Room-temperature quantum optomechanics using an ultra-low noise cavity

Ponderomotive squeezing of light, where a mechanical oscillator creates quantum correlations between the phase and amplitude of the interacting light field, is a canonical signature of the quantum regime of optomechanics. At room temperature, this has only been reached in pioneering experiments where an optical restoring force controls the oscillator stiffness, akin to the vibrational motion of atoms in an optical lattice. These include both levitated nanoparticles and optically-trapped cantilevers. Recent advances in engineered mechanical resonators, where the restoring force is provided by material rigidity rather than an external optical potential, have realized ultra-high quality factors (Q) by exploiting `soft clamping'. However entering the quantum regime with such resonators, has so far been prevented by optical cavity frequency fluctuations and thermal intermodulation noise. Here, we overcome this challenge and demonstrate optomechanical squeezing at room temperature in a phononic-engineered membrane-in-the-middle system. By using a high finesse cavity whose mirrors are patterned with phononic crystal structures, we reduce cavity frequency noise by more than 700-fold. In this ultra-low noise cavity, we introduce a silicon nitride membrane oscillator whose density is modulated by silicon nano-pillars, yielding both high thermal conductance and a localized mechanical mode with Q of 1.8e8. These advances enable operation within a factor of 2.5 of the Heisenberg limit, leading to squeezing of the probing field by 1.09 dB below the vacuum fluctuations. Moreover, the long thermal decoherence time of the membrane oscillator (more than 30 vibrational periods) allows us to obtain conditional displaced thermal states of motion with an occupation of 0.97 phonon, using a multimode Kalman filter. Our work extends quantum control of engineered macroscopic oscillators to room temperature

Clamp-tapering increases the quality factor of stressed nanobeams

Stressed nanomechanical resonators are known to have exceptionally high quality factors ($Q$) due to the dilution of intrinsic dissipation by stress. Typically, the amount of dissipation dilution and thus the resonator $Q$ is limited by the high mode curvature region near the clamps. Here we study the effect of clamp geometry on the $Q$ of nanobeams made of high-stress $\mathrm{Si_3N_4}$. We find that tapering the beam near the clamp - and locally increasing the stress - leads to increased $Q$ of MHz-frequency low order modes due to enhanced dissipation dilution. Contrary to recent studies of tethered-membrane resonators, we find that widening the clamps leads to decreased $Q$ despite increased stress in the beam bulk. The tapered-clamping approach has practical advantages compared to the recently developed "soft-clamping" technique. Tapered-clamping enhances the $Q$ of the fundamental mode and can be implemented without increasing the device size

Thermal intermodulation noise in cavity-based measurements

Thermal frequency fluctuations in optical cavities limit the sensitivity of precision experiments ranging from gravitational wave observatories to optical atomic clocks. Conventional modeling of these noises assumes a linear response of the optical field to the fluctuations of cavity frequency. Fundamentally, however, this response is nonlinear. Here we show that nonlinearly transduced thermal fluctuations of cavity frequency can dominate the broadband noise in photodetection, even when the magnitude of fluctuations is much smaller than the cavity linewidth. We term this noise "thermal intermodulation noise" and show that for a resonant laser probe it manifests as intensity fluctuations. We report and characterize thermal intermodulation noise in an optomechanical cavity, where the frequency fluctuations are caused by mechanical Brownian motion, and find excellent agreement with our developed theoretical model. We demonstrate that the effect is particularly relevant to quantum optomechanics: using a phononic crystal $Si_3N_4$ membrane with a low mass, soft-clamped mechanical mode we are able to operate in the regime where measurement quantum backaction contributes as much force noise as the thermal environment does. However, in the presence of intermodulation noise, quantum signatures of measurement are not revealed in direct photodetectors. The reported noise mechanism, while studied for an optomechanical system, can exist in any optical cavity

