140 research outputs found
Magnetic versus nonmagnetic doping effects on the magnetic ordering in the Haldane chain compound PbNi2V2O8
A study of an impurity driven phase-transition into a magnetically ordered
state in the spin-liquid Haldane chain compound PbNi2V2O8 is presented. Both,
macroscopic magnetization as well as 51V nuclear magnetic resonance (NMR)
measurements reveal that the spin nature of dopants has a crucial role in
determining the stability of the induced long-range magnetic order. In the case
of nonmagnetic (Mg2+) doping on Ni2+ spin sites (S=1) a metamagnetic transition
is observed in relatively low magnetic fields. On the other hand, the magnetic
order in magnetically (Co2+) doped compounds survives at much higher magnetic
fields and temperatures, which is attributed to a significant anisotropic
impurity-host magnetic interaction. The NMR measurements confirm the predicted
staggered nature of impurity-liberated spin degrees of freedom, which are
responsible for the magnetic ordering. In addition, differences in the
broadening of the NMR spectra and the increase of nuclear spin-lattice
relaxation in doped samples, indicate a diverse nature of electron spin
correlations in magnetically and nonmagnetically doped samples, which begin
developing at rather high temperatures with respect to the antiferromagnetic
phase transition.Comment: 10 pages, 7 figure
NMR and dc-susceptibility studies of NaVGe2O6
We report the results of measurements of the dc magnetic susceptibility
chi(T) and of the 23Na nuclear magnetic resonance (NMR) response of NaVGe2O6, a
material in which the V ions form a network of interacting one-dimensional spin
S=1 chains. The experiments were made at temperatures between 2.5 and 300 K.
The chi(T) data suggest that the formation of the expected low-temperature
Haldane phase is intercepted by an antiferromagnetic phase transition at 18 K.
The transition is also reflected in the 23Na NMR spectra and the corresponding
spin-lattice relaxation rate 1/T1(T). In the ordered phase, 1/T1(T) decreases
by orders of magnitude with decreasing temperature, indicating the formation of
a gap of the order of 12 K in the magnetic excitation spectrum.Comment: 10 pages, 15 figures; v2 with minor revisions of the tex
^{17}O and ^{51}V NMR for the zigzag spin-1 chain compound CaV2O4
V NMR studies on CaV2O4 single crystals and O NMR studies on
O-enriched powder samples are reported. The temperature dependences of
the O NMR line width and nuclear spin-lattice relaxation rate give
strong evidence for a long-range antiferromagnetic transition at Tn = 78 K in
the powder. Magnetic susceptibility measurements show that Tn = 69 K in the
crystals. A zero-field V NMR signal was observed at low temperatures (f
237 MHz at 4.2 K) in the crystals. The field swept spectra with the
field in different directions suggest the presence of two antiferromagnetic
substructures. Each substructure is collinear, with the easy axes of the two
substructures separated by an angle of 19(1) degree, and with their average
direction pointing approximately along the b-axis of the crystal structure. The
two spin substructures contain equal number of spins. The temperature
dependence of the ordered moment, measured up to 45 K, shows the presence of an
energy gap Eg in the antiferromagnetic spin wave excitation spectrum.
Antiferromagnetic spin wave theory suggests that Eg lies between 64 and 98 K.Comment: 11 pages, 14 figures. v2: 2 new figures; version published in Phys.
Rev.
Elastic properties of FeSi
Measurements of the sound velocities in a single crystal of FeSi were
performed in the temperature range 4-300 K. Elastic constants and
deviate from a quasiharmonic behavior at high temperature; whereas,
increases anomalously in the entire range of temperature, indicating a
change in the electron structure of this materia
Thermal and Dynamical Properties of the Two-band Hubbard Model Compared with FeSi
We study the two-band Hubbard model introduced by Fu and Doniach as a model
for FeSi which is suggested to be a Kondo insulator. Using the self-consistent
second-order perturbation theory combined with the local approximation which
becomes exact in the limit of infinite dimensions, we calculate the specific
heat, the spin susceptibility and the dynamical conductivity and point out that
the reduction of the energy gap due to correlation is not significant in
contrast to the previous calculation. It is also demonstrated that the gap at
low temperatures in the optical conductivity is filled up at a rather low
temperature than the gap size, which is consistent with the experiment.Comment: 6 pages, LaTeX, 7 PS figures included, uses RevTe
Correlation functions in the two-dimensional random-field Ising model
Transfer-matrix methods are used to study the probability distributions of
spin-spin correlation functions in the two-dimensional random-field Ising
model, on long strips of width sites, for binary field
distributions at generic distance , temperature and field intensity
. For moderately high , and of the order of magnitude used in
most experiments, the distributions are singly-peaked, though rather
asymmetric. For low temperatures the single-peaked shape deteriorates, crossing
over towards a double- ground-state structure. A connection is obtained
between the probability distribution for correlation functions and the
underlying distribution of accumulated field fluctuations. Analytical
expressions are in good agreement with numerical results for ,
low , not too small, and near G=1. From a finite-size {\it ansatz} at
, , averaged correlation functions are predicted to
scale with , . From numerical data we estimate y=0.875 \pm
0.025WR/L=1W \sim h_0^{\kappa} f(L h_0^u)\kappa \simeq 0.45u \simeq 0.8f(x)x \to \inftyW \sim
h_0^{\kappa}d=2$.Comment: RevTeX code for 8 pages, 7 eps figures, to appear in Physical Review
E (1999
Interesting magnetic properties of FeCoSi alloys
Solid solution between nonmagnetic narrow gap semiconductor FeSi and
diamagnetic semi-metal CoSi gives rise to interesting metallic alloys with
long-range helical magnetic ordering, for a wide range of intermediate
concentration. We report various interesting magnetic properties of these
alloys, including low temperature re-entrant spin-glass like behaviour and a
novel inverted magnetic hysteresis loop. Role of Dzyaloshinski-Moriya
interaction in the magnetic response of these non-centrosymmetric alloys is
discussed.Comment: 11 pages and 3 figure
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