Non-local coherent coupling between excitons in a disordered quantum well

We investigated coherent coupling among multiple exciton resonances formed in a single disordered quantum well using the powerful electronic two-dimensional Fourier transform spectroscopy. Our experiment revealed clear signatures of non-local coherent coupling between the heavy-hole and light-hole excitons residing in regions that differ in thickness by one atomic layer. The experimental observation is qualitatively explained by spatial overlap between exciton linear response functions calculated within a single defect model

Locally defined quantum emission from epitaxial few-layer tungsten diselenide

Recently, single photons have been observed emanating from point defects in two-dimensional (2D) materials including WSe2, WS2, hexagonal-BN, and GaSe, with their energy residing in the direct electronic bandgap. Here, we report single photon emission from a nominal weakly emitting indirect bandgap 2D material through deterministic strain induced localization. A method is demonstrated to create highly spatially localized and spectrally well-separated defect emission sites in the 750-800nm regime in a continuous epitaxial film of few-layer WSe2 synthesized by a multistep diffusion-mediated gas source chemical vapor deposition technique. To separate the effects of mechanical strain from the substrate or dielectric-environment induced changes in the electronic structure, we created arrays of large isotropically etched ultrasharp silicon dioxide tips with spatial dimensions on the order of 10 mu m. We use bending based on the small radius of these tips-on the order of 4nm-to impart electronic localization effects through morphology alone, as the WSe2 film experiences a uniform SiO2 dielectric environment in the device geometry chosen for this investigation. When the continuous WSe2 film was transferred onto an array of SiO2 tips, an similar to 87% yield of localized emission sites on the tips was observed. The outcomes of this report provide fundamental guidelines for the integration of beyond-lab-scale quantum materials into photonic device architectures for all-optical quantum information applications.U. S. National Science Foundation [CAREER-1553987, REU-1560098]; FEI Company Graduate Fellowship [2018AU0058]; Laboratory Directed Research and Development Program of Los Alamos National Laboratory [20190516ECR]; Los Alamos National Laboratory; U. S. Department of Energy's NNSA [89233218CNA000001, 2DCC-MIP]; NSF [DMR-1539916]; Air Force Office of Scientific Research [FA9550-15RYCOR159]Open access articleThis item from the UA Faculty Publications collection is made available by the University of Arizona with support from the University of Arizona Libraries. If you have questions, please contact us at [email protected]