Attosecond two-photon interferometry for doubly excited states of helium

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto experimentally easily accessible non-coincident single electron spectra. We analyze the interferometric signal in terms of a semi-analytical model which is validated by a numerical solution of the time-dependent two-electron Schr\"odinger equation in its full dimensionality.Comment: 5 pages, 4 figure

Probing Electron Correlation via Attosecond XUV Pulses in the Two-Photon Double Ionization of Helium

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime (photon energy above 54.4 eV) in the two-photon double ionization of helium. We show that attosecond pulses allow to induce and probe angular and energy correlations of the emitted electrons. The final momentum distribution reveals regions dominated by the Wannier ridge break-up scenario and by post-collision interaction.Comment: 4 pages, 5 figure

Claytonia virginica L.

https://thekeep.eiu.edu/herbarium_specimens_byname/5143/thumbnail.jp

Tailored high-contrast attosecond electron pulses for coherent excitation and scattering

Temporally shaping the density of electron beams using light forms the basis for a wide range of established and emerging technologies, including free-electron lasers and attosecond electron microscopy. The modulation depth of compressed electron pulses is a key figure of merit limiting applications. In this work, we present an approach for generating background-free attosecond electron pulse trains by sequential inelastic electron-light scattering. Harnessing quantum interference in the fractional Talbot effect, we suppress unwanted background density in electron compression by several orders of magnitude. Our results will greatly enhance applications of coherent electron-light scattering, such as stimulated cathodoluminescence and streaking

Nano-wires with surface disorder: Giant localization lengths and dynamical tunneling in the presence of directed chaos

We investigate electron quantum transport through nano-wires with one-sided surface roughness in the presence of a perpendicular magnetic field. Exponentially diverging localization lengths are found in the quantum-to-classical crossover regime, controlled by tunneling between regular and chaotic regions of the underlying mixed classical phase space. We show that each regular mode possesses a well-defined mode-specific localization length. We present analytic estimates of these mode localization lengths which agree well with the numerical data. The coupling between regular and chaotic regions can be determined by varying the length of the wire leading to intricate structures in the transmission probabilities. We explain these structures quantitatively by dynamical tunneling in the presence of directed chaos.Comment: 15 pages, 12 figure

Thermalization and Cooling of Plasmon-Exciton Polaritons: Towards Quantum Condensation

We present indications of thermalization and cooling of quasi-particles, a precursor for quantum condensation, in a plasmonic nanoparticle array. We investigate a periodic array of metallic nanorods covered by a polymer layer doped with an organic dye at room temperature. Surface lattice resonances of the array---hybridized plasmonic/photonic modes---couple strongly to excitons in the dye, and bosonic quasi-particles which we call plasmon-exciton-polaritons (PEPs) are formed. By increasing the PEP density through optical pumping, we observe thermalization and cooling of the strongly coupled PEP band in the light emission dispersion diagram. For increased pumping, we observe saturation of the strong coupling and emission in a new weakly coupled band, which again shows signatures of thermalization and cooling.Comment: 8 pages, 5 figures including supplemental material. The newest version includes new measurements and corrections to the interpretation of the result

Nano-wires with surface disorder: Giant localization lengths and quantum-to-classical crossover

We investigate electronic quantum transport through nano-wires with one-sided surface roughness. A magnetic field perpendicular to the scattering region is shown to lead to exponentially diverging localization lengths in the quantum-to-classical crossover regime. This effect can be quantitatively accounted for by tunneling between the regular and the chaotic components of the underlying mixed classical phase space.Comment: 4 pages, 3 figures; final version (including added references

Structural dynamics probed by high-coherence electron pulses

Ultrafast measurement technology provides essential contributions to our understanding of the properties and functions of solids and nanostructures. Atomic-scale vistas with ever-growing spatial and temporal resolution are offered by methods based on short pulses of x-rays and electrons. Time-resolved electron diffraction and microscopy are among the most powerful approaches to investigate nonequilibrium structural dynamics. In this article, we discuss recent advances in ultrafast electron imaging enabled by significant improvements in the coherence of pulsed electron beams. Specifically, we review the development and first application of ultrafast low-energy electron diffraction for the study of structural dynamics at surfaces, and discuss novel opportunities for ultrafast transmission electron microscopy facilitated by laser-triggered field-emission sources. These and further developments will render coherent electron beams an essential component in future ultrafast nanoscale imaging