156 research outputs found
Nodal Superconducting Order Parameter and Thermodynamic Phase Diagram of (TMTSF)2ClO4
The organic materials (TMTSF)2X are unique unconventional superconductors
with archetypal quasi-one-dimensional (Q1D) electronic structures. Here, based
on our comprehensive field-angle-resolved calorimetry of (TMTSF)2ClO4, we
succeeded in mapping the nodal gap structure for the first time in Q1D systems,
by discriminating between the Fermi wavevectors and Fermi velocities. In
addition, the thermodynamic phase diagrams of (TMTSF)2ClO4 for all principal
field directions are obtained. These findings, providing strong evidence of
nodal spin-singlet superconductivity, serves as solid bases for further
elucidation of anomalous superconducting phenomena in (TMTSF)2X.Comment: 7 pages, 7 figures, including Supplemental Information added at the
end of the manuscrip
The optical conductivity of the quasi one-dimensional conductors: the role of forward scattering by impurities
We calculate the average conductivity sigma (omega) of interacting electrons
in one dimension in the presence of a long-range random potential (forward
scattering disorder). Taking the curvature of the energy dispersion into
account, we show that weak disorder leads to a transport scattering rate that
vanishes as omega^2 for small frequency omega. This implies that the real part
of the conductivity remains finite for omega -> 0, while the imaginary part
diverges. These effects are lost within the usual bosonization approach, which
relies on the linearization of the energy dispersion. We discuss our result in
the light of a recent experiment.Comment: 5 RevTex pages; more careful comparison with experiments and
discussion of interchain hopping added; some references added; to appear in
Phys. Rev.
Upper critical field divergence induced by mesoscopic phase separation in the organic superconductor (TMTSF)2ReO4
Due to the competition of two anion orders, (TMTSF)2ReO4, presents a phase
coexistence between semiconducting and metallic (superconducting) regions
(filaments or droplets) in a wide range of pressure. In this regime, the
superconducting upper critical field for H parallel to both c* and b' axes
present a linear part at low fields followed by a divergence above a cross-over
field. This cross-over corresponds to the 3D-2D decoupling transition expected
in filamentary or granular superconductors. The sharpness of the transition
also demonstrates that all filaments are of similar sizes and self organize in
a very ordered way. The distance between the filaments and their cross-section
are estimated.Comment: 4 pages, 4 figure
Magnetic-Field Variations of the Pair-Breaking Effects of Superconductivity in (TMTSF)2ClO4
We have studied the onset temperature of the superconductivity Tc_onset of
the organic superconductor (TMTSF)2ClO4, by precisely controlling the direction
of the magnetic field H. We compare the results of two samples with nearly the
same onset temperature but with different scattering relaxation time tau. We
revealed a complicated interplay of a variety of pair-breaking effects and
mechanisms that overcome these pair-breaking effects. In low fields, the linear
temperature dependences of the onset curves in the H-T phase diagrams are
governed by the orbital pair-breaking effect. The dips in the in-plane
field-angle phi dependence of Tc_onset, which were only observed in the
long-tau sample, provides definitive evidence that the field-induced
dimensional crossover enhances the superconductivity if the field direction is
more than about 19-degrees away from the a axis. In the high-field regime for
H//a, the upturn of the onset curve for the long-tau sample indicates a new
superconducting state that overcomes the Pauli pair-breaking effect but is
easily suppressed by impurity scatterings. The Pauli effect is also overcome
for H//b' by a realization of another state for which the maximum of
Tc_onset(phi) occurs in a direction different from the crystalline axes. The
effect on Tc_onset of tilting the applied field out of the conductive plane
suggests that the Pauli effect plays a significant role in determining
Tc_onset. The most plausible explanation of these results is that (TMTSF)2ClO4
is a singlet superconductor and exhibits Fulde-Ferrell-Larkin-Ovchinnikov
(FFLO) states in high fields.Comment: 12 pages, 10 figures. To be published in J. Phys. Soc. Jpn. (vol.77,
2008
Correlation Effect on Peierls Transition
The effect of correlation on Peierls transition, which is accompanied by a
dimerization, t_d, of a bond alternation for transfer energy, has been examined
for a half-filled one-dimensional electron system with on-site repulsive
interaction (U). By applying the renormalization group method to the
interaction of the bosonized Hamiltonian, the dimerization has been calculated
variationally and self-consistently with a fixed electron-phonon coupling
constant (\lambda) and it is shown that t_d takes a maximum as a function of U.
The result is examined in terms of charge gap and spin gap and is compared with
that of the numerical simulation by Hirsch [Phys. Rev. Lett 51 (1983) 296].
Relevance to the spin Peierls transition in organic conductors is discussed.Comment: 4 pages, 4 figures, to be published in J. Phys. Soc. Jpn. 71 No.3
(2002
Competition of Dimerization and Charge Ordering in the Spin-Peierls State of Organic Conductors
The effect of the charge ordering on the spin-Peierls (SP) state has been
examined by using a Peierls-Hubbard model at quarter-filling with dimerization,
on-site and nearest-neighbor repulsive interactions. By taking account of the
presence of dimerization, a bond distortion is calculated variationally with
the renormalization group method based on bosonization. When the charge
ordering appears at V=V_c with increasing the nearest-neighbor interaction (V),
the distortion exhibits a maximum due to competition between the dimerization
and the charge ordering. It is shown that the second-order phase transition
occurs from the SP state with the bond alternation to a mixed state with an
additional component of the site alternationat V = V_c.Comment: 11 pages, 13 figures, to be published in J. Phys. Soc. Jpn. 72 No.6
(2003
Fermi Liquid Damping and NMR Relaxation in Superconductors
Electron collisions for a two dimensional Fermi liquid (FL) are shown to give
a quasiparticle damping with interesting frequency and temperature variations
in the BCS superconducting state. The spin susceptibility which determines the
structure of the damping is analyzed in the normal state for a Hubbard model
with a constant on--site Coulomb repulsion. This is then generalized to the
superconducting state by including coherence factors and self energy and vertex
corrections. Calculations of the NMR relaxation rate reveal that the FL damping
structure can reduce the Hebel--Slichter peak, in agreement with data on the
organic superconductor (MDT-TTF)AuI. However, the strongly suppressed
FL damping in the superconducting state does not eliminate the Hebel-Slichter
peak, and thus suggests that other mechanisms are needed to explain the NMR
data on (TMTSF)ClO, the BEDT organic compounds, and cuprate
superconductors. Predictions of the temperature variation of the damping and
the spin response are given over a wide frequency range as a guide to
experimental probes of the symmetry of the superconducting pairs.Comment: 10 pages, RevTeX 3.0, 9 figures in uuencoded postscrip
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