Primary thermometry triad at 6 mK in mesoscopic circuits

Quantum physics emerge and develop as temperature is reduced. Although mesoscopic electrical circuits constitute an outstanding platform to explore quantum behavior, the challenge in cooling the electrons impedes their potential. The strong coupling of such micrometer-scale devices with the measurement lines, combined with the weak coupling to the substrate, makes them extremely difficult to thermalize below 10 mK and imposes in-situ thermometers. Here we demonstrate electronic quantum transport at 6 mK in micrometer-scale mesoscopic circuits. The thermometry methods are established by the comparison of three in-situ primary thermometers, each involving a different underlying physics. The employed combination of quantum shot noise, quantum back-action of a resistive circuit and conductance oscillations of a single-electron transistor covers a remarkably broad spectrum of mesoscopic phenomena. The experiment, performed in vacuum using a standard cryogen-free dilution refrigerator, paves the way toward the sub-millikelvin range with additional thermalization and refrigeration techniques.Comment: Article and Supplementar

Wigner and Kondo physics in quantum point contacts revealed by scanning gate microscopy

Quantum point contacts exhibit mysterious conductance anomalies in addition to well known conductance plateaus at multiples of 2e^2/h. These 0.7 and zero-bias anomalies have been intensively studied, but their microscopic origin in terms of many-body effects is still highly debated. Here we use the charged tip of a scanning gate microscope to tune in situ the electrostatic potential of the point contact. While sweeping the tip distance, we observe repetitive splittings of the zero-bias anomaly, correlated with simultaneous appearances of the 0.7 anomaly. We interpret this behaviour in terms of alternating equilibrium and non-equilibrium Kondo screenings of different spin states localized in the channel. These alternating Kondo effects point towards the presence of a Wigner crystal containing several charges with different parities. Indeed, simulations show that the electron density in the channel is low enough to reach one-dimensional Wigner crystallization over a size controlled by the tip position

Circuit Quantum Simulation of a Tomonaga-Luttinger Liquid with an Impurity

The Tomonaga-Luttinger liquid (TLL) concept is believed to generically describe the strongly-correlated physics of one-dimensional systems at low temperatures. A hallmark signature in 1D conductors is the quantum phase transition between metallic and insulating states induced by a single impurity. However, this transition impedes experimental explorations of real-world TLLs. Furthermore, its theoretical treatment, explaining the universal energy rescaling of the conductance at low temperatures, has so far been achieved exactly only for specific interaction strengths. Quantum simulation can provide a powerful workaround. Here, a hybrid metal-semiconductor dissipative quantum circuit is shown to implement the analogue of a TLL of adjustable electronic interactions comprising a single, fully tunable scattering impurity. Measurements reveal the renormalization group `beta-function' for the conductance that completely determines the TLL universal crossover to an insulating state upon cooling. Moreover, the characteristic scaling energy locating at a given temperature the position within this conductance renormalization flow is established over nine decades versus circuit parameters, and the out-of-equilibrium regime is explored. With the quantum simulator quality demonstrated from the precise parameter-free validation of existing and novel TLL predictions, quantum simulation is achieved in a strong sense, by elucidating interaction regimes which resist theoretical solutions.Comment: To be published in Phys. Rev.

Heat Coulomb Blockade of One Ballistic Channel

Quantum mechanics and Coulomb interaction dictate the behavior of small circuits. The thermal implications cover fundamental topics from quantum control of heat to quantum thermodynamics, with prospects of novel thermal machines and an ineluctably growing influence on nanocircuit engineering. Experimentally, the rare observations thus far include the universal thermal conductance quantum and heat interferometry. However, evidences for many-body thermal effects paving the way to markedly different heat and electrical behaviors in quantum circuits remain wanting. Here we report on the observation of the Coulomb blockade of electronic heat flow from a small metallic circuit node, beyond the widespread Wiedemann-Franz law paradigm. We demonstrate this thermal many-body phenomenon for perfect (ballistic) conduction channels to the node, where it amounts to the universal suppression of precisely one quantum of conductance for the transport of heat, but none for electricity. The inter-channel correlations that give rise to such selective heat current reduction emerge from local charge conservation, in the floating node over the full thermal frequency range ($\lesssim$temperature$\times k_\mathrm{B}/h$). This observation establishes the different nature of the quantum laws for thermal transport in nanocircuits.Comment: Letter: 5 pages including 3 figures; Methods: 3 pages and 4 figure

Heteroepitaxial growth of ferromagnetic MnSb(0001) films on Ge/Si(111) virtual substrates

Molecular beam epitaxial growth of ferromagnetic MnSb(0001) has been achieved on high quality, fully relaxed Ge(111)/Si(111) virtual substrates grown by reduced pressure chemical vapor deposition. The epilayers were characterized using reflection high energy electron diffraction, synchrotron hard X-ray diffraction, X-ray photoemission spectroscopy, and magnetometry. The surface reconstructions, magnetic properties, crystalline quality, and strain relaxation behavior of the MnSb films are similar to those of MnSb grown on GaAs(111). In contrast to GaAs substrates, segregation of substrate atoms through the MnSb film does not occur, and alternative polymorphs of MnSb are absent

Vanadyl phthalocyanines on graphene/SiC(0001): toward a hybrid architecture for molecular spin qubits

Vanadyl phthalocyanine (VOPc) contains a highly coherent spin S = ½, which is of interest for applications in quantum information. Preservation of long coherence times upon deposition on conductive materials is crucial for use of single-spin in devices. Here, we report a detailed investigation of the structural, electronic and magnetic properties of a hybrid architecture constituted by a monolayer film of VOPc molecules deposited on graphene/SiC(0001). Graphene (Gr) is a two-dimensional conductor with exceptional chemical stability, a property which we exploited here to preserve the spin of VOPc. Low temperature-scanning tunneling microscopy supported by density functional theory (DFT) simulations revealed that VOPc molecules were adsorbed intact on the Gr/SiC(0001) surface in a planar geometry assuming a unique configuration in which the vanadyl group is projected out toward the vacuum, different to that found commonly on other conductive surfaces. Furthermore, X-ray photoelectron spectroscopy and UV-photoelectron spectroscopy (flanked theoretically by DFT) showed that VOPc interact weakly with the Gr/SiC(0001) substrate to preserve its electronic configuration with the unpaired electron located on the V ion. These findings were confirmed by X-ray magnetic circular dichroism, revealing that the S = ½ character of the VOPc assembly on Gr/SiC(0001) was preserved, in agreement with the theoretical prediction. Hence, molecules could be adsorbed and used as qubits on substrates of technological importance, such as graphene. This new hybrid architecture could be employed for local investigation of static and dynamic spin properties and as molecular qubits for spintronic applications

Surface morphology and characterization of thin graphene films on SiC vicinal substrate

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