24,446 research outputs found
Magnetization profile for impurities in graphene nanoribbons
The magnetic properties of graphene-related materials and in particular the
spin-polarised edge states predicted for pristine graphene nanoribbons (GNRs)
with certain edge geometries have received much attention recently due to a
range of possible technological applications. However, the magnetic properties
of pristine GNRs are not predicted to be particularly robust in the presence of
edge disorder. In this work, we examine the magnetic properties of GNRs doped
with transition-metal atoms using a combination of mean-field Hubbard and
Density Functional Theory techniques. The effect of impurity location on the
magnetic moment of such dopants in GNRs is investigated for the two principal
GNR edge geometries - armchair and zigzag. Moment profiles are calculated
across the width of the ribbon for both substitutional and adsorbed impurities
and regular features are observed for zigzag-edged GNRs in particular. Unlike
the case of edge-state induced magnetisation, the moments of magnetic
impurities embedded in GNRs are found to be particularly stable in the presence
of edge disorder. Our results suggest that the magnetic properties of
transition-metal doped GNRs are far more robust than those with moments arising
intrinsically due to edge geometry.Comment: submitte
Impurity segregation in graphene nanoribbons
The electronic properties of low-dimensional materials can be engineered by
doping, but in the case of graphene nanoribbons (GNR) the proximity of two
symmetry-breaking edges introduces an additional dependence on the location of
an impurity across the width of the ribbon. This introduces energetically
favorable locations for impurities, leading to a degree of spatial segregation
in the impurity concentration. We develop a simple model to calculate the
change in energy of a GNR system with an arbitrary impurity as that impurity is
moved across the ribbon and validate its findings by comparison with ab initio
calculations. Although our results agree with previous works predicting the
dominance of edge disorder in GNR, we argue that the distribution of adsorbed
impurities across a ribbon may be controllable by external factors, namely an
applied electric field. We propose that this control over impurity segregation
may allow manipulation and fine-tuning of the magnetic and transport properties
of GNRs.Comment: 5 pages, 4 figures, submitte
Two-component mixture of charged particles confined in a channel: melting
The melting of a binary system of charged particles confined in a {\it
quasi}-one-dimensional parabolic channel is studied through Monte Carlo
simulations. At zero temperature the particles are ordered in parallel chains.
The melting is anisotropic and different melting temperatures are obtained
according to the spatial direction, and the different types of particles
present in the system. Melting is very different for the single-, two- and
four-chain configurations. A temperature induced structural phase transition is
found between two different four chain ordered states which is absent in the
mono-disperse system. In the mixed regime, where the two types of particles are
only slightly different, melting is almost isotropic and a thermally induced
homogeneous distribution of the distinct types of charges is observed.Comment: To appear in Journal of Physics: condensed matter ; (13 pages, 12
figures
Exponential behavior of the interlayer exchange coupling across non-magnetic metallic superlattices
It is shown that the coupling between magnetic layers separated by
non-magnetic metallic superlattices can decay exponentially as a function of
the spacer thickness , as opposed to the usual decay. This effect
is due to the lack of constructive contributions to the coupling from extended
states across the spacer. The exponential behavior is obtained by properly
choosing the distinct metals and the superlattice unit cell composition.Comment: To appear in Phys. Rev.
Analytical results for long time behavior in anomalous diffusion
We investigate through a Generalized Langevin formalism the phenomenon of
anomalous diffusion for asymptotic times, and we generalized the concept of the
diffusion exponent. A method is proposed to obtain the diffusion coefficient
analytically through the introduction of a time scaling factor . We
obtain as well an exact expression for for all kinds of diffusion.
Moreover, we show that is a universal parameter determined by the
diffusion exponent. The results are then compared with numerical calculations
and very good agreement is observed. The method is general and may be applied
to many types of stochastic problem
Light scattering by a medium with a spatially modulated optical conductivity: the case of graphene
We describe light scattering from a graphene sheet having a modulated optical
conductivity. We show that such modulation enables the excitation of surface
plasmon-polaritons by an electromagnetic wave impinging at normal incidence.
The resulting surface plasmon-polaritons are responsible for a substantial
increase of electromagnetic radiation absorption by the graphene sheet. The
origin of the modulation can be due either to a periodic strain field or to
adatoms (or absorbed molecules) with a modulated adsorption profile.Comment: http://iopscience.iop.org/0953-8984/24/24/24530
The effect of heat pretreatment on the analysis of bacterial community for fermentative hydrogen production.
Avaliação sensorial de variedades de mandioca de mesa com raízes de cores diversas.
Este trabalho teve como objetivo avaliar a aceitabilidade de uma cultivar de raiz de cor amarela provavelmente com maior teor de carotenóides, através de teste sensorial em escala hedônica, por consumidores que têm preferência cultural por mandioca de mesa de raiz com cor variando de branca a creme
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