A new experimental procedure for characterizing quantum effects in small magnetic particle systems

A new experimental procedure is discussed, which aims at separating thermal from quantum behavior independently of the energy barrier distribution in small particle systems. Magnetization relaxation data measured between 60 mK and 5 K on a sample of nanoparticles is presented. The comparison between experimental data and numerical calculations shows a clear departure from thermal dynamics for our sample, which was not obvious without using the new procedure presented here.Comment: LaTeX source, 6 pages, 5 PostScript figure

Fluctuation-dissipation ratio of a spin glass in the aging regime

We present the first experimental determination of the time autocorrelation $C(t',t)$ of magnetization in the non-stationary regime of a spin glass. Quantitative comparison with the response, the magnetic susceptibility $\chi(t',t)$, is made using a new experimental setup allowing both measurements in the same conditions. Clearly, we observe a non-linear fluctuation-dissipation relation between $C$ and $\chi$, depending weakly on the waiting time $t'$. Following theoretical developments on mean-field models, and lately on short range models, it is predicted that in the limit of long times, the $\chi(C)$ relationship should become independent on $t'$. A scaling procedure allows us to extrapolate to the limit of long waiting times.Comment: 4 pages, 3 figure

A Search for Fluctuation-Dissipation Theorem Violations in Spin-Glasses from Susceptibility Data

We propose an indirect way of studying the fluctuation-dissipation relation in spin-glasses that only uses available susceptibility data. It is based on a dynamic extension of the Parisi-Toulouse approximation and a Curie-Weiss treatment of the average magnetic couplings. We present the results of the analysis of several sets of experimental data obtained from various samples.Comment: 7 pages, 4 figure

Thermopower in the strongly overdoped region of single-layer Bi2Sr2CuO6+d superconductor

The evolution of the thermoelectric power S(T) with doping, p, of single-layer Bi2Sr2CuO6+d ceramics in the strongly overdoped region is studied in detail. Analysis in term of drag and diffusion contributions indicates a departure of the diffusion from the T-linear metallic behavior. This effect is increased in the strongly overdoped range (p~0.2-0.28) and should reflect the proximity of some topological change.Comment: 4 pages, 4 figure

Extended droplet theory for aging in short-ranged spin glasses and a numerical examination

We analyze isothermal aging of a four dimensional Edwards-Anderson model in detail by Monte Carlo simulations. We analyze the data in the view of an extended version of the droplet theory proposed recently (cond-mat/0202110) which is based on the original droplet theory plus conjectures on the anomalously soft droplets in the presence of domain walls. We found that the scaling laws including some fundamental predictions of the original droplet theory explain well our results. The results of our simulation strongly suggest the separation of the breaking of the time translational invariance and the fluctuation dissipation theorem in agreement with our scenario.Comment: 27 pages, 39 epsfiles, revised versio

Extraction of the Spin Glass Correlation Length

The peak of the spin glass relaxation rate, S(t)=d{-M_{TRM}(t,t_w)}/H/{d ln t}, is directly related to the typical value of the free energy barrier which can be explored over experimental time scales. A change in magnetic field H generates an energy E_z={N_s}{X_fc}{H^2} by which the barrier heights are reduced, where X_{fc} is the field cooled susceptibility per spin, and N_s is the number of correlated spins. The shift of the peak of S(t) gives E_z, generating the correlation length, Ksi(t,T), for Cu:Mn 6at.% and CdCr_{1.7}In_{0.3}S_4. Fits to power law dynamics, Ksi(t,T)\propto {t}^{\alpha(T)} and activated dynamics Ksi(t,T) \propto {ln t}^{1/psi} compare well with simulation fits, but possess too small a prefactor for activated dynamics.Comment: 4 pages, 4 figures. Department of Physics, University of California, Riverside, California, and Service de Physique de l'Etat Condense, CEA Saclay, Gif sur Yvette, France. To appear in Phys. Rev. Lett. January 4, 199

Non-Fermi-Liquid Scaling in Ce(Ru_{0.5}Rh_{0.5})_2Si_2

We study the temperature and field dependence of the magnetic and transport properties of the non-Fermi-liquid compound Ce(Ru_{1-x}Rh_x)_2Si_2 at x=0.5. For fields $\lesssim$0.1T the experimental results show signatures of the presence of Kondo-disorder, expected to be large at this concentration. For larger fields, however, magnetic and transport properties are controlled by the coupling of the conduction electrons to critical spin-fluctuations. The temperature dependence of the susceptibility as well as the scaling properties of the magnetoresistance are in very good agreement with the predictions of recent dynamical mean-field theories of Kondo alloys close to a spin-glass quantum critical point.Comment: 4 pages, 4 figures. Improved discussion. To appear in Phys. Rev. Let

A Crash Course on Aging

In these lecture notes I describe some of the main theoretical ideas emerged to explain the aging dynamics. This is meant to be a very short introduction to aging dynamics and no previous knowledge is assumed. I will go through simple examples that allow one to grasp the main results and predictions.Comment: Lecture Notes (22 pages) given at "Unifying Concepts in Glass Physics III", Bangalore (2004); to be published in JSTA

Slow dynamics and aging in spin-glasses

Contribution presented by Eric Vincent in the Conference `Complex Behaviour of Glassy Systems', Sitges, Barcelona, Spain, June, 1996. It contains a review of the experimental results on Slow dynamics and aging in spin-glasses. It also presents their comparison with recent theoretical developments in the description of the out of equilibrium dynamics of disordered systems; namely, the trap model and the mean-field theory.Comment: 35 pages, 12 figures, macro lmamult.sty (included