been directly observed at the surface of a pure silver single crystal under strong Landau quantization in magnetic fields up to 10 T. The inhomogeneous induction occurs in the theoretically predicted part of the H-T Condon domain phase diagram. Information about size, shape and orientation of the domains is obtained by analyzing Hall probes placed along and across the long sample axis and by tilting the sample. On a beryllium surface the induction inhomogeneity is almost absent although the expected induction splitting here is at least ten times higher than in silver.Comment: 4 pages, 6 figures, submitted to PR

59Co NMR study of the Co states in superconducting and anhydrous cobaltates

$^{59}$Co NMR spectra in oriented powders of Na$_{0.35}$CoO$_{2}$ and in its hydrated superconducting phase (HSC) Na$_{0.35}$CoO$_{2}$,1.3H$_{2}$O reveal a single electronic Co state with identical $T$ independent NMR shift tensor. These phases differ markedly from Na$_{0.7}$CoO$_{2}$, in which we resolve 3 types of Co sites. The large T variation of their spin susceptibilities $\chi ^{s}$ and the anisotropy of the orbital susceptibility $\chi ^{orb}$ allow us to conclude that charge disproportionation occurs, in a non magnetic Co$^{3+}$ and two magnetic sites with about 0.3 and 0.7 holes in the $t_{2g}$ multiplet. The data are consistent with those for the single Co site in the anhydrous and HSC phase assuming the expected Co$^{3.65+}$ charge.Comment: 5 pages, 3 figures, accepted for publication in Phys. Rev. Let

Compton scattering sequence reconstruction algorithm for the liquid xenon gamma-ray imaging telescope (LXeGRIT)

The Liquid Xenon Gamma-Ray Imaging Telescope (LXeGRIT) is a balloon born experiment sensitive to \g -rays in the energy band of 0.2-20 MeV. The main detector is a time projection chamber filled with high purity liquid xenon (LXeTPC), in which the three-dimensional location and energy deposit of individual \g -ray interactions are accurately measured in one homogeneous volume. To determine the \g -ray initial direction (Compton imaging), as well as to reject background, the correct sequence of interactions has to be determined. Here we report the development and optimization of an algorithm to reconstruct the Compton scattering sequence and show its performance on Monte Carlo events and LXeGRIT data.Comment: To appear in: Hard X-Ray, Gamma-Ray, and Neutron Detector Physics II, 2000; Proc. SPIE, vol. 4141; R.B. James & R.C. Schirato, ed