Full Quantum Analysis of Two-Photon Absorption Using Two-Photon Wavefunction: Comparison with One-Photon Absorption

For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon absorption can be substantially enhanced by adjusting the time correlation of photon pairs. We study two typical cases: Gaussian wavefunction and rectangular wavefunction. In the latter, we find that under special conditions one-photon transition is completely suppressed while the high probability of two-photon transition is maintained.Comment: 6 pages, 4 figure

Photon number resolution using a time-multiplexed single-photon detector

Photon number resolving detectors are needed for a variety of applications including linear-optics quantum computing. Here we describe the use of time-multiplexing techniques that allows ordinary single photon detectors, such as silicon avalanche photodiodes, to be used as photon number-resolving detectors. The ability of such a detector to correctly measure the number of photons for an incident number state is analyzed. The predicted results for an incident coherent state are found to be in good agreement with the results of a proof-of-principle experimental demonstration.Comment: REVTeX4, 6 pages, 8 eps figures, v2: minor changes, v3: changes in response to referee report, appendix added, 1 reference adde

Topological Dirac Semimetal Na3Bi Films in the Ultrathin Limit via Alternating Layer Molecular Beam Epitaxy

Ultrathin films of Na3Bi on insulating substrates are desired for opening a bulk band gap and generating the quantum spin Hall effect from a topological Dirac semimetal, though continuous films in the few nanometer regime have been difficult to realize. Here, we utilize alternating layer molecular beam epitaxy (MBE) to achieve uniform and continuous single crystal films of Na3Bi(0001) on insulating Al2O3(0001) substrates and demonstrate electrical transport on films with 3.8 nm thickness (4 unit cells). The high material quality is confirmed through in situ reflection high-energy electron diffraction (RHEED), scanning tunneling microscopy (STM), x-ray diffraction (XRD), and x-ray photoelectron spectroscopy (XPS). In addition, these films are employed as seed layers for subsequent growth by codeposition, leading to atomic layer-by-layer growth as indicated by RHEED intensity oscillations. These material advances facilitate the pursuit of quantum phenomena in thin films of Dirac semimetals.Comment: 11 pages, 5 figure

Interference in dielectrics and pseudo-measurements

Inserting a lossy dielectric into one arm of an interference experiment acts in many ways like a measurement. If two entangled photons are passed through the interferometer, a certain amount of information is gained about which path they took, and the interference pattern in a coincidence count measurement is suppressed. However, by inserting a second dielectric into the other arm of the interferometer, one can restore the interference pattern. Two of these pseudo-measurements can thus cancel each other out. This is somewhat analogous to the proposed quantum eraser experiments.Comment: 7 pages RevTeX 3.0 + 2 figures (postscript). Submitted to Phys. Rev.

Experimental Controlled-NOT Logic Gate for Single Photons in the Coincidence Basis

We report a proof-of-principle demonstration of a probabilistic controlled-NOT gate for single photons. Single-photon control and target qubits were mixed with a single ancilla photon in a device constructed using only linear optical elements. The successful operation of the controlled-NOT gate relied on post-selected three-photon interference effects which required the detection of the photons in the output modes.Comment: 4 pages, 4 figures; minor change

Clock synchronization with dispersion cancellation

The dispersion cancellation feature of pulses which are entangled in frequency is employed to synchronize clocks of distant parties. The proposed protocol is insensitive to the pulse distortion caused by transit through a dispersive medium. Since there is cancellation to all orders, also the effects of slowly fluctuating dispersive media are compensated. The experimental setup can be realized with currently available technology, at least for a proof of principle.Comment: 4 pages, 3 figure

Violation of Bell's Inequality with Photons from Independent Sources

We report a violation of Bell's inequality using one photon from a parametric down-conversion source and a second photon from an attenuated laser beam. The two photons were entangled at a beam splitter using the post-selection technique of Shih and Alley [Phys. Rev. Lett. 61, 2921 (1988)]. A quantum interference pattern with a visibility of 91% was obtained using the photons from these independent sources, as compared with a visibility of 99.4% using two photons from a central parametric down-conversion source.Comment: 4 pages, 5 figures; minor change

Quantum-inspired interferometry with chirped laser pulses

We introduce and implement an interferometric technique based on chirped femtosecond laser pulses and nonlinear optics. The interference manifests as a high-visibility (> 85%) phase-insensitive dip in the intensity of an optical beam when the two interferometer arms are equal to within the coherence length of the light. This signature is unique in classical interferometry, but is a direct analogue to Hong-Ou-Mandel quantum interference. Our technique exhibits all the metrological advantages of the quantum interferometer, but with signals at least 10^7 times greater. In particular we demonstrate enhanced resolution, robustness against loss, and automatic dispersion cancellation. Our interferometer offers significant advantages over previous technologies, both quantum and classical, in precision time delay measurements and biomedical imaging.Comment: 6 pages, 4 figure

Entanglement from longitudinal and scalar photons

The covariant quantization of the electromagnetic field in the Lorentz gauge gives rise to longitudinal and scalar photons in addition to the usual transverse photons. It is shown here that the exchange of longitudinal and scalar photons can produce entanglement between two distant atoms or harmonic oscillators. The form of the entangled states produced in this way is very different from that obtained in the Coulomb gauge, where the longitudinal and scalar photons do not exist. A generalized gauge transformation is used to show that all physically observable effects are the same in the two gauges, despite the differences in the form of the entangled states. An approach of this kind may be useful for a covariant description of the dynamics of quantum information processing.Comment: 12 pages, 1 figur