Hierarchical tensile structures with ultralow mechanical dissipation

Structural hierarchy is found in myriad biological systems and has improved man-made structures ranging from the Eiffel tower to optical cavities. Hierarchical metamaterials utilize structure at multiple size scales to realize new and highly desirable properties which can be strikingly different from those of the constituent materials. In mechanical resonators whose rigidity is provided by static tension, structural hierarchy can reduce the dissipation of the fundamental mode to ultralow levels due to an unconventional form of soft clamping. Here, we apply hierarchical design to silicon nitride nanomechanical resonators and realize binary tree-shaped resonators with quality factors as high as $10^9$ at 107 kHz frequency, reaching the parameter regime of levitated particles. The resonators' thermal-noise-limited force sensitivities reach $740\ \mathrm{zN/\sqrt{Hz}}$ at room temperature and $\mathrm{90\ zN/\sqrt{Hz}}$ at 6 K, surpassing state-of-the-art cantilevers currently used for force microscopy. We also find that the self-similar structure of binary tree resonators results in fractional spectral dimensions, which is characteristic of fractal geometries. Moreover, we show that the hierarchical design principles can be extended to 2D trampoline membranes, and we fabricate ultralow dissipation membranes suitable for interferometric position measurements in Fabry-P\'erot cavities. Hierarchical nanomechanical resonators open new avenues in force sensing, signal transduction and quantum optomechanics, where low dissipation is paramount and operation with the fundamental mode is often advantageous.Comment: 19 pages, 11 figures. Fixed link to Zenodo repositor

Generalized dissipation dilution in strained mechanical resonators

Mechanical resonators with high quality factors are of relevance in precision experiments, ranging from gravitational wave detection and force sensing to quantum optomechanics. Beams and membranes are well known to exhibit flexural modes with enhanced quality factors when subjected to tensile stress. The mechanism for this enhancement has been a subject of debate, but is typically attributed to elastic energy being "diluted" by a lossless potential. Here we clarify the origin of the lossless potential to be the combination of tension and geometric nonlinearity of strain. We present a general theory of dissipation dilution that is applicable to arbitrary resonator geometries and discuss why this effect is particularly strong for flexural modes of nanomechanical structures with high aspect ratios. Applying the theory to a non-uniform doubly clamped beam, we show analytically how dissipation dilution can be enhanced by modifying the beam shape to implement "soft clamping", thin clamping and geometric strain engineering, and derive the ultimate limit for dissipation dilution

High-yield wafer-scale fabrication of ultralow-loss, dispersion-engineered silicon nitride photonic circuits

Low-loss photonic integrated circuits (PIC) and microresonators have enabled novel applications ranging from narrow-linewidth lasers, microwave photonics, to chip-scale optical frequency combs and quantum frequency conversion. To translate these results into a widespread technology, attaining ultralow optical losses with established foundry manufacturing is critical. Recent advances in fabrication of integrated Si3N4 photonics have shown that ultralow-loss, dispersion-engineered microresonators can be attained at die-level throughput. For emerging nonlinear applications such as integrated travelling-wave parametric amplifiers and mode-locked lasers, PICs of length scales of up to a meter are required, placing stringent demands on yield and performance that have not been met with current fabrication techniques. Here we overcome these challenges and demonstrate a fabrication technology which meets all these requirements on wafer-level yield, performance and length scale. Photonic microresonators with a mean Q factor exceeding 30 million, corresponding to a linear propagation loss of 1.0 dB/m, are obtained over full 4-inch wafers, as determined from a statistical analysis of tens of thousands of optical resonances and cavity ringdown with 19 ns photon storage time. The process operates over large areas with high yield, enabling 1-meter-long spiral waveguides with 2.4 dB/m loss in dies of only 5x5 mm size. Using a modulation response measurement self-calibrated via the Kerr nonlinearity, we reveal that, strikingly, the intrinsic absorption-limited Q factor of our Si3N4 microresonators exceeds a billion. Transferring the present Si3N4 photonics technology to standard commercial foundries, and merging it with silicon photonics using heterogeneous integration technology, will significantly expand the scope of today's integrated photonics and seed new applications

Electron-Photon Quantum State Heralding Using Photonic Integrated Circuits

Recently, integrated photonic circuits have brought new capabilities to electron microscopy and been used to demonstrate efficient electron phase modulation and electron-photon correlations. Here, we quantitatively analyze the feasibility of high-fidelity and high-purity quantum state heralding using a free electron and a photonic integrated circuit with parametric coupling, and propose schemes to shape useful electron and photonic states in different application scenarios. Adopting a dissipative quantum electrodynamics treatment, we formulate a framework for the coupling of free electrons to waveguide spatial-temporal modes. To avoid multimode-coupling-induced state decoherence, we show that with proper waveguide design, the interaction can be reduced to a single-mode coupling to a quasi-TM_{00} mode. In the single-mode coupling limit, we go beyond the conventional state ladder treatment, and show that the electron-photon energy correlations within the ladder subspace can still lead to a fundamental purity and fidelity limit on complex optical and electron state preparations through heralding schemes. We propose applications that use this underlying correlation to their advantage, but also show that the imposed limitations for general applications can be overcome by using photonic integrated circuits with an experimentally feasible interaction length, showing its promise as a platform for free-electron quantum optics