Two-step phase changes in cubic relaxor ferroelectrics

The field-driven conversion between the zero-field-cooled frozen relaxor state and a ferroelectric state of several cubic relaxors is found to occur in at least two distinct steps, after a period of creep, as a function of time. The relaxation of this state back to a relaxor state under warming in zero field also occurs via two or more sharp steps, in contrast to a one-step relaxation of the ferroelectric state formed by field-cooling. An intermediate state can be trapped by interrupting the polarization. Giant pyroelectric noise appears in some of the non-equilibrium regimes. It is suggested that two coupled types of order, one ferroelectric and the other glassy, may be required to account for these data.Comment: 27 pages with 8 figures to appear in Phys. Rev.

Aging in the Relaxor Ferroelectric PMN/PT

The relaxor ferroelectric (PbMn$_{1/3}$Nb$_{2/3}$O$_3$)$_{1-x}$(PbTiO$_3$)$_{x}$, $x=0.1$, (PMN/PT(90/10)) is found to exhibit several regimes of complicated aging behavior. Just below the susceptibility peak there is a regime exhibiting rejuvenation but little memory. At lower temperature, there is a regime with mainly cumulative aging, expected for simple domain-growth. At still lower temperature, there is a regime with both rejuvenation and memory, reminiscent of spin glasses. PMN/PT (88/12) is also found to exhibit some of these aging regimes. This qualitative aging behavior is reminiscent of that seen in reentrant ferromagnets, which exhibit a crossover from a domain-growth ferromagnetic regime into a reentrant spin glass regime at lower temperatures. These striking parallels suggest a picture of competition in PMN/PT (90/10) between ferroelectric correlations formed in the domain-growth regime with glassy correlations formed in the spin glass regime. PMN/PT (90/10) is also found to exhibit frequency-aging time scaling of the time-dependent part of the out-of-phase susceptibility for temperatures 260 K and below. The stability of aging effects to thermal cycles and field perturbations is also reported.Comment: 8 pages RevTeX4, 11 figures; submitted to Phys. Rev.

Nontrivial dependence of dielectric stiffness and SHG on dc bias in relaxors and dipole glasses

Dielectric permittivity and Second Harmonic Generation (SHG) studies in the field-cooled mode show a linear dependence of dielectric stiffness (inverse dielectric permittivity) on dc bias in PMN-PT crystals and SHG intensity in KTaO$_{3}$:Li at small Li concentrations. We explain this unusual result in the framework of a theory of transverse, hydrodynamic-type, instability of local polarization.Comment: 5 figure

Barkhausen Noise in a Relaxor Ferroelectric

Barkhausen noise, including both periodic and aperiodic components, is found in and near the relaxor regime of a familiar relaxor ferroelectric, PbMg$_{1/3}$Nb$_{2/3}$O$_3$, driven by a periodic electric field. The temperature dependences of both the amplitude and spectral form show that the size of the coherent dipole moment changes shrink as the relaxor regime is entered, contrary to expectations based on some simple models.Comment: 4 pages RevTeX4, 5 figures; submitted to Phys Rev Let

Dielectric nonlinearity of relaxor ferroelectric ceramics at low ac drives

Dielectric nonlinear response of (PbMg$_{1/3}$Nb$_{2/3}$O$_3$)$_{0.9}$(PbTiO$_3$)$_{0.1}$ (0.9PMN-0.1PT) relaxor ceramics was investigated under different ac drive voltages. It was observed that: (i) the dielectric permittivity is independent on ac field amplitude at high temperatures; (ii) with increasing ac drive, the permittivity maximum increases, and the temperature of the maximum shifts to lower temperature; (iii) the nonlinear effect is weakened when the measurement frequency increases. The influences of increasing ac drive were found to be similar to that of decreasing frequency. It is believed that the dielectric nonlinearities of relaxors at low drives can be explained by the phase transition theory of ergodic space shrinking in succession. A Monte Carlo simulation was performed on the flips of micro polarizations at low ac drives to verify the theory.Comment: Submitted to J. Phys.: Cond. Matte

