1,293 research outputs found
Transport properties of diluted magnetic semiconductors: Dynamical mean field theory and Boltzmann theory
The transport properties of diluted magnetic semiconductors (DMS) are
calculated using dynamical mean field theory (DMFT) and Boltzmann transport
theory. Within DMFT we study the density of states and the dc-resistivity,
which are strongly parameter dependent such as temperature, doping, density of
the carriers, and the strength of the carrier-local impurity spin exchange
coupling. Characteristic qualitative features are found distinguishing weak,
intermediate, and strong carrier-spin coupling and allowing quantitative
determination of important parameters defining the underlying ferromagnetic
mechanism. We find that spin-disorder scattering, formation of bound state, and
the population of the minority spin band are all operational in DMFT in
different parameter range. We also develop a complementary Boltzmann transport
theory for scattering by screened ionized impurities. The difference in the
screening properties between paramagnetic () and ferromagnetic ()
states gives rise to the temperature dependence (increase or decrease) of
resistivity, depending on the carrier density, as the system goes from the
paramagnetic phase to the ferromagnetic phase. The metallic behavior below
for optimally doped DMS samples can be explained in the Boltzmann theory
by temperature dependent screening and thermal change of carrier spin
polarization.Comment: 15 pages, 15 figure
Lifetime of Gapped Excitations in a Collinear Quantum Antiferromagnet
We demonstrate that local modulations of magnetic couplings have a profound
effect on the temperature dependence of the relaxation rate of optical magnons
in a wide class of antiferromagnets in which gapped excitations coexist with
acoustic spin waves. In a two-dimensional collinear antiferromagnet with an
easy-plane anisotropy, the disorder-induced relaxation rate of the gapped mode,
Gamma_imp=Gamma_0+A(TlnT)^2, greatly exceeds the magnon-magnon damping,
Gamma_m-m=BT^5, negligible at low temperatures. We measure the lifetime of
gapped magnons in a prototype XY antiferromagnet BaNi2(PO4)2 using a
high-resolution neutron-resonance spin-echo technique and find experimental
data in close accord with the theoretical prediction. Similarly strong effects
of disorder in the three-dimensional case and in noncollinear antiferromagnets
are discussed.Comment: 4.5 pages + 2.5 pages supplementary material, published versio
Expression, Purification, Crystallization and Preliminary X-ray Studies of Histamine Dehydroganase from Nocardioides simplex
This is the publisher's version, also available electronically from http://scripts.iucr.org/cgi-bin/paper?S1744309108023336.Histamine dehydrogenase (HADH) from Nocardioides simplex catalyzes the oxidative deamination of histamine to produce imidazole acetaldehyde and an ammonium ion. HADH is functionally related to trimethylamine dehydrogenase (TMADH), but HADH has strict substrate specificity towards histamine. HADH is a homodimer, with each 76 kDa subunit containing two redox cofactors: a [4Fe-4S] cluster and an unusual covalently bound flavin mononucleotide, 6-S-cysteinyl-FMN. In order to understand the substrate specificity of HADH, it was sought to determine its structure by X-ray crystallography. This enzyme has been expressed recombinantly in Escherichia coli and successfully crystallized in two forms. Diffraction data were collected to 2.7 Å resolution at the SSRL synchrotron with 99.7% completeness. The crystals belonged to the orthorhombic space group P212121, with unit-cell parameters a = 101.14, b = 107.03, c = 153.35 Å
Ultrafast demagnetization in the sp-d model: a theoretical study
We propose and analyze a theoretical model of ultrafast light-induced
magnetization dynamics in systems of localized spins that are coupled to
carriers' spins by sp-d exchange interaction. A prominent example of a class of
materials falling into this category are ferromagnetic (III,Mn)V
semiconductors, in which ultrafast demagnetization has been recently observed.
