505 research outputs found
Temperature-dependent photoemission spectral weight transfer and chemical potential shift in PrCaMnO : Implications for charge density modulation
We have studied the temperature dependence of the photoemission spectra of
PrCaMnO (PCMO) with , 0.3 and 0.5. For and 0.5,
we observed a gap in the low-temperature CE-type charge-ordered (CO) phase and
a pseudogap with a finite intensity at the Fermi level () in the
high-temperature paramagnetic insulating (PI) phase. Within the CO phase, the
spectral intensity near gradually increased with temperature. These
observations are consistent with the results of Monte Carlo simulations on a
model including charge ordering and ferromagnetic fluctuations [H. Aliaga {\it
et al.} Phys. Rev. B {\bf 68}, 104405 (2003)]. For , on the other hand,
little temperature dependence was observed within the low-temperature
ferromagnetic insulating (FI) phase and the intensity at remained low in
the high-temperature PI phase. We attribute the difference in the temperature
dependence near between the CO and FI phases to the different correlation
lengths of orbital order between both phases. Furthermore, we observed a
chemical potential shift with temperature due to the opening of the gap in the
FI and CO phases. The doping dependent chemical potential shift was recovered
at low temperatures, corresponding to the disappearance of the doping dependent
change of the modulation wave vector. Spectral weight transfer with hole
concentration was clearly observed at high temperatures but was suppressed at
low temperatures. We attribute this observation to the fixed periodicity with
hole doping in PCMO at low temperatures.Comment: 5pages, 7figure
Orbital ordering in LaSrMnO studied by model Hartree-Fock calculation
We have investigated orbital ordering in the half-doped manganite
LaSrMnO, which displays spin, charge and orbital ordering,
by means of unrestricted Hartree-Fock calculations on the multiband -
model. From recent experiment, it has become clear that
LaSrMnO exhibits a cross-type orbital
ordering rather than the widely believed rod-type orbital
ordering. The calculation reveals that cross-type orbital
ordering results from an effect of in-plane distortion as well as from the
relatively long out-of-plane Mn-O distance. For the "Mn" site, it is
shown that the elongation along the c-axis of the MnO octahedra leads to an
anisotropic charge distribution rather than the isotropic one.Comment: 4 pages, 5 figure
Chemical potential shift induced by double-exchange and polaronic effects in Nd_{1-x}Sr_xMnO_3
We have studied the chemical potential shift as a function of temperature in
NdSrMnO (NSMO) by measurements of core-level photoemission
spectra. For ferromagnetic samples ( and 0.45), we observed an unusually
large upward chemical potential shift with decreasing temperature in the
low-temperature region of the ferromagnetic metallic (FM) phase. This can be
explained by the double-exchange (DE) mechanism if the band is split by
dynamical/local Jahn-Teller effect. The shift was suppressed near the Curie
temperature (), which we attribute to the crossover from the DE to
lattice-polaron regimes.Comment: 5 pages, 6 figure
Military Children’s Difficulty with Reintegration after Deployment: A Relational Turbulence Model Perspective
This study drew on the relational turbulence model to investigate how the interpersonal dynamics of military couples predict parents’ reports of the reintegration difficulty of military children upon homecoming after deployment. Longitudinal data were collected from 118 military couples once per month for 3 consecutive months after reunion. Military couples reported on their depressive symptoms, characteristics of their romantic relationship, and the reintegration difficulty of their oldest child. Results of dyadic growth curve models indicated that the mean levels of parents’ depressive symptoms (H1), relationship uncertainty (H2), and interference from a partner (H3) were positively associated with parents’ reports of military children’s reintegration difficulty. These findings suggest that the relational turbulence model has utility for illuminating the reintegration difficulty of military children during the postdeployment transition
Global density-dependent -nucleon interaction for -nucleus elastic scattering
We provide a global density-dependent He-nucleon (DD-)
interaction to construct the -nucleus optical model potential (OMP) in
a wide range of incident energies. The global parametrization for the
DD- interaction is obtained based on the proton-He OMP which
reproduces the elastic scattering cross-section data very well in the incident