Effects of ac-field amplitude on the dielectric susceptibility of relaxors

The thermally activated flips of the local spontaneous polarization in relaxors were simulated to investigate the effects of the applied-ac-field amplitude on the dielectric susceptibility. It was observed that the susceptibility increases with increasing the amplitude at low temperatures. At high temperatures, the susceptibility experiences a plateau and then drops. The maximum in the temperature dependence of susceptibility shifts to lower temperatures when the amplitude increases. A similarity was found between the effects of the amplitude and frequency on the susceptibility.Comment: 8 pages, 7 figures, Phys. Rev. B (in July 1st

Soft Phonon Anomalies in the Relaxor Ferroelectric Pb(Zn_1/3Nb_2/3)_0.92Ti_0.08O_3

Neutron inelastic scattering measurements of the polar TO phonon mode dispersion in the cubic relaxor Pb(Zn_1/3Nb_2/3)_0.92Ti_0.08O_3 at 500K reveal anomalous behavior in which the optic branch appears to drop precipitously into the acoustic branch at a finite value of the momentum transfer q=0.2 inverse Angstroms, measured from the zone center. We speculate this behavior is the result of nanometer-sized polar regions in the crystal.Comment: 4 pages, 4 figure

Aging and scaling laws in β\beta-hydroquinone-clathrate

The dielectric permittivity of the orientational glass methanol(x=0.73)-$\beta$-hydroquinone-clathrate has been studied as function of temperature and waiting time using different temperature-time-protocols. We study aging, rejuvenation and memory effects in the glassy phase and discuss similarities and differences to aging in spin-glasses. We argue that the diluted methanol-clathrate, although conceptually close to its magnetic pendants, takes an intermediate character between a true spin-glass and a pure random field system

X-ray-emitting Atmospheres of B2 Radio Galaxies

We report ROSAT PSPC spatial and spectral analysis of the eight B2 radio galaxies NGC 315, NGC 326, 4C 35.03, B2 0326+39, NGC 2484, B2 1040+31, B2 1855+37, and 3C 449, expected to be representative of the class of low-power radio galaxies. Multiple X-ray components are present in each, and the gas components have a wide range of linear sizes and follow an extrapolation of the cluster X-ray luminosity/temperature correlation, implying that there is no relationship between the presence of a radio galaxy and the gas fraction of the environment. No large-scale cooling flows are found. There is no correlation of radio-galaxy size with the scale or density of the X-ray atmosphere. This suggests that it is processes on scales less than those of the overall gaseous environments which are the major influence on radio-source dynamics. The intergalactic medium is usually sufficient to confine the outer parts of the radio structures, in some cases even to within 5 kpc of the core. In the case of NGC 315, an extrapolation suggests that the pressure of the atmosphere may match the minimum pressure in the radio source over a factor of about 40 in linear size (a factor of about 1600 in pressure).Comment: 34 pages, including 10 figures, using aasms4.sty To appear in the Ap

Anomalous transverse acoustic phonon broadening in the relaxor ferroelectric Pb(Mg_1/3Nb_2/3)O_3

The intrinsic linewidth $\Gamma_{TA}$ of the transverse acoustic (TA) phonon observed in the relaxor ferroelectric compound Pb(Mg$_{1/3}$Nb$_{2/3})_{0.8}$Ti$_{0.2}$O$_3$ (PMN-20%PT) begins to broaden with decreasing temperature around 650 K, nearly 300 K above the ferroelectric transition temperature $T_c$ ($\sim 360$ K). We speculate that this anomalous behavior is directly related to the condensation of polarized, nanometer-sized, regions at the Burns temperature $T_d$. We also observe the ``waterfall'' anomaly previously seen in pure PMN, in which the transverse optic (TO) branch appears to drop precipitously into the TA branch at a finite momentum transfer $q_{wf} \sim 0.15$ \AA$^{-1}$. The waterfall feature is seen even at temperatures above $T_d$. This latter result suggests that the PNR exist as dynamic entities above $T_d$.Comment: 6 pages, 4 figure