38 research outputs found
Ferromagnetic Domain Structure of La0.78Ca0.22MnO3 Single Crystals
The magneto-optical technique has been employed to observe spontaneous
ferromagnetic domain structures in La0.78Ca0.22MnO3 single crystals. The
magnetic domain topology was found to be correlated with the intrinsic twin
structure of the investigated crystals. With decreasing temperature the regular
network of ferromagnetic domains undergoes significant changes resulting in
apparent rotation of the domain walls in the temperature range of 70-150 K. The
apparent rotation of the domain walls can be understood in terms of the
Jahn-Teller deformation of the orthorhombic unit cell, accompanied by
additional twinning.Comment: 7 pages, 5 figures, to be published in PR
Spin dynamics of strongly-doped La_{1-x}Sr_xMnO_3
Cold neutron triple-axis measurements have been used to investigate the
nature of the long-wavelength spin dynamics in strongly-doped
LaSrMnO single crystals with =0.2 and 0.3. Both systems
behave like isotropic ferromagnets at low T, with a gapless ( meV)
quadratic dispersion relation . The values of the spin-wave
stiffness constant are large ( = 166.77 meV for =0.2
and D = 175.87 meV for =0.3), which directly shows that the
electron transfer energy for the band is large. exhibits a power law
behavior as a function of temperature, and appears to collapse as T -> T_C.
Nevertheless, an anomalously strong quasielastic central component develops and
dominates the fluctuation spectrum as T -> T_C. Bragg scattering indicates that
the magnetization near exhibits power law behavior, with for both systems, as expected for a three-dimensional ferromagnet.Comment: 4 pages (RevTex), 3 figures (encapsulated postscript
Confined spin waves reveal an assembly of nanosize domains in ferromagnetic La(1-x)CaxMnO3 (x=0.17,0.2)
We report a study of spin-waves in ferromagnetic LaCaMnO,
at concentrations x=0.17 and x=0.2 very close to the metallic transition
(x=0.225). Below T, in the quasi-metallic state (T=150K), nearly
q-independent energy levels are observed. They are characteristic of standing
spin waves confined into finite-size ferromagnetic domains, defined in {\bf a,
b) plane for x=0.17 and in all q-directions for x=0.2. They allow an estimation
of the domain size, a few lattice spacings, and of the magnetic coupling
constants inside the domains. These constants, anisotropic, are typical of an
orbital-ordered state, allowing to characterize the domains as "hole-poor". The
precursor state of the CMR metallic phase appears, therefore, as an assembly of
small orbital-ordered domains.Comment: 4 pages, 5 figure
Quantized spin waves in the metallic state of magnetoresistive manganites
High resolution spin waves measurements have been carried out in
ferromagnetic (F) La(1-x)(Sr,Ca)xMnO3 with x(Sr)=0.15, 0.175, 0.2, 0.3 and
x(Ca)=0.3. In all q-directions, close to the zone boundary, the spin wave
spectra consist of several energy levels, with the same values in the metallic
and the x\approx 1/8 ranges. Mainly the intensity varies, jumping from the
lower energy levels determined in the x\approx 1/8 range to the higher energy
ones observed in the metallic state. On the basis of a quantitative agreement
found for x(Sr)=0.15 in a model of ordered 2D clusters, the spin wave anomalies
of the metallic state can be interpreted in terms of quantized spin waves
within the same 2D clusters, embedded in a 3D matrix.Comment: 4 pages, 5 figure
Phase diagram and magnetic properties of LaCaMnO compound for
In this article a detailed study of LaCaMnO () phase diagram using powder x-ray diffraction and magnetization
measurements is presented. Unfortunately, in the related literature no properly
characterized samples have been used, with consequence the smearing of the real
physics in this complicated system. As the present results reveal, there are
two families of samples. The first family concerns samples prepared in
atmosphere ( Atm) which are all ferromagnetic with Curie
temperature rising with . The second family concerns samples, where a post
annealing in nearly zero oxygen partial pressure is applied. These samples show
a canted antiferromagnetic structure for below , while
for an unconventional ferromagnetic insulated phase is
present below . The most important difference between nonstoichiometric
and stoichiometric samples concerning the magnetic behavior, is the anisotropy
in the exchange interactions, in the stoichiometric samples putting forward the
idea that a new orbital ordered phase is responsible for the ferromagnetic
insulating regime in the LaCaMnO compound
First-order nature of the ferromagnetic phase transition in (La-Ca)MnO_3 near optimal doping
Neutron scattering has been used to study the nature of the ferromagnetic
transition in single crystals of La_0.7Ca_0.3MnO_3 and La_0.8Ca_0.2MnO_3, and
polycrystalline samples of La_0.67Ca_0.33MnO_3 and La_5/8Ca_3/8MnO_3 where the
naturally occurring O-16 can be replaced with the O-18 isotope. Small angle
neutron scattering on the x=0.3 single crystal reveals a discontinuous change
in the scattering at the Curie temperature for wave vectors below ~0.065 A^-1.
