Thermodynamic phase transitions in a frustrated magnetic metamaterial

The research leading to these results has received funding from the European Community’s Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 290605 (COFUND: PSI-FELLOW) and from the EPSRC (grant EP/J01060X).Materials with interacting magnetic degrees of freedom display a rich variety of magnetic behaviour that can lead to novel collective equilibrium and out-of-equilibrium phenomena. In equilibrium, thermodynamic phases appear with the associated phase transitions providing a characteristic signature of the underlying collective behaviour. Here we create a thermally active artificial kagome spin ice that is made up of a large array of dipolar interacting nanomagnets and undergoes phase transitions predicted by microscopic theory. We use low energy muon spectroscopy to probe the dynamic behaviour of the interacting nanomagnets and observe peaks in the muon relaxation rate that can be identified with the critical temperatures of the predicted phase transitions. This provides experimental evidence that a frustrated magnetic metamaterial can be engineered to admit thermodynamic phases.Publisher PDFPeer reviewe

Control of superconductivity with a single ferromagnetic layer in niobium/erbium bilayers

Superconducting spintronics in hybrid superconductor{ferromagnet (S{F) heterostructures provides an exciting potential new class of device. The prototypical super-spintronic device is the superconducting spin-valve, where the critical temperature, Tc, of the S-layer can be controlledby the relative orientation of two (or more) F-layers. Here, we show that such control is also possible in a simple S/F bilayer. Using eld history to set the remanent magnetic state of a thin Er layer, we demonstrate for a Nb/Er bilayer a high level of control of both Tc and the shape of the resistive transition, R(T), to zero resistance. We are able to model the origin of the remanent magnetization, treating it as an increase in the e ective exchange eld of the ferromagnet and link this, using conventional S{F theory, to the suppression of Tc. We observe stepped features in the R(T) which we argue is due to a fundamental interaction of superconductivity with inhomogeneous ferromagnetism, a phenomena currently lacking theoretical description

Continuously tuneable critical current in superconductor-ferromagnet multilayers

We demonstrate that the critical current of superconducting Nb/Ni multilayers can be continuously tuned by up to a factor of three during magnetization reversal of the Ni films under an applied in-plane magnetic field. Our observations are in reasonably good agreement with a model of vortex pinning by Bloch domain walls that proliferate in the samples during magnetization reversal, whereby each vortex interacts with at most one wall in any of the Ni layers. Our model suggests ways in which the controllable pinning effect could be significantly enhanced, with important potential applications in tuneable superconducting devices

Intrinsic Paramagnetic Meissner Effect due to s-wave Odd-Frequency Superconductivity

In 1933, Meissner and Ochsenfeld reported the expulsion of magnetic flux, the diamagnetic Meissner effect, from the interior of superconducting lead. This discovery was crucial in formulating the Bardeen-Cooper-Schrieffer (BCS) theory of superconductivity. In exotic superconducting systems BCS theory does not strictly apply. A classical example is a superconductor-magnet hybrid system where magnetic ordering breaks time-reversal symmetry of the superconducting condensate and results in the stabilisation of an odd-frequency superconducting state. It has been predicted that under appropriate conditions, odd-frequency superconductivity should manifest in the Meissner state as fluctuations in the sign of the magnetic susceptibility meaning that the superconductivity can either repel (diamagnetic) or attract (paramagnetic) external magnetic flux. Here we report local probe measurements of faint magnetic fields in a Au/Ho/Nb trilayer system using low energy muons, where antiferromagnetic Ho (4.5 nm) breaks time-reversal symmetry of the proximity induced pair correlations in Au. From depth-resolved measurements below the superconducting transition of Nb we observe a local enhancement of the magnetic field in Au that exceeds the externally applied field, thus proving the existence of an intrinsic paramagnetic Meissner effect arising from an odd-frequency superconducting state.publishe

Research data supporting "Muon spectroscopy data on Au/Ho/Nb thin films"

Measurements data collected at Paul Scherrer Institute showing a paramagnetic Meissner effect due to odd-frequency superconductivity. The data were collected at Paul Scherrer Insitute by performing low-energy spectroscopy on Au/Ho/Nb thin film samples.This record supports publication and is available at http://journals.aps.org/prx/abstract/10.1103/PhysRevX.5.041021This work was supported by the EPSRC, Engineering and Physical Sciences Research Council [FundRef ID http://dx.doi.org/10.13039/501100000266], Royal Society [FundRef ID http://dx.doi.org/10.13039/501100000288] and the Leverhulme Trust [FundRef ID http://dx.doi.org/10.13039/501100000275]

Beating the Stoner criterion using molecular interfaces

Only three elements are ferromagnetic at room temperature: the transition metals iron, cobalt and nickel. The Stoner criterion explains why iron is ferromagnetic but manganese, for example, is not, even though both elements have an unfilled 3d shell and are adjacent in the periodic table: according to this criterion, the product of the density of states and the exchange integral must be greater than unity for spontaneous spin ordering to emerge. Here we demonstrate that it is possible to alter the electronic states of non-ferromagnetic materials, such as diamagnetic copper and paramagnetic manganese, to overcome the Stoner criterion and make them ferromagnetic at room temperature. This effect is achieved via interfaces between metallic thin films and C60 molecular layers. The emergent ferromagnetic state exists over several layers of the metal before being quenched at large sample thicknesses by the materiala € s bulk properties. Although the induced magnetization is easily measurable by magnetometry, low-energy muon spin spectroscopy provides insight into its distribution by studying the depolarization process of low-energy muons implanted in the sample. This technique indicates localized spin-ordered states at, and close to, the metal-molecule interface. Density functional theory simulations suggest a mechanism based on magnetic hardening of the metal atoms, owing to electron transfer. This mechanism might allow for the exploitation of molecular coupling to design magnetic metamaterials using abundant, non-toxic components such as organic semiconductors. Charge transfer at molecular interfaces may thus be used to control spin polarization or magnetization, with consequences for the design of devices for electronic, power or computing applications (see, for example, refs 6 and 7)

Data underpinning: Manifestation of the electromagnetic proximity effect in superconductor-ferromagnet thin film structures

M(H) squid data; LEM stopping profiles and raw data sets (in .root and .nemu format

Data underpinning: Observation of Anomalous Meissner Screening in Cu=Nb and Cu=Nb=Co Thin Films

R(T) and Hc2(T) transport data; LEM stopping profiles and raw data sets (in .root and .nemu format