346 research outputs found
Yttria and Ceria Doped Zirconia Thin Films Grown by Pulsed Laser Deposition
The Yttria stabilized Zirconia (YSZ) is a standard electrolyte for solid oxide fuel cells (SOFCs), which are potential candidates for next generation portable and mobile power sources. YSZ electrolyte thin films having a cubic single phase allow reducing the SOFC operating temperature without diminishing the electrochemical power density. Films of 8 mol % Yttria stabilized Zirconia (8YSZ) and films with addition of 4 weight % Ceria (8YSZ + 4CeO2) were grown by pulsed laser deposition (PLD) technique using 8YSZ and 8YSZ + 4CeO2 targets and a Nd-YAG laser (355 nm). Films have been deposited on Soda-Calcia-Silica glass and Si(100) substrates at room temperature. The morphology and structural characteristics of the samples have been studied by means of X-ray diffraction and scanning electron microscopy. Films of a cubic-YSZ single phase with thickness in the range of 1-3 µm were grown on different substrates.Fil: Saporiti, F.. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Ingeniería Mecánica. Grupo de Materiales Avanzados; Argentina;Fil: Juarez, R. E.. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Ingeniería Mecánica. Grupo de Materiales Avanzados; Argentina;Fil: Audebert, Fernando Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Houssay. Instituto de Tecnologías y Ciencias de la Ingeniería; Argentina; Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Ingeniería Mecánica. Grupo de Materiales Avanzados; Argentina;Fil: Boudard, M.. Centre National de la Recherche Scientifique. Laboratoire des Matériaux et du Génie Physique; Francia
Measurement of nuclide cross-sections of spallation residues in 1 A GeV 238U + proton collisions
The production of heavy nuclides from the spallation-evaporation reaction of
238U induced by 1 GeV protons was studied in inverse kinematics. The
evaporation residues from tungsten to uranium were identified in-flight in mass
and atomic number. Their production cross-sections and their momentum
distributions were determined. The data are compared with empirical
systematics. A comparison with previous results from the spallation of 208Pb
and 197Au reveals the strong influence of fission in the spallation of 238U.Comment: 20 pages, 10 figures, background information at
http://www-wnt.gsi.de/kschmidt
Singlet-to-triplet ratio in the deuteron breakup reaction at 585 MeV
Available experimental data on the exclusive reaction at 585 MeV
show a narrow peak in the proton-neutron final-state interaction region. It was
supposed previously, on the basis of a phenomenological analysis of the shape
of this peak, that the final spin-singlet state provided about one third
of the observed cross section. By comparing the absolute value of the measured
cross section with that of elastic scattering using the F\"aldt-Wilkin
extrapolation theorem, it is shown here that the data can be
explained mainly by the spin-triplet final state with a singlet admixture of a
few percent. The smallness of the singlet contribution is compatible with
existing data and the one-pion exchange mechanism of the reaction.Comment: 10 pages, Latex, 2 Postscript figure
Isotopic and velocity distributions of Bi produced in charge-pickup reactions of 208Pb at 1 A GeV
Isotopically resolved cross sections and velocity distributions have been
measured in charge-pickup reactions of 1 A GeV 208Pb with proton, deuterium and
titanium target. The total and partial charge-pickup cross sections in the
reactions 208Pb + 1H and 208Pb + 2H are measured to be the same in the limits
of the error bars. A weak increase in the total charge-pickup cross section is
seen in the reaction of 208Pb with the titanium target. The measured velocity
distributions show different contributions - quasi-elastic scattering and
Delta-resonance excitation - to the charge-pickup production. Data on total and
partial charge-pickup cross sections from these three reactions are compared
with other existing data and also with model calculations based on the coupling
of different intra-nuclear cascade codes and an evaporation code.Comment: 20 pages, 12 figures, background information on
http://www-w2k.gsi.de/kschmidt
Fission-Residues Produced in the Spallation Reaction 238U+p at 1 A GeV
Fission fragments from 1 A GeV 238U projectiles irradiating a hydrogen target
were investigated by using the fragment separator FRS for magnetic selection of
reaction products including ray-tracing and DE-ToF techniques. The momentum
spectra of 733 identified fragments were analysed to provide isotopic
production cross sections, fission-fragment velocities and recoil momenta of
the fissioning parent nuclei. Besides their general relevance, these quantities
are also demanded for applications. Calculations and simulations with codes
commonly used and recently developed or improved are compared to the data.Comment: 60 pages, 21 figures, 4 tables, 2 appendices (15 pages
