Pressure induced enhancement of ferroelectricity in multiferroic RRMn2_2O5_5(RR=Tb,Dy, and Ho)

Measurements of ferroelectric polarization and dielectric constant were done on $R$Mn$_2$O$_5$ ($R$=Tb, Dy, and Ho) with applied hydrostatic pressures of up to 18 kbar. At ambient pressure, distinctive anomalies were observed in the temperature profile of both physical properties at critical temperatures marking the onset of long range AFM order (T$_{N1}$), ferroelectricity (T$_{C1}$) as well as at temperatures when anomalous changes in the polarization, dielectric constant and spin wave commensurability have been previously reported. In particular, the step in the dielectric constant at low temperatures (T$_{C2}$), associated with both a drop in the ferroelectric polarization and an incommensurate magnetic structure, was shown to be suddenly quenched upon passing an $R$-dependent critical pressure. This was shown to correlate with the stabilization of the high ferroelectric polarization state which is coincident with the commensurate magnetic structure. The observation is suggested to be due to a pressure induced phase transition into a commensurate magnetic structure as exemplified by the pressure-temperature ($p$-$T$) phase diagrams constructed in this work. The $p$-$T$ phase diagrams are determined for all three compounds.Comment: 8 pages, 6 figures, submitted for review in Phys. Rev.

Strong spin-lattice coupling in multiferroic HoMnO3_{3}: Thermal expansion anomalies and pressure effect

Evidence for a strong spin-lattice coupling in multiferroic HoMnO_3 is derived from thermal expansion measurements along a- and c-axis. The magnetoelastic effect results in sizable anomalies of the thermal expansivities at the antiferromagnetic (T_N) and the spin rotation (T_{SR}) transition temperatures as well as in a negative c-axis expansivity below room temperature. The coupling between magnetic orders and dielectric properties below T_N is explained by the lattice strain induced by the magnetoelastic effect. At T_{SR} various physical quantities show discontinuities that are thermodynamically consistent with a first order phase transition

Low temperature dielectric anomalies in HoMnO_3: The complex phase diagram

The dielectric constant of multiferroic hexagonal HoMnO_3 exhibits an unprecedented diversity of anomalies at low temperatures (1.8 K< T <10 K) and under external magnetic fields related to magnetic phase transitions in the coupled system of Ho moments, Mn spins, and ferroelectric polarization. The derived phase diagram is far more complex than previously assumed including reentrant phases, phase transitions with distinct thermal and field hysteresis, as well as several multicritical points. Magnetoelastic interactions introduce lattice anomalies at the magnetic phase transitions. The re-evaluation of the T-H phase diagram of HoMnO_3 is demanded.Comment: 12 pages, 3 figure

Unusual Field-Dependence of the Intragrain Superconductive Transition in RuSr2EuCu2O8

A narrow intragrain phase-lock transition was observed in RuSr2EuCu2O8 under a magnetic field H up to a few Tesla. The corresponding transition temperature, T2, decreases rapidly (about 100 K/T at low fields) with H indicating that the grains of RuSr2EuCu2O8 behave like a Josephson-junction-array instead of a homogeneous bulk superconductor. Our data suggest that the bulk superconducting transition may occur on a length scale well below the grain size of 2 to 6 micrometer