Quantum interference in laser-induced nonsequential double ionization in diatomic molecules: the role of alignment and orbital symmetry

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work within the strong-field approximation and assume that the second electron is dislodged by electron-impact ionization, and also consider the classical limit of this model. We show that the electron-momentum distributions exhibit interference maxima and minima due to the electron emission at spatially separated centers. The interference patterns survive the integration over the transverse momenta for a small range of alignment angles, and are sharpest for parallel-aligned molecules. Due to the contributions of transverse-momentum components, these patterns become less defined as the alignment angle increases, until they disappear for perpendicular alignment. This behavior influences the shapes and the peaks of the electron momentum distributions.Comment: 12 pages, 7 figures; some discussions have been extended and some figures slightly modifie

Laser-induced nonsequential double ionization: kinematic constraints for the recollision-excitation-tunneling mechanism

We investigate the physical processes in which an electron, upon return to its parent ion, promotes a second electron to an excited state, from which it subsequently tunnels. Employing the strong-field approximation and saddle-point methods, we perform a detailed analysis of the dynamics of the two electrons, in terms of quantum orbits, and delimit constraints for their momentum components parallel to the laser-field polarization. The kinetic energy of the first electron, upon return, exhibits a cutoff slightly lower than $10U_p$, where $U_p$ is the ponderomotive energy, as in rescattered above-threshold ionization (ATI). The second electron leaves the excited state in a direct ATI-like process, with the maximal energy of $2U_p$. We also compute electron-momentum distributions, whose maxima agree with our estimates and with other methods.Comment: 13 pages, 4 figure