749 research outputs found
Collective Spin-Density-Wave Response Perpendicular to the Chains of the Quasi One-Dimensional Conductor (TMTSF)2PF6
Microwave experiments along all three directions of the spin-density-wave
model compound (TMTSF)PF reveal that the pinned mode resonance is
present along the and axes. The collective transport is
considered to be the fingerprint of the condensate. In contrast to common quasi
one-dimensional models, the density wave also slides in the perpendicular
direction. The collective response is absent along the least
conducting direction.Comment: 3 pages, 4 figure
Competition between Charge Ordering and Superconductivity in Layered Organic Conductors -(BEDT-TTF)Hg(SCN) (M = K, NH)
While the optical properties of the superconducting salt
-(BEDT-TTF)NHHg(SCN) remain metallic down to 2 K, in the
non-superconducting K-analog a pseudogap develops at frequencies of about 200
cm for temperatures T < 200 K. Based on exact diagonalisation
calculations on an extended Hubbard model at quarter-filling we argue that
fluctuations associated with short range charge ordering are responsible for
the observed low-frequency feature. The different ground states, including
superconductivity, are a consequence of the proximity of these compounds to a
quantum phase charge-ordering transition driven by the intermolecular Coulomb
repulsion.Comment: 4 pages, 3 figure
Zero temperature optical conductivity of ultra-clean Fermi liquids and superconductors
We calculate the low-frequency optical conductivity sigma(w) of clean metals
and superconductors at zero temperature neglecting the effects of impurities
and phonons. In general, the frequency and temperature dependences of sigma
have very little in common. For small Fermi surfaces in three dimensions (but
not in 2D) we find for example that Re sigma(w>0)=const. for low w which
corresponds to a scattering rate Gamma proportional to w^2 even in the absence
of Umklapp scattering when there is no T^2 contribution to Gamma. In the main
part of the paper we discuss in detail the optical conductivity of d-wave
superconductors in 2D where Re sigma(w>0) \propto w^4 for the smallest
frequencies and the Umklapp processes typically set in smoothly above a finite
threshold w_0 smaller than twice the maximal gap Delta. In cases where the
nodes are located at (pi/2, pi/2), such that direct Umklapp scattering among
them is possible, one obtains Re sigma(w) \propto w^2.Comment: 7 pages, 3 figure
Electrodynamics of electron doped iron-pnictide superconductors: Normal state properties
The electrodynamic properties of Ba(FeCoAs and
Ba(FeNi_{2}T^2m^*/m_b\approx 5$ in the static limit) and scattering rate that does not
disclose a simple power law. The spectral weight shifts to lower energies upon
cooling; a significant fraction is not recovered within the infrared range of
frequencies.Comment: 13 pages, 9 figure
Transient terahertz spectroscopy of excitons and unbound carriers in quasi two-dimensional electron-hole gases
We report a comprehensive experimental study and detailed model analysis of
the terahertz dielectric response and density kinetics of excitons and unbound
electron-hole pairs in GaAs quantum wells. A compact expression is given, in
absolute units, for the complex-valued terahertz dielectric function of
intra-excitonic transitions between the 1s and higher-energy exciton and
continuum levels. It closely describes the terahertz spectra of resonantly
generated excitons. Exciton ionization and formation are further explored,
where the terahertz response exhibits both intra-excitonic and Drude features.
Utilizing a two-component dielectric function, we derive the underlying exciton
and unbound pair densities. In the ionized state, excellent agreement is found
with the Saha thermodynamic equilibrium, which provides experimental
verification of the two-component analysis and density scaling. During exciton
formation, in turn, the pair kinetics is quantitatively described by a Saha
equilibrium that follows the carrier cooling dynamics. The terahertz-derived
kinetics is, moreover, consistent with time-resolved luminescence measured for
comparison. Our study establishes a basis for tracking pair densities via
transient terahertz spectroscopy of photoexcited quasi-two-dimensional
electron-hole gases.Comment: 14 pages, 8 figures, final versio
Electronic correlations and unusual superconducting response in the optical properties of the iron-chalcogenide FeTe0.55Se0.45
The in-plane complex optical properties of the iron-chalcogenide
superconductor FeTe0.55Se0.45 have been determined above and below the critical
temperature Tc = 14 K. At room temperature the conductivity is described by a
weakly-interacting Fermi liquid; however, below 100 K the scattering rate
develops a frequency dependence in the terahertz region, signaling the
increasingly correlated nature of this material. We estimate the dc
conductivity just above Tc to be sigma_dc ~ 3500 Ohm-1cm-1 and the superfluid
density rho_s0 ~ 9 x 10^6 cm-2, which places this material close to the scaling
line rho_s0/8 ~ 8.1 sigma_dc Tc for a BCS dirty-limit superconductor. Below Tc
the optical conductivity reveals two gap features at Delta_1,2 ~ 2.5 and ~ 5.1
meV.Comment: Minor revisions, 5 pages, 4 figure
Hybridization gap versus hidden order gap in URuSi as revealed by optical spectroscopy
We present the in-plane optical reflectance measurement on single crystals of
URuAs. The study revealed a strong temperature-dependent spectral
evolution. Above 50 K, the low frequency optical conductivity is rather flat
without a clear Drude-like response, indicating a very short transport life
time of the free carriers. Well below the coherence temperature, there appears
an abrupt spectral weight suppression below 400 cm, yielding evidence
for the formation of a hybridization energy gap arising from the mixing of the
conduction electron and narrow f-electron bands. A small part of the suppressed
spectral weight was transferred to the low frequency side, leading to a narrow
Drude component, while the majority of the suppressed spectral weight was
transferred to the high frequency side centered near 4000 cm. Below the
hidden order temperature, another very prominent energy gap structure was
observed, which leads to the removal of a large part of the Drude component and
a sharp reduction of the carrier scattering rate. The study revealed that the
hybridization gap and the hidden orger gap are distinctly different: they occur
at different energy scales and exhibit completely different spectral
characteristics.Comment: 5 page
Direct Observation of Quantum Coherence in Single-Molecule Magnets
Direct evidence of quantum coherence in a single-molecule magnet in frozen
solution is reported with coherence times as long as T2 = 630 ns. We can
strongly increase the coherence time by modifying the matrix in which the
single-molecule magnets are embedded. The electron spins are coupled to the
proton nuclear spins of both the molecule itself and interestingly, also to
those of the solvent. The clear observation of Rabi oscillations indicates that
we can manipulate the spin coherently, an essential prerequisite for performing
quantum computations.Comment: 5 Pages, 4 Figures, final version published in PR
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