Four-photon orbital angular momentum entanglement

Quantum entanglement shared between more than two particles is essential to foundational questions in quantum mechanics, and upcoming quantum information technologies. So far, up to 14 two-dimensional qubits have been entangled, and an open question remains if one can also demonstrate entanglement of higher-dimensional discrete properties of more than two particles. A promising route is the use of the photon orbital angular momentum (OAM), which enables implementation of novel quantum information protocols, and the study of fundamentally new quantum states. To date, only two of such multidimensional particles have been entangled albeit with ever increasing dimensionality. Here we use pulsed spontaneous parametric downconversion (SPDC) to produce photon quadruplets that are entangled in their OAM, or transverse-mode degrees of freedom; and witness genuine multipartite Dicke-type entanglement. Apart from addressing foundational questions, this could find applications in quantum metrology, imaging, and secret sharing.Comment: 5 pages, 4 figure

Photoluminescence quantum efficiency of dense silicon nanocrystal ensembles in SiO2

The photoluminescence decay characteristics of silicon nanocrystals in dense ensembles fabricated by ion implantation into silicon dioxide are observed to vary in proportion to the calculated local density of optical states. A comparison of the experimental 1/e photoluminescence decay rates to the expected spontaneous emission rate modification yields values for the internal quantum efficiency and the intrinsic radiative decay rate of silicon nanocrystals. A photoluminescence quantum efficiency as high as 59%±9% is found for nanocrystals emitting at 750 nm at low excitation power. A power dependent nonradiative decay mechanism reduces the quantum efficiency at high pump intensity

Non-linear photonic crystals as a source of entangled photons

Non-linear photonic crystals can be used to provide phase-matching for frequency conversion in optically isotropic materials. The phase-matching mechanism proposed here is a combination of form birefringence and phase velocity dispersion in a periodic structure. Since the phase-matching relies on the geometry of the photonic crystal, it becomes possible to use highly non-linear materials. This is illustrated considering a one-dimensional periodic Al$_{0.4}$Ga$_{0.6}$As / air structure for the generation of 1.5 $\mu$m light. We show that phase-matching conditions used in schemes to create entangled photon pairs can be achieved in photonic crystals.Comment: 4 pages, 3 figure

Photon statistics from coupled quantum dots

We present an optical study of closely-spaced self-assembled InAs/GaAs quantum dots. The energy spectrum and correlations between photons subsequently emitted from a single pair provide not only clear evidence of coupling between the quantum dots but also insight into the coupling mechanism. Our results are in agreement with recent theories predicting that tunneling is largely suppressed between nonidentical quantum dots and that the interaction is instead dominated by dipole-dipole coupling and phonon-assisted energy transfer processes.Comment: 4 pages, 4 figures, to appear in Phys. Re