Evaporation residues produced in spallation of 208Pb by protons at 500A MeV
The production cross sections of fragmentation-evaporation residues in the
reaction Pb+p at 500A MeV have been measured using the inverse-kinematics
method and the FRS spectrometer (GSI). Fragments were identified in nuclear
charge using ionisation chambers. The mass identification was performed
event-by-event using the B-rho - TOF - Delta-E technique. Although
partially-unresolved ionic charge states induced an ambiguity on the mass of
some heavy fragments, production rates could be obtained with a high accuracy
by systematically accounting for the polluting ionic charge states. The
contribution of multiple reactions in the target was subtracted using a new,
partly self-consistent code. The isobaric distributions are found to have a
shape very close to the one observed in experiments at higher energy. Kinematic
properties of the fragments were also measured. The total and the isotopic
cross sections, including charge-pickup cross sections, are in good agreement
with previous measurements. The data are discussed in the light of previous
spallation measurements, especially on lead at 1 GeV
Production of medium-mass neutron-rich nuclei in reactions induced by 136Xe projectiles at 1 A GeV on a beryllium target
Production cross sections of medium-mass neutron-rich nuclei obtained in the
fragmentation of 136Xe projectiles at 1 A GeV have been measured with the
FRagment Separator (FRS) at GSI. 125Pd was identified for the first time. The
measured cross sections are compared to 238U fission yields and model
calculations in order to determine the optimum reaction mechanism to extend the
limits of the chart of the nuclides around the r-process waiting point at N=82.Comment: 9 pages, 6 figure
Coincidence measurement of residues and light particles in the reaction 56Fe+p at 1 GeV per nucleon with SPALADIN
The spallation of Fe in collisions with hydrogen at 1 A GeV has been
studied in inverse kinematics with the large-aperture setup SPALADIN at GSI.
Coincidences of residues with low-center-of-mass kinetic energy light particles
and fragments have been measured allowing the decomposition of the total
reaction cross-section into the different possible de-excitation channels.
Detailed information on the evolution of these de-excitation channels with
excitation energy has also been obtained. The comparison of the data with
predictions of several de-excitation models coupled to the INCL4 intra-nuclear
cascade model shows that only GEMINI can reasonably account for the bulk of
collected results, indicating that in a light system with no compression and
little angular momentum, multifragmentation might not be necessary to explain
the data.Comment: 4 pages, 5 figures, revised version accepted in Phys. Rev. Let
Measurement of residual nucleus cross sections and recoil energies in p + Fe collisions at 300, 500, 750, 1000 and 1500 MeV
The production of residual nuclei in p + Fe collisions has been measured at GSI on the FRS facility by means of the reverse kinematic techniques at 300, 500, 750, 1000 and 1500 MeV/A. The cross-sections larger than 0.01 mb of all isotopes with Z larger than 8 have been obtained. Velocity distributions were also measured. Comparisons to models describing spallation reactions and some empirical formulae often used in astrophysics are presented. These data are directly used to calculate impurety production and DPAs in a thin window as foreseen in spallation sources or accelerator-driven systems
Spallation Residues in the Reaction 56Fe + p at 0.3, 0.5, 0.75, 1.0 and 1.5 A GeV
The spallation residues produced in the bombardment of 56}Fe at 1.5, 1.0,
0.75, 0.5 and 0.3 A GeV on a liquid-hydrogen target have been measured using
the reverse kinematics technique and the Fragment Separator at GSI (Darmstadt).
This technique has permitted the full identification in charge and mass of all
isotopes produced with cross-sections larger than 10^{-2} mb down to Z=8. Their
individual production cross-sections and recoil velocities at the five energies
are presented. Production cross-sections are compared to previously existing
data and to empirical parametric formulas, often used in cosmic-ray
astrophysics. The experimental data are also extensively compared to different
combinations of intra-nuclear cascade and de-excitation models. It is shown
that the yields of the lightest isotopes cannot be accounted for by standard
evaporation models. The GEMINI model, which includes an asymmetric fission
decay mode, gives an overall good agreement with the data. These experimental
data can be directly used for the estimation of composition modifications and
damages in materials containing iron in spallation sources. They are also
useful for improving high precision cosmic-ray measurements.Comment: Submited to Phys. Rev. C (10/2006
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