479 research outputs found

    High-temperature superconductivity from fine-tuning of Fermi-surface singularities in iron oxypnictides

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    In the family of the iron-based superconductors, the REREFeAsO-type compounds (with RERE being a rare-earth metal) exhibit the highest bulk superconducting transition temperatures (TcT_{\mathrm{c}}) up to 55 K55\ \textrm{K} and thus hold the key to the elusive pairing mechanism. Recently, it has been demonstrated that the intrinsic electronic structure of SmFe0.92_{0.92}Co0.08_{0.08}AsO (Tc=18 KT_{\mathrm{c}}=18\ \textrm{K}) is highly nontrivial and consists of multiple band-edge singularities in close proximity to the Fermi level. However, it remains unclear whether these singularities are generic to the REREFeAsO-type materials and if so, whether their exact topology is responsible for the aforementioned record TcT_{\mathrm{c}}. In this work, we use angle-resolved photoemission spectroscopy (ARPES) to investigate the inherent electronic structure of the NdFeAsO0.6_{0.6}F0.4_{0.4} compound with a twice higher Tc=38 KT_{\mathrm{c}}=38\ \textrm{K}. We find a similarly singular Fermi surface and further demonstrate that the dramatic enhancement of superconductivity in this compound correlates closely with the fine-tuning of one of the band-edge singularities to within a fraction of the superconducting energy gap Δ\Delta below the Fermi level. Our results provide compelling evidence that the band-structure singularities near the Fermi level in the iron-based superconductors must be explicitly accounted for in any attempt to understand the mechanism of superconducting pairing in these materials.Comment: Open access article available online at http://www.nature.com/articles/srep1827
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