In the proposed model light excitation heats up the population of carriers,
taking it out of equilibrium with the localized spins. This triggers the
process of energy and angular momentum exchange between the two spin systems,
which lasts for the duration of the energy relaxation of the carriers. We
derive the Master equation for the density matrix of a localized spin
interacting with the hot carriers and couple it with a phenomenological
treatment of the carrier dynamics. We develop a general theory within the sp-d
model and we apply it to the ferromagnetic semiconductors, taking into account
the valence band structure of these materials. We show that the fast spin
relaxation of the carriers can sustain the flow of polarization between the
localized and itinerant spins leading to significant demagnetization of the
localized spin system, observed in (III,Mn)V materials.Comment: 15 pages, 8 figure
Interlayer Magnetic Frustration in Quasi-stoichiometric Li1-xNi1+xO2
Susceptibility, high-field magnetization and submillimeter wave electron spin
resonance measurements of layered quasi-stoichiometric Li1-xNi1+xO2 are
reported and compared to isomorphic NaNiO2. A new mechanism of magnetic
frustration induced by the excess Ni ions always present in the Li layers is
proposed. We finally comment on the possible realization of an orbital liquid
state in this controversial compound.Comment: 4 pages, 5 figures, submitted to Phys.Rev.B, Rapid Com
Comparison of formaldehyde and methanol fixatives used in the detection of ion channel proteins in isolated rat ventricular myocytes by immunofluorescence labelling and confocal microscopy
In this study, a fixation protocol using a 10% neutral buffered formalin (FA) solution and another protocol using a methanol (MeOH) solution were compared for detection of ion channels, Kv1.5, Kv4.2, Cav1.2, Kir6.2, Nav1.5 and Nav1.1 in rat myocytes by immunolabelling. Kv1.5 and Kv4.2 at intercalated discs and Cav1.2 at transverse tubules were not detected by FA but were detected by MeOH. Kir6.2 at transverse tubules and Nav1.5 at sarcolemma were detected by FA but not by MeOH. It is suggested that both FA and MeOH fixation protocols should be used for the detection of cardiac ion channels by immunolabellin
Optical properties of metallic (III,Mn)V ferromagnetic semiconductors in the infrared to visible range
We report on a study of the ac conductivity and magneto-optical properties of
metallic ferromagnetic (III,Mn)V semiconductors in the infrared to visible
spectrum. Our analysis is based on the successful kinetic exchange model for
(III,Mn)V ferromagnetic semiconductors. We perform the calculations within the
Kubo formalism and treat the disorder effects pertubatively within the Born
approximation, valid for the metallic regime. We consider an eight-band
Kohn-Luttinger model (six valence bands plus two conduction bands) as well as a
ten-band model with additional dispersionless bands simulating
phenomenologically the upper-mid-gap states induced by antisite and
interstitial impurities. These models qualitatively account for
optical-absorption experiments and predict new features in the mid-infrared
Kerr angle and magnetic-circular-dichroism properties as a function of Mn
concentration and free carrier density.Comment: 10 pages, 7 figures, some typos correcte
Interactions in high-mobility 2D electron and hole systems
Electron-electron interactions mediated by impurities are studied in several
high-mobility two-dimensional (electron and hole) systems where the parameter
changes from 0.1 to 10 ( is the momentum relaxation
time). This range corresponds to the \textit{intermediate} and \textit
{ballistic} regimes where only a few impurities are involved in
electron-electron interactions. The interaction correction to the Drude
conductivity is detected in the temperature dependence of the resistance and in
the magnetoresistance in parallel and perpendicular magnetic fields. The
effects are analysed in terms of the recent theories of electron interactions
developed for the ballistic regime. It is shown that the character of the
fluctuation potential (short-range or long-range) is an important factor in the
manifestation of electron-electron interactions in high-mobility 2D systems.Comment: 22 pages, 11 figures; to appear in proceedings of conference
"Fundamental Problems of Mesoscopic Physics", Granada, Spain, 6-11 September,
200
Orbital Configurations and Magnetic Properties of Double-Layered Antiferromagnet CsCuClBr
We report the single-crystal X-ray analysis and magnetic properties of a new
double-layered perovskite antiferromagnet, CsCuClBr. This
structure is composed of CuClBr double layers with elongated
CuClBr octahedra and is closely related to the SrTiO
structure. An as-grown crystal has a singlet ground state with a large
excitation gap of K, due to the strong
antiferromagnetic interaction between the two layers. CsCuClBr
undergoes a structural phase transition at K accompanied
by changes in the orbital configurations of Cu ions. Once a
CsCuClBr crystal is heated above , its magnetic
susceptibility obeys the Curie-Weiss law with decreasing temperature even below
and does not exhibit anomalies at . This implies that in
the heated crystal, the orbital state of the high-temperature phase remains
unchanged below , and thus, this orbital state is the metastable
state. The structural phase transition at is characterized as an
order-disorder transition of Cu orbitals.Comment: 6pages. 6figures, to appear in J. Phys. Soc. Jpn. Vol.76 No.
- …