49 research outputs found
Nanotube field of C60 molecules in carbon nanotubes: atomistic versus continuous tube approach
We calculate the van der Waals energy of a C60 molecule when it is
encapsulated in a single-walled carbon nanotube with discrete atomistic
structure. orientational degrees of freedom and longitudinal displacements of
the molecule are taken into account, and several achiral and chiral carbon
nanotubes are considered. A comparison with earlier work where the tube was
approximated by a continuous cylindrical distribution of carbon atoms is made.
We find that such an approximation is valid for high and intermediate tube
radii; for low tube radii, minor chirality effects come into play. Three
molecular orientational regimes are found when varying the nanotube radius.Comment: 14 pages, 9 figures, accepted for publication in Phys. Rev.
How Sandcastles Fall
Capillary forces significantly affect the stability of sandpiles. We analyze
the stability of sandpiles with such forces, and find that the critical angle
is unchanged in the limit of an infinitely large system; however, this angle is
increased for finite-sized systems. The failure occurs in the bulk of the
sandpile rather than at the surface. This is related to a standard result in
soil mechanics. The increase in the critical angle is determined by the surface
roughness of the particles, and exhibits three regimes as a function of the
added-fluid volume. Our theory is in qualitative agreement with the recent
experimental results of Hornbaker et al., although not with the interpretation
they make of these results.Comment: 4 pages, 2 figures, revte
Temperature dependence of the charge carrier mobility in gated quasi-one-dimensional systems
The many-body Monte Carlo method is used to evaluate the frequency dependent
conductivity and the average mobility of a system of hopping charges,
electronic or ionic on a one-dimensional chain or channel of finite length. Two
cases are considered: the chain is connected to electrodes and in the other
case the chain is confined giving zero dc conduction. The concentration of
charge is varied using a gate electrode. At low temperatures and with the
presence of an injection barrier, the mobility is an oscillatory function of
density. This is due to the phenomenon of charge density pinning. Mobility
changes occur due to the co-operative pinning and unpinning of the
distribution. At high temperatures, we find that the electron-electron
interaction reduces the mobility monotonically with density, but perhaps not as
much as one might intuitively expect because the path summation favour the
in-phase contributions to the mobility, i.e. the sequential paths in which the
carriers have to wait for the one in front to exit and so on. The carrier
interactions produce a frequency dependent mobility which is of the same order
as the change in the dc mobility with density, i.e. it is a comparably weak
effect. However, when combined with an injection barrier or intrinsic disorder,
the interactions reduce the free volume and amplify disorder by making it
non-local and this can explain the too early onset of frequency dependence in
the conductivity of some high mobility quasi-one-dimensional organic materials.Comment: 9 pages, 8 figures, to be published in Physical Review
Aging in humid granular media
Aging behavior is an important effect in the friction properties of solid
surfaces. In this paper we investigate the temporal evolution of the static
properties of a granular medium by studying the aging over time of the maximum
stability angle of submillimetric glass beads. We report the effect of several
parameters on these aging properties, such as the wear on the beads, the stress
during the resting period, and the humidity content of the atmosphere. Aging
effects in an ethanol atmosphere are also studied. These experimental results
are discussed at the end of the paper.Comment: 7 pages, 9 figure
Nanoelectromechanical coupling in fullerene peapods probed via resonant electrical transport experiments
Fullerene peapods, that is carbon nanotubes encapsulating fullerene
molecules, can offer enhanced functionality with respect to empty nanotubes.
However, the present incomplete understanding of how a nanotube is affected by
entrapped fullerenes is an obstacle for peapods to reach their full potential
in nanoscale electronic applications. Here, we investigate the effect of C60
fullerenes on electron transport via peapod quantum dots. Compared to empty
nanotubes, we find an abnormal temperature dependence of Coulomb blockade
oscillations, indicating the presence of a nanoelectromechanical coupling
between electronic states of the nanotube and mechanical vibrations of the
fullerenes. This provides a method to detect the C60 presence and to probe the
interplay between electrical and mechanical excitations in peapods, which thus
emerge as a new class of nanoelectromechanical systems.Comment: 7 pages, 3 figures. Published in Nature Communications. Free online
access to the published version until Sept 30th, 2010, see
http://www.nature.com/ncomms/journal/v1/n4/abs/ncomms1034.htm
How to detect fluctuating order in the high-temperature superconductors
We discuss fluctuating order in a quantum disordered phase proximate to a
quantum critical point, with particular emphasis on fluctuating stripe order.
Optimal strategies for extracting information concerning such local order from
experiments are derived with emphasis on neutron scattering and scanning
tunneling microscopy. These ideas are tested by application to two model
systems - the exactly solvable one dimensional electron gas with an impurity,
and a weakly-interacting 2D electron gas. We extensively review experiments on
the cuprate high-temperature superconductors which can be analyzed using these
strategies. We adduce evidence that stripe correlations are widespread in the
cuprates. Finally, we compare and contrast the advantages of two limiting
perspectives on the high-temperature superconductor: weak coupling, in which
correlation effects are treated as a perturbation on an underlying metallic
(although renormalized) Fermi liquid state, and strong coupling, in which the
magnetism is associated with well defined localized spins, and stripes are
viewed as a form of micro-phase separation. We present quantitative indicators
that the latter view better accounts for the observed stripe phenomena in the
cuprates.Comment: 43 pages, 11 figures, submitted to RMP; extensively revised and
greatly improved text; one new figure, one new section, two new appendices
and more reference
Wet Granular Materials
Most studies on granular physics have focused on dry granular media, with no
liquids between the grains. However, in geology and many real world
applications (e.g., food processing, pharmaceuticals, ceramics, civil
engineering, constructions, and many industrial applications), liquid is
present between the grains. This produces inter-grain cohesion and drastically
modifies the mechanical properties of the granular media (e.g., the surface
angle can be larger than 90 degrees). Here we present a review of the
mechanical properties of wet granular media, with particular emphasis on the
effect of cohesion. We also list several open problems that might motivate
future studies in this exciting but mostly unexplored field.Comment: review article, accepted for publication in Advances in Physics;
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