Oriented polar molecules in a solid inert-gas matrix: a proposed method for measuring the electric dipole moment of the electron

We propose a very sensitive method for measuring the electric dipole moment of the electron using polar molecules embedded in a cryogenic solid matrix of inert-gas atoms. The polar molecules can be oriented in the $\hat{\rm{z}}$ direction by an applied electric field, as has recently been demonstrated by Park, et al. [Angewandte Chemie {\bf 129}, 1066 (2017)]. The trapped molecules are prepared into a state which has its electron spin perpendicular to $\hat{\rm{z}}$, and a magnetic field along $\hat{\rm{z}}$ causes precession of this spin. An electron electric dipole moment $d_e$ would affect this precession due to the up to 100~GV/cm effective electric field produced by the polar molecule. The large number of polar molecules that can be embedded in a matrix, along with the expected long coherence times for the precession, allows for the possibility of measuring $d_e$ to an accuracy that surpasses current measurements by many orders of magnitude. Because the matrix can inhibit molecular rotations and lock the orientation of the polar molecules, it may not be necessary to have an electric field present during the precession. The proposed technique can be applied using a variety of polar molecules and inert gases, which, along with other experimental variables, should allow for careful study of systematic uncertainties in the measurement

Deflection of barium monofluoride molecules using the bichromatic force: A density-matrix simulation

A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We show that the force is sufficient to separate BaF molecules from the other products generated in a helium-buffer-gas-cooled ablation source. For our simulations, the density-matrix and force equations are numerically integrated during the entire time that the molecules pass through a laser beam to ensure that effects of the evolution of the Doppler shift and of the optical intensity and phase at the position of the molecule are properly included. The results of this work are compared to those of a deflection scheme (Phys. Rev. A 107, 032811 (2023)) which uses $\pi$ pulses to drive frequency-resolved transitions. This work is part of an effort by the EDM$^3$ collaboration to measure the electric dipole moment of the electron using BaF molecules embedded in a cryogenic argon solid. Separation of BaF molecules will aid in producing a sufficiently pure solid.Comment: 8 pages, 5 figure

A Strong Upper Limit on the Pulsed Radio Luminosity of the Compact Object 1RXS J141256.0+792204

The ROSAT X-ray source 1RXS J141256.0+792204 has recently been identified as a likely compact object whose properties suggest it could be a very nearby radio millisecond pulsar at d = 80 - 260pc. We investigated this hypothesis by searching for radio pulsations using the Westerbork Synthesis Radio Telescope. We observed 1RXS J141256.0+792204 at 385 and 1380MHz, recording at high time and frequency resolution in order to maintain sensitivity to millisecond pulsations. These data were searched both for dispersed single pulses and using Fourier techniques sensitive to constant and orbitally modulated periodicities. No radio pulsations were detected in these observations, resulting in pulsed radio luminosity limits of L_400 ~ 0.3 (d/250pc)^2 mJy kpc^2 and L_1400 ~ 0.03 (d/250pc)^2 mJy kpc^2 at 400 and 1400MHz respectively. The lack of detectable radio pulsations from 1RXS J141256.0+792204 brings into question its identification as a nearby radio pulsar, though, because the pulsar could be beamed away from us, this hypothesis cannot be strictly ruled out.Comment: To appear in A&A. 3 page