The role of crosslinking density in surface stress and surface energy of soft solids

Surface stress and surface energy are two fundamental parameters that determine the surface properties of any materials. While it is commonly believed that the surface stress and surface energy of liquids are identical, the relationship between the two parameters in soft polymeric gels remains debatable. In this work, we measured the surface stress and surface energy of soft silicone gels with varying weight ratios of crosslinkers in soft wetting experiments. Above a critical density, $k_0$, the surface stress was found to increase significantly with crosslinking density while the surface energy remained unchanged. In this regime, we can estimate a non-zero surface elastic modulus that also increases with the ratio of crosslinkers. By comparing the surface mechanics of the soft gels with their bulk rheology, the surface properties near the critical density $k_0$ were found to be closely related to the underlying percolation transition of the polymer networks.Comment: 9 pages, 7 figure

Alpha Decay Width of 212^{212}Po from a quartetting wave function approach

A microscopic calculation of $\alpha$-cluster preformation probability and $\alpha$ decay width in the typical $\alpha$ emitter $^{212}$Po is presented. Results are obtained by improving a recent approach to describe $\alpha$ preformation in $^{212}$Po [Phys. Rev. C 90, 034304 (2014)] implementing four-nucleon correlations (quartetting). Using the actually measured density distribution of the $^{208}$ Pb core, the calculated alpha decay width of $^{212}$Po agrees fairly well with the measured one.Comment: 7 pages, 5 figures, 1 table, submitted to Phys. Rev.