Strong relaxation effects are observed for this domain scattering, for the
magnetic order parameter, and for the quasielastic scattering, demonstrating
that the transition is not continuous in nature. There is a large oxygen
isotope effect observed for the T_C in the polycrystalline samples. For the
optimally doped x=3/8 sample we observed T_C(O-16)=266.5 K and T_C(O-18)=261.5
K at 90% O-18 substitution. The temperature dependence of the spin-wave
stiffness is found to be identical for the two samples despite changes in T_C.
Hence, T_C is not solely determined by the magnetic subsystem, but instead the
ferromagnetic phase is truncated by the formation of polarons which cause an
abrupt transition to the paramagnetic, insulating state. Application of
uniaxial stress in the x=0.3 single crystal sharply enhances the polaron
scattering at room temperature. Measurements of the phonon density-of-states
show only modest differences above and below T_C and between the two different
isotopic samples.Comment: 13 pages, 16 figures, submitted to Phys. Rev.
Influence of magnetic field on paramagnetic-ferromagnetic transition in LaCaMnO () crystal: ultrasonic and transport studies
The ultrasonic properties of LaCaMnO ()
with the Curie temperature about 200 K are studied. Temperature
dependences of longitudinal and transverse sound velocities were measured in
zero magnetic field and for different constant magnetic fields as well. The
ultrasonic study is supported by magnetic, resistive, magnetoresistive,
structural and other measurements of the sample that facilitate interpretation
of the results obtained. The magnetic field influence on sound properties found
in this study presents some new features of the interplay between the elastic
and magnetic properties of these compounds. It is shown that the
paramagnetic-ferromagnetic transition in the sample studied is first order, but
can become second order under the influence of applied magnetic field.Comment: submitted to Phys. Rev.
Approach to the metal-insulator transition in La(1-x)CaxMnO3 (0<x<.2): magnetic inhomogeneity and spin wave anomaly
We describe the evolution of the static and dynamic spin correlations of
LaCaMnO, for x=0.1, 0.125 and 0.2, where the system evolves
from the canted magnetic state towards the insulating ferromagnetic state,
approaching the metallic transition (x=0.22).
In the x=0.1 sample, the observation of two spin wave branches typical of two
distinct types of magnetic coupling, and of a modulation in the elastic diffuse
scattering characteristic of ferromagnetic inhomogeneities, confirms the static
and dynamic inhomogeneous features previously observed at x0.1. The
anisotropic q-dependence of the intensity of the low-energy spin wave suggests
a bidimensionnal character for the static inhomogeneities. At x=0.125, which
corresponds to the occurence of a ferromagnetic and insulating state, the two
spin wave branches reduce to a single one, but anisotropic. At this
concentration, an anomaly appears at {\bf q}=(1.25,1.25,0), that could be
related to an underlying periodicity, as arising from (1.5,1.5,0)
superstructures.
At x=0.2, the spin-wave branch is isotropic. In addition to the anomaly
observed at q, extra magnetic excitations are observed at larger q, forming
an optical branch. The two dispersion curves suggest an anti-crossing behavior
at some {\bf q'} value, which could be explained by a folding due to an
underlying perodicity involving four cubic lattice spacings