51 research outputs found
Strong interference effects in the resonant Auger decay of atoms induced by intense X-Ray fields
The theory of resonant Auger decay of atoms in a high intensity coherent
X-ray pulse is presented. The theory includes the coupling between the ground
state and the resonance due to an intense X-ray pulse, taking into account the
decay of the resonance and the direct photoionization of the ground state, both
populating the final ionic states coherently. The theory also considers the
impact of the direct photoionization of the resonance state itself which
typically populates highly-excited ionic states. The combined action of the
resonant decay and of the direct ionization of the ground state in the field
induces a non-hermitian time-dependent coupling between the ground and the
'dressed' resonance stats. The impact of these competing processes on the total
electron yield and on the 2s2p3p P spectator and
2s2p S participator Auger decay spectra of the Ne 1s3p
resonance is investigated. The role of the direct photoionization of the ground
state and of the resonance increases dramatically with the field intensity.
This results in strong interference effects with distinct patterns in the
electron spectra, different for the participator and spectator final states.Comment: 31 pages, 6 figure
Resonant Auger decay of the core-excited CO molecule in intense X-ray laser fields
The dynamics of the resonant Auger (RA) process of the core-excited
CO(1s) molecule in an intense X-ray laser field is
studied theoretically. The theoretical approach includes the analogue of the
conical intersections of the complex potential energy surfaces of the ground
and `dressed' resonant states due to intense X-ray pulses, taking into account
the decay of the resonance and the direct photoionization of the ground state,
both populating the same final ionic states coherently, as well as the direct
photoionization of the resonance state itself. The light-induced non-adiabatic
effect of the analogue of the conical intersections of the resulting complex
potential energy surfaces gives rise to strong coupling between the electronic,
vibrational and rotational degrees of freedom of the diatomic CO molecule. The
interplay of the direct photoionization of the ground state and of the decay of
the resonance increases dramatically with the field intensity. The coherent
population of a final ionic state via both the direct photoionization and the
resonant Auger decay channels induces strong interference effects with distinct
patterns in the RA electron spectra. The individual impact of these physical
processes on the total electron yield and on the CO electron
spectrum are demonstrated.Comment: 13 figs, 1 tabe
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