31,337 research outputs found

    Out of plane effect on the superconductivity of Sr2-xBaxCuO3+y with Tc up to 98K

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    A series of new Sr2-xBaxCuO3+y (0 x 0.6) superconductors were prepared using high-pressure and high-temperature synthesis. A Rietveld refinement based on powder x-ray diffraction confirms that the superconductors crystallize in the K2NiF4-type structure of a space group I4/mmm similar to that of La2CuO4 but with partially occupied apical oxygen sites. It is found that the superconducting transition temperature Tc of this Ba substituted Sr2CuO3+y superconductor with constant carrier doping level, i.e., constant d, is controlled not only by order/disorder of apical-O atoms but also by Ba content. Tcmax =98 K is achieved in the material with x=0.6 that reaches the record value of Tc among the single-layer copper oxide superconductors, and is higher than Tc=95K of Sr2CuO3+y with optimally ordered apical-O atoms. There is Sr-site disorder in Sr2-xBaxCuO3+y which might lead to a reduction of Tc. The result indicates that another effect surpasses the disorder effect that is related either to the increased in-plane Cu-O bond length or to elongated apical-O distance due to Ba substitution with larger cation size. The present experiment demonstrates that the optimization of local geometry out of the Cu-O plane can dramatically enhance Tc in the cuprate superconductors.Comment: 23 Pages, 1 Table, 5 Figure

    Surface phase separation in nanosized charge-ordered manganites

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    Recent experiments showed that the robust charge-ordering in manganites can be weakened by reducing the grain size down to nanoscale. Weak ferromagnetism was evidenced in both nanoparticles and nanowires of charge-ordered manganites. To explain these observations, a phenomenological model based on surface phase separation is proposed. The relaxation of superexchange interaction on the surface layer allows formation of a ferromagnetic shell, whose thickness increases with decreasing grain size. Possible exchange bias and softening of the ferromagnetic transition in nanosized charge-ordered manganites are predicted.Comment: 4 pages, 3 figure

    Consistency of shared reference frames should be reexamined

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    In a recent Letter [G. Chiribella et al., Phys. Rev. Lett. 98, 120501 (2007)], four protocols were proposed to secretly transmit a reference frame. Here We point out that in these protocols an eavesdropper can change the transmitted reference frame without being detected, which means the consistency of the shared reference frames should be reexamined. The way to check the above consistency is discussed. It is shown that this problem is quite different from that in previous protocols of quantum cryptography.Comment: 3 pages, 1 figure, comments are welcom
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