496 research outputs found
Selective coherence transfers in homonuclear dipolar coupled spin systems
Mapping the physical dipolar Hamiltonian of a solid-state network of nuclear
spins onto a system of nearest-neighbor couplings would be extremely useful for
a variety of quantum information processing applications, as well as NMR
structural studies. We demonstrate such a mapping for a system consisting of an
ensemble of spin pairs, where the coupling between spins in the same pair is
significantly stronger than the coupling between spins on different pairs. An
amplitude modulated RF field is applied on resonance with the Larmor frequency
of the spins, with the frequency of the modulation matched to the frequency of
the dipolar coupling of interest. The spin pairs appear isolated from each
other in the regime where the RF power (omega_1) is such that omega_weak <<
omega_1 << omega_strong. Coherence lifetimes within the two-spin system are
increased from 19 us to 11.1 ms, a factor of 572.Comment: 4 pages. Paper re-submitted with minor changes to clarify that the
scheme demonstrated is not an exact mapping onto a nearest neighbor system.
However, this is the first demonstration of a controlled evolution in a
subspace of an extended spin system, on a timescale that is much larger than
the dipolar dephasing tim
Dynamics of entanglement in a one-dimensional Ising chain
The evolution of entanglement in a one-dimensional Ising chain is numerically
studied under various initial conditions. We analyze two problems concerning
the dynamics of the entanglement: (i) generation of the entanglement from the
pseudopure separable state and (ii) transportation of the entanglement from one
end of the chain to the other. The investigated model is a one-dimensional
Ising spin-1/2 chain with nearest-neighbor interactions placed in an external
magnetic field and irradiated by a weak resonant transverse field. The
possibility of selective initialization of partially entangled states is
considered. It was shown that, in spite of the use of a model with the direct
interactions between the nearest neighbors, the entanglement between remote
spins is generated.Comment: 19 pages, 7 figure
Principles of human movement augmentation and the challenges in making it a reality
Augmenting the body with artificial limbs controlled concurrently to one's natural limbs has long appeared in science fiction, but recent technological and neuroscientific advances have begun to make this possible. By allowing individuals to achieve otherwise impossible actions, movement augmentation could revolutionize medical and industrial applications and profoundly change the way humans interact with the environment. Here, we construct a movement augmentation taxonomy through what is augmented and how it is achieved. With this framework, we analyze augmentation that extends the number of degrees-of-freedom, discuss critical features of effective augmentation such as physiological control signals, sensory feedback and learning as well as application scenarios, and propose a vision for the field
Controlling coherence using the internal structure of hard pi pulses
The tiny difference between hard pi pulses and their delta-function
approximation can be exploited to control coherence. Variants on the magic echo
that work despite a large spread in resonance offsets are demonstrated using
the zeroth- and first-order average Hamiltonian terms, for 13-C NMR in C60. The
29-Si NMR linewidth of Silicon has been reduced by a factor of about 70,000
using this approach, which also has potential applications in magnetic
resonance microscopy and imaging of solids.Comment: 4 pages, 4 color figure
Long-lived memory for mesoscopic quantum bits
We describe a technique to create long-lived quantum memory for quantum bits
in mesoscopic systems. Specifically we show that electronic spin coherence can
be reversibly mapped onto the collective state of the surrounding nuclei. The
coherent transfer can be efficient and fast and it can be used, when combined
with standard resonance techniques, to reversibly store coherent superpositions
on the time scale of seconds. This method can also allow for ``engineering''
entangled states of nuclear ensembles and efficiently manipulating the stored
states. We investigate the feasibility of this method through a detailed
analysis of the coherence properties of the system.Comment: 4 pages, 2 figure
Vortex State of TlBaCuO via Tl NMR at 2 Tesla
We report a Tl NMR study of vortex state for an aligned
polycrystalline sample of an overdoped high- superconductor
TlBaCuO (85 K) with magnetic field 2 T along
the c axis. We observed an imperfect vortex lattice, so-called Bragg glass at
=5 K, coexistence of vortex solid with liquid between 10 and 60 K, and
vortex melting between 65 and 85 K. No evidence for local antiferromagnetic
ordering at vortex cores was found for our sample.Comment: 4 pages with 5 figure
The Intrinsic Origin of Spin Echoes in Dipolar Solids Generated by Strong Pi Pulses
In spectroscopy, it is conventional to treat pulses much stronger than the
linewidth as delta-functions. In NMR, this assumption leads to the prediction
that pi pulses do not refocus the dipolar coupling. However, NMR spin echo
measurements in dipolar solids defy these conventional expectations when more
than one pi pulse is used. Observed effects include a long tail in the CPMG
echo train for short delays between pi pulses, an even-odd asymmetry in the
echo amplitudes for long delays, an unusual fingerprint pattern for
intermediate delays, and a strong sensitivity to pi-pulse phase. Experiments
that set limits on possible extrinsic causes for the phenomena are reported. We
find that the action of the system's internal Hamiltonian during any real pulse
is sufficient to cause the effects. Exact numerical calculations, combined with
average Hamiltonian theory, identify novel terms that are sensitive to
parameters such as pulse phase, dipolar coupling, and system size.
