Commensurate Fluctuations in the Pseudogap and Incommensurate spin-Peierls Phases of TiOCl

X-ray scattering measurements on single crystals of TiOCl reveal the presence of commensurate dimerization peaks within both the incommensurate spin-Peierls phase and the so-called pseudogap phase above T_c2. This scattering is relatively narrow in Q-space indicating long correlation lengths exceeding ~ 100 A below T* ~ 130 K. It is also slightly shifted in Q relative to that of the commensurate long range ordered state at the lowest temperatures, and it coexists with the incommensurate Bragg peaks below T_c2. The integrated scattering over both commensurate and incommensurate positions evolves continuously with decreasing temperature for all temperatures below T* ~ 130 K.Comment: To appear in Physical Review B: Rapid Communications. 5 page

Fluctuations of Entropy Production in Partially Masked Electric Circuits: Theoretical Analysis

In this work we perform theoretical analysis about a coupled RC circuit with constant driven currents. Starting from stochastic differential equations, where voltages are subject to thermal noises, we derive time-correlation functions, steady-state distributions and transition probabilities of the system. The validity of the fluctuation theorem (FT) is examined for scenarios with complete and incomplete descriptions.Comment: 4 pages, 1 figur

Suppression of the commensurate spin-Peierls state in Sc-doped TiOCl

We have performed x-ray scattering measurements on single crystals of the doped spin-Peierls compound Ti(1-x)Sc(x)OCl (x = 0, 0.01, 0.03). These measurements reveal that the presence of non-magnetic dopants has a profound effect on the unconventional spin-Peierls behavior of this system, even at concentrations as low as 1%. Sc-doping suppresses commensurate fluctuations in the pseudogap and incommensurate spin-Peierls phases of TiOCl, and prevents the formation of a long-range ordered spin-Peierls state. Broad incommensurate scattering develops in the doped compounds near Tc2 ~ 93 K, and persists down to base temperature (~ 7 K) with no evidence of a lock-in transition. The width of the incommensurate dimerization peaks indicates short correlation lengths on the order of ~ 12 angstroms below Tc2. The intensity of the incommensurate scattering is significantly reduced at higher Sc concentrations, indicating that the size of the associated lattice displacement decreases rapidly as a function of doping.Comment: 7 pages, 5 figure

Momentum Distribution for Bosons with Positive Scattering Length in a Trap

The coordinate-momentum double distribution function $\rho ({\bf r}, {\bf p}) d^{3}rd^{3}p$ is calculated in the local density approximation for bosons with positive scattering length $a$ in a trap. The calculation is valid to the first order of $a$. To clarify the meaning of the result, it is compared for a special case with the double distribution function $\rho_{w}d^{3} rd^{3}p$ of Wigner.Comment: Latex fil

Giant phonon anomalies in the pseudo-gap phase of TiOCl

We report infrared and Raman spectroscopy results of the spin-1/2 quantum magnet TiOCl. Giant anomalies are found in the temperature dependence of the phonon spectrum, which hint to unusual coupling of the electronic degrees of freedom to the lattice. These anomalies develop over a broad temperature interval, suggesting the presence of an extended fluctuation regime. This defines a pseudo-gap phase, characterized by a local spin-gap. Below 100 K a dimensionality cross-over leads to a dimerized ground state with a global spin-gap of about 2$\Delta_{spin}\approx$~430 K.Comment: 4 pages, 3 figures, for further information see http://www.peter-lemmens.d