Na atomic order, Co charge disproportionation and magnetism in Nax_{x}CoO2_{2} for large Na contents

We have synthesized and characterized four different stable phases of Na ordered Na$_{x}$CoO$_{2}$, for $0.65<x<0.8$. Above 100 K they display similar Curie-Weiss susceptibilities as well as ferromagnetic $q=0$ spin fluctuations in the CoO$_{2}$ planes revealed by $^{23}$Na NMR data. In all phases from $^{59}$Co NMR data we display evidences that the Co disproportionate already above 300 K into non magnetic Co$^{3+}$ and magnetic $\approx$Co$^{3.5+}$ sites on which holes delocalize. This allows us to understand that metallic magnetism is favored for these large Na contents. Below 100 K the phases differentiate, and a magnetic order sets in only for $x\gtrsim 0.75$ at $T_{N}=$22 K. We suggest that the charge order also governs the low $T$ energy scales and transverse couplings

Anode-Coupled Readout for Light Collection in Liquid Argon TPCs

This paper will discuss a new method of signal read-out from photon detectors in ultra-large, underground liquid argon time projection chambers. In this design, the signal from the light collection system is coupled via capacitive plates to the TPC wire-planes. This signal is then read out using the same cabling and electronics as the charge information. This greatly benefits light collection: it eliminates the need for an independent readout, substantially reducing cost; It reduces the number of cables in the vapor region of the TPC that can produce impurities; And it cuts down on the number of feed-throughs in the cryostat wall that can cause heat-leaks and potential points of failure. We present experimental results that demonstrate the sensitivity of a LArTPC wire plane to photon detector signals. We also simulate the effect of a 1 $\mu$s shaping time and a 2 MHz sampling rate on these signals in the presence of noise, and find that a single photoelectron timing resolution of $\sim$30 ns can be achieved.Comment: 16 pages, 15 figure

59Co NMR study of the Co states in superconducting and anhydrous cobaltates

$^{59}$Co NMR spectra in oriented powders of Na$_{0.35}$CoO$_{2}$ and in its hydrated superconducting phase (HSC) Na$_{0.35}$CoO$_{2}$,1.3H$_{2}$O reveal a single electronic Co state with identical $T$ independent NMR shift tensor. These phases differ markedly from Na$_{0.7}$CoO$_{2}$, in which we resolve 3 types of Co sites. The large T variation of their spin susceptibilities $\chi ^{s}$ and the anisotropy of the orbital susceptibility $\chi ^{orb}$ allow us to conclude that charge disproportionation occurs, in a non magnetic Co$^{3+}$ and two magnetic sites with about 0.3 and 0.7 holes in the $t_{2g}$ multiplet. The data are consistent with those for the single Co site in the anhydrous and HSC phase assuming the expected Co$^{3.65+}$ charge.Comment: 5 pages, 3 figures, accepted for publication in Phys. Rev. Let

Strong orientational effect of stretched aerogel on the 3He order parameter

Deformation of aerogel strongly modifies the orientation of the order parameter of superfluid 3He confined in aerogel. We used a radial squeezing of aerogel to keep the orbital angular momentum of the 3He Cooper pairs in the plane perpendicular to the magnetic field. We did not find strong evidence for a "polar" phase, with a nodal line along the equator of the Fermi surface, predicted to occur at large radial squeezing. Instead we observed 3He-A with a clear experimental evidence of the destruction of the long-range order by random anisotropy -- the Larkin-Imry-Ma effect. In 3He-B we observed and identified new modes of NMR, which are impossible to obtain in bulk 3He-B. One of these modes is characterized by a repulsive interaction between magnons, which is suitable for the magnon Bose-Einstein condensation (BEC).Comment: 4 pages, 3 figures, revtex, submitted to PR

The Effects of Dissolved Methane upon Liquid Argon Scintillation Light

In this paper we report on measurements of the effects of dissolved methane upon argon scintillation light. We monitor the light yield from an alpha source held 20 cm from a cryogenic photomultiplier tube (PMT) assembly as methane is injected into a high-purity liquid argon volume. We observe significant suppression of the scintillation light yield by dissolved methane at the 10 part per billion (ppb) level. By examining the late scintillation light time constant, we determine that this loss is caused by an absorption process and also see some evidence of methane-induced scintillation quenching at higher concentrations (50-100 ppb). Using a second PMT assembly we look for visible re-emission features from the dissolved methane which have been reported in gas-phase argon methane mixtures, and we find no evidence of visible re-emission from liquid-phase argon methane mixtures at concentrations between 10 ppb and 0.1%.Comment: 18 pages, 11 figures Updated to match published versio

Cu NMR evidence for enhanced antiferromagnetic correlations around Zn impurities in YBa2Cu3O6.7

Doping the high-Tc superconductor YBa2Cu3O6.7 with 1.5 % of non-magnetic Zn impurities in CuO2 planes is shown to produce a considerable broadening of 63Cu NMR spectra, as well as an increase of low-energy magnetic fluctuations detected in 63Cu spin-lattice relaxation measurements. A model-independent analysis demonstrates that these effects are due to the development of staggered magnetic moments on many Cu sites around each Zn and that the Zn-induced moment in the bulk susceptibility might be explained by this staggered magnetization. Several implications of these enhanced antiferromagnetic correlations are discussed.Comment: 4 pages including 2 figure

Ga-NMR local susceptibility of the kagome-based magnet SrCr_9pGa_(12-9p)O_19. A high temperature study

We report a high-$T$ Ga-NMR study in the kagome-based antiferromagnetic compound SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$ ($.81\leq p\leq .96$), and present a refined mean-field analysis of the high T local NMR susceptibility of Cr frustrated moments. We find that the intralayer kagome coupling is $J=86(6)$ K, and the interlayer coupling through non-kagome Cr moments is $J^{\prime }=69(7)$ K. The $J^{\prime}/J=0.80(1)$ ratio confirms the common belief that the frustrated entity is a pyrochlore slab.Comment: 8 pages, 4 figures Conference paper: Highly Frustrated Magnetism 2000, Waterloo (Canada) Submitted to Canadian Journal of Physic