Visualization of the entire density matrix shows a unique flow of quantum
coherence from non-observable to observable channels when applying repeated pi
pulses.Comment: 24 pages, 27 figures. Revised from helpful referee comments. Added
new Table IV, new paragraphs on pages 3 and 1
Second-order shaped pulses for solid-state quantum computation
We present the constructon and detailed analysis of highly-optimized
self-refocusing pulse shapes for several rotation angles. We characterize the
constructed pulses by the coefficients appearing in the Magnus expansion up to
second order. This allows a semi-analytical analysis of the performance of the
constructed shapes in sequences and composite pulses by computing the
corresponding leading-order error operators. Higher orders can be analyzed with
the numerical technique suggested by us previously. We illustrate the technique
by analysing several composite pulses designed to protect against pulse
amplitude errors, and on decoupling sequences for potentially long chains of
qubits with on-site and nearest-neighbor couplings.Comment: 16 pages, 29 figure
Gaps and excitations in fullerides with partially filled bands : NMR study of Na2C60 and K4C60
We present an NMR study of Na2C60 and K4C60, two compounds that are related
by electron-hole symmetry in the C60 triply degenerate conduction band. In both
systems, it is known that NMR spin-lattice relaxation rate (1/T1) measurements
detect a gap in the electronic structure, most likely related to
singlet-triplet excitations of the Jahn-Teller distorted (JTD) C60^{2-} or
C60^{4-}. However, the extended temperature range of the measurements presented
here (10 K to 700 K) allows to reveal deviations with respect to this general
trend, both at high and low temperatures. Above room temperature, 1/T1 deviates
from the activated law that one would expect from the presence of the gap and
saturates. In the same temperature range, a lowering of symmetry is detected in
Na2C60 by the appearance of quadrupole effects on the 23Na spectra. In K4C60,
modifications of the 13C spectra lineshapes also indicate a structural
modification. We discuss this high temperature deviation in terms of a coupling
between JTD and local symmetry. At low temperatures, 1/TT tends to a
constant value for Na2C60, both for 13C and 23Na NMR. This indicates a residual
metallic character, which emphasizes the proximity of metallic and insulting
behaviors in alkali fullerides.Comment: 12 pages, 13 figure
Charge Order Driven spin-Peierls Transition in NaV2O5
We conclude from 23Na and 51V NMR measurements in NaxV2O5(x=0.996) a charge
ordering transition starting at T=37 K and preceding the lattice distortion and
the formation of a spin gap Delta=106 K at Tc=34.7 K. Above Tc, only a single
Na site is observed in agreement with the Pmmn space group of this first
1/4-filled ladder system. Below Tc=34.7 K, this line evolves into eight
distinct 23Na quadrupolar split lines, which evidences a lattice distortion
with, at least, a doubling of the unit cell in the (a,b) plane. A model for
this unique transition implying both charge density wave and spin-Peierls order
is discussed.Comment: 4 pages, 3 figures, submitted to Phys. Rev. Let
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