993 research outputs found
Spin phonon coupling in frustrated magnet CdCrO
The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function
temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the
paramagnetic phase as temperature is lowered below 100 K and then split into a
singlet and doublet in the low T antiferromagnetic phase which is tetragonally
distorted to relieve the geometric frustration in the pyrochlore lattice of
Cr ions. The phonon splitting is inconsistent with the simple increase
(decrease) in the force constants due to deceasing (increasing) bond lengths in
the tetragonal phase. Rather they correspond to changes in the force constants
due to the magnetic order in the antiferromagnetic state. The phonon splitting
in this system is opposite of that observed earlier in ZnCr2O4 as predicted by
theory. The magnitude of the splitting gives a measure of the spin phonon
coupling strength which is smaller than in the case of ZnCr2O4.Comment: 4.2 pages, 4 figures, 1 reference added, submmite
Colossal magnon-phonon coupling in multiferroic EuYMnO
We report the spectra of magnetically induced electric dipole absorption in
EuYMnO from temperature dependent far infrared
spectroscopy (10-250 cm). These spectra, which occur only in the
polarization, consist of two relatively narrow electromagnon features that
onset at K and a broad absorption band that persists to
temperatures well above K. The observed excitations account for the
step up of the static dielectric constant in the ferroelectric phase. The
electromagnon at 80 cm is observed to be strongly coupled to the nearby
lowest optical phonon which transfers more than 1/2 of its spectral weight to
the magnon. We attribute the origin of the broad background absorption to the
two magnon emission decay process of the phonon.Comment: 4 pages, 3 figure
Effect of magnetic order on the superfluid response of single-crystal ErNiBC: A penetration depth study
We report measurements of the in-plane magnetic penetration depth (T) in single crystals of ErNiBC down to 0.1 K using
a tunnel-diode based, self-inductive technique at 21 MHz. We observe four
features: (1) a slight dip in (T) at the Nel
temperature = 6.0 K, (2) a peak at = 2.3 K, where a weak
ferromagnetic component sets in, (3) another maximum at 0.45 K, and (4) a final
broad drop down to 0.1 K. Converting to superfluid density , we see
that the antiferromagnetic order at 6 K only slightly depresses
superconductivity. We seek to explain some of the above features in the context
of antiferromagnetic superconductors, where competition between the
antiferromagnetic molecular field and spin fluctuation scattering determines
increased or decreased pairbreaking. Superfluid density data show only a slight
decrease in pair density in the vicinity of the 2.3 K feature, thus supporting
other evidences against bulk ferromagnetism in this temperature range.Comment: 15 pages, 5 figure
Grand Rounds: An Outbreak of Toxic Hepatitis among Industrial Waste Disposal Workers
CONTEXT: Industrial waste (which is composed of various toxic chemicals), changes to the disposal process, and addition of chemicals should all be monitored and controlled carefully in the industrial waste industry to reduce the health hazard to workers. CASE PRESENTATION: Five workers in an industrial waste plant developed acute toxic hepatitis, one of whom died after 3 months due to fulminant hepatitis. In the plant, we detected several chemicals with hepatotoxic potential, including pyridine, dimethylformamide, dimethylacetamide, and methylenedianiline. The workers had been working in the high-vapor-generating area of the plant, and the findings of pathologic examination showed typical features of acute toxic hepatitis. DISCUSSION: Infectious hepatitis and drug-induced hepatitis were excluded by laboratory findings, as well as the clinical course of hepatitis. All cases of toxic hepatitis in this plant developed after the change of the disposal process to thermochemical reaction–type treatment using unslaked lime reacted with industrial wastes. During this chemical reaction, vapor containing several toxic materials was generated. Although we could not confirm the definitive causative chemical, we suspect that these cases of hepatitis were caused by one of the hepatotoxic agents or by a synergistic interaction among several of them. RELEVANCE TO CLINICAL OR PROFESSIONAL PRACTICE: In the industrial waste treatment process, the danger of developing toxic hepatitis should be kept in mind, because any subtle change of the treatment process can generate various toxic materials and threaten the workers’ health. A mixture of hepatotoxic chemicals can induce clinical manifestations that are quite different from those predicted by the toxic property of a single agent
Coupling between magnon and ligand-field excitations in magnetoelectric Tb3Fe5O12 garnet
The spectra of far-infrared transmission in Tb3Fe5O12 magnetoelectric single
crystals have been studied in the range between 15 and 100 cm-1, in magnetic
fields up to 10 T, and for temperatures between 5 and 150 K. We attribute some
of the observed infrared-active excitations to electric-dipole transitions
between ligand-field split states of Tb3+ ions. Anticrossing between the
magnetic exchange excitation and the ligand-field transition occurs at the
temperature between 60 and 80 K. The corresponding coupling energy for this
interaction is 6 cm-1. Temperature-induced softening of the hybrid IR
excitation correlates with the increase of the static dielectric constant. We
discuss the possibility for hybrid excitations of magnons and ligand-field
states and their possible connection to the magnetoelectric effect in
Tb3Fe5O12.Comment: submitted to Phys. Rev. B on May 15th, 201
Collective magnetism at multiferroic vortex domain walls
Topological defects have been playgrounds for many emergent phenomena in
complex matter such as superfluids, liquid crystals, and early universe.
Recently, vortex-like topological defects with six interlocked structural
antiphase and ferroelectric domains merging into a vortex core were revealed in
multiferroic hexagonal manganites. Numerous vortices are found to form an
intriguing self-organized network. Thus, it is imperative to find out the
magnetic nature of these vortices. Using cryogenic magnetic force microscopy,
we discovered unprecedented alternating net moments at domain walls around
vortices that can correlate over the entire vortex network in hexagonal ErMnO3
The collective nature of domain wall magnetism originates from the
uncompensated Er3+ moments and the correlated organization of the vortex
network. Furthermore, our proposed model indicates a fascinating phenomenon of
field-controllable spin chirality. Our results demonstrate a new route to
achieving magnetoelectric coupling at domain walls in single-phase
multiferroics, which may be harnessed for nanoscale multifunctional devices.Comment: 18 pages, 10 figure
Origin of electromagnon excitations in \textit{R}MnO
The origin of electromagnon excitations in cycloidal \textit{R}MnO is
explained in terms of the Heisenberg coupling between spins despite the fact
that the static polarization arises from the much weaker Dzyaloshinskii-Moriya
(DM) exchange interaction. We present a model that incorporates structural
characteristics of this family of manganites that is confirmed by far infrared
transmission data as a function of temperature and magnetic field and inelastic
neutron scattering results. A deep connection is found between the
magnetoelectric dynamics of the spiral phase and the static magnetoelectric
coupling in the collinear E-phase of this family of manganites.Comment: 4 pages, 3 figures, submitte
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