565 research outputs found
Dynamics of cluster deposition on Ar surface
Using a combined quantum mechanical/classical method, we study the dynamics
of deposition of small Na clusters on Ar(001) surface. We work out basic
mechanisms by systematic variation of substrate activity, impact energy,
cluster orientations, cluster sizes, and charges. The soft Ar material is found
to serve as an extremely efficient shock absorber which provides cluster
capture in a broad range of impact energies. Reflection is only observed in
combination with destruction of the substrate. The kinetic energy of the
impinging cluster is rapidly transfered at first impact. The distribution of
the collision energy over the substrate proceeds very fast with velocity of
sound. The full thermalization of ionic and atomic energies goes at a much
slower pace with times of several ps. Charged clusters are found to have a much
stronger interface interaction and thus get in significantly closer contact
with the surface.Comment: 10 pages, 6 figures, accepted in Euro. Phys. J.
Hindered Coulomb explosion of embedded Na clusters -- stopping, shape dynamics and energy transport
We investigate the dynamical evolution of a Na cluster embedded in Ar
matrices of various sizes from N=30 to 1048. The system is excited by an
intense short laser pulse leading to high ionization stages. We analyze the
subsequent highly non-linear motion of cluster and Ar environment in terms of
trajectories, shapes, and energy flow. The most prominent effects are:
temporary stabilization of high charge states for several ps, sudden stopping
of the Coulomb explosion of the embedded Na clusters associated with an
extremely fast energy transfer to the Ar matrix, fast distribution of energy
throughout the Ar layers by a sound wave. Other ionic-atomic transfer and
relaxation processes proceed at slower scale of few ps. The electron cloud is
almost thermally decoupled from ions and thermalizes far beyond the ps scale.Comment: 12 pages, 10 figures, accepted in Euro. Phys. J.
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