energies of 12.04--500 MeV per nucleon. We derive the -nucleus
potential by a folding procedure with the point-nucleon density obtained by a
microscopic mean-field model using the present DD- interaction. The
density dependence of the DD- interaction is fixed phenomenologically
to reproduce the -nucleus elastic scattering cross-section data by the
O, Ca, Ni, Zr, and Pb targets at
10--342.5 MeV. We also show the total reaction cross sections, which are
helpful in fixing one free parameter, the renormalization factor for the
imaginary part of the -nucleus potential. Lastly, we show some
examples, which clearly demonstrate the validity and power of the present
DD- approach.Comment: 20 pages, 11 figure
Depth profile photoemission study of thermally diffused Mn/GaAs (001) interfaces
We have performed a depth profile study of thermally diffused Mn/GaAs (001)
interfaces using photoemission spectroscopy combined with Ar-ion
sputtering. We found that Mn ion was thermally diffused into the deep region of
the GaAs substrate and completely reacted with GaAs. In the deep region, the Mn
2 core-level and Mn 3 valence-band spectra of the Mn/GaAs (001) sample
heated to 600 C were similar to those of GaMnAs,
zinc-blende-type MnAs dots, and/or interstitial Mn in tetrahedrally coordinated
by As atoms, suggesting that the Mn 3 states were essentially localized but
were hybridized with the electronic states of the host GaAs. Ferromagnetism was
observed in the dilute Mn phase.Comment: 5 pages, 4 figure
Chemical potential landscape in band filling and bandwidth-control of manganites: Photoemission spectroscopy measurements
We have studied the effects of band filling and bandwidth control on the
chemical potential in perovskite manganites MnO ( : rare
earth, : alkaline earth) by measurements of core-level photoemission
spectra. A suppression of the doping-dependent chemical potential shift was
observed in and around the CE-type charge-ordered composition range, indicating
that there is charge self-organization such as stripe formation or its
fluctuations. As a function of bandwidth, we observed a downward chemical
potential shift with increasing bandwidth due to the reduction of the
orthorhombic distortion. After subtracting the latter contribution, we found an
upward chemical potential shift in the ferromagnetic metallic region
, which we attribute to the enhancement of double-exchange
interaction involving the Jahn-Teller-split band.Comment: 5 pages, 4 figure
Chemical potential shift and spectral weight transfer in PrCaMnO revealed by photoemission spectroscopy
We have studied the chemical potential shift and changes in the electronic
density of states near the Fermi level () as a function of carrier
concentration in PrCaMnO (PCMO, ) through
the measurements of photoemission spectra. The results showed that the chemical
potential shift was suppressed for x \agt 0.3, where the charge exchange
(CE)-type antiferromagnetic charge-ordered state appears at low temperatures.
We consider this observation to be related to charge self-organization such as
stripe formation on a microscopic scale in this composition range. Together
with the previous observation of monotonous chemical potential shift in
LaSrMnO, we conclude that the tendency toward the charge
self-organization increases with decreasing bandwidth. In the valence band,
spectral weight of the Mn 3 electrons in PCMO was transferred from
1 eV below to the region near with hole doping, leading to a
finite intensity at even in the paramagnetic insulating phase for x \agt
0.3, probably related with the tendency toward charge self-organization. The
finite intensity at in spite of the insulating transport behavior is
consistent with fluctuations involving ferromagnetic metallic states.Comment: 6 pages, 5 figure
Theoretical demonstration of highly efficient cw THz generation by using composite photonic-structure elements
We theoretically propose one-dimensional composite photonic structures for high-resolution THz spectroanalysis. We compare the performance of two GaAs/AlAs composite photonic-structure devices, one with usual 1/4-wavelength layers of distributed Bragg reflectors (DBRs), and the other with the designed DBRs. The device with designed DBRs shows the optical-to-terahertz conversion efficiency up to 10^-5 and wide frequency tunability ranging from sub-THz to 3 THz. We found that the composite photonic structure allows us to control photonic modes with a high degree of freedom by flexible structure designs. This device achieve a cw THz source with a highly narrow bandwidth operating at room temperature
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