175 research outputs found
Dynamical Structure Factors for Dimerized Spin Systems
We discuss the transition strength between the disordered ground state and
the basic low-lying triplet excitation for interacting dimer materials by
presenting theoretical calculations and series expansions as well as inelastic
neutron scattering results for the material KCuCl_3. We describe in detail the
features resulting from the presence of two differently oriented dimers per
unit cell and show how energies and spectral weights of the resulting two modes
are related to each other. We present results from the perturbation expansion
in the interdimer interaction strength and thus demonstrate that the wave
vector dependence of the simple dimer approximation is modified in higher
orders. Explicit results are given in 10th order for dimers coupled in 1D, and
in 2nd order for dimers coupled in 3D with application to KCuCl_3 and TlCuCl_3.Comment: 17 pages, 6 figures, part 2 is based on cond-mat/021133
Field-Induced Magnetic Ordering in the Quantum Spin System KCuCl
KCuCl is a three-dimensional coupled spin-dimer system and has a singlet
ground state with an excitation gap K. High-field
magnetization measurements for KCuCl have been performed in static magnetic
fields of up to 30 T and in pulsed magnetic fields of up to 60 T. The entire
magnetization curve including the saturation region was obtained at K.
From the analysis of the magnetization curve, it was found that the exchange
parameters determined from the dispersion relations of the magnetic excitations
should be reduced, which suggests the importance of the renormalization effect
in the magnetic excitations. The field-induced magnetic ordering accompanied by
the cusplike minimum of the magnetization was observed as in the isomorphous
compound TlCuCl. The phase boundary was almost independent of the field
direction, and is represented by the power law. These results are consistent
with the magnon Bose-Einstein condensation picture for field-induced magnetic
ordering.Comment: 9 pages, 7 figures, 9 eps files, revtex styl
Pasture Management in the US Midwest – An Assessment of Current Practices and Future Opportunities
Managed grazing offers significant potential to improve the sustainability of livestock farms in the US Midwest, however the benefits of managed grazing are largely influenced by the management practices employed on farm. The objective of this study was to gain an understanding of current grazing practices on Midwest farms and to identify the knowledge and support needs of graziers. A total of 185 responses were received from a range of different enterprises including dairy, beef, and sheep production. Results show a substantial degree of variation in grazing management practices between respondents and highlights significant scope for improvement on farms particularly in the areas of pasture measurement and budgeting, and grazing infrastructure. Reported benefits of managed grazing included lower environmental impact, better pasture and animal performance, better animal health and welfare, and lower costs. Challenges with managed grazing included time and labor input, maintaining pasture quantity and quality during the grazing season, adverse weather conditions such as excessive rain and drought, and animal health challenges such as heat stress, parasites and in some cases coyotes. The study highlighted opportunities for research and extension providers to better support farmers with information and advice and identified knowledge gaps in areas such as pasture species selection, soil fertility, grazing infrastructure, pasture budgeting, legumes, and pasture measurement. The study successfully gained an insight into graziers in the Midwest, the outputs of which, will be valuable to a number of key stakeholders going forward, including researchers, extension agents, farmers and policy makers
Pressure-Induced Magnetic Quantum Phase Transition in Gapped Spin System KCuCl3
Magnetization and neutron elastic scattering measurements under a hydrostatic
pressure were performed on KCuCl3, which is a three-dimensionally coupled spin
dimer system with a gapped ground state. It was found that an intradimer
interaction decreases with increasing pressure, while the sum of interdimer
interactions increases. This leads to the shrinkage of spin gap. A quantum
phase transition from a gapped state to an antiferromagnetic state occurs at Pc
? 8.2 kbar. For P > P c, magnetic Bragg reflections were observed at reciprocal
lattice points equivalent to those for the lowest magnetic excitation at zero
pressure. This confirms that the spin gap decreases and closes under applied
pressure.Comment: 7 pages, 10 figures, submitted to J. Phys. Soc. Jp
Field- and pressure-induced magnetic quantum phase transitions in TlCuCl_3
Thallium copper chloride is a quantum spin liquid of S = 1/2 Cu^2+ dimers.
Interdimer superexchange interactions give a three-dimensional magnon
dispersion and a spin gap significantly smaller than the dimer coupling. This
gap is closed by an applied hydrostatic pressure of approximately 2kbar or by a
magnetic field of 5.6T, offering a unique opportunity to explore the both types
of quantum phase transition and their associated critical phenomena. We use a
bond-operator formulation to obtain a continuous description of all disordered
and ordered phases, and thus of the transitions separating these. Both
pressure- and field-induced transitions may be considered as the Bose-Einstein
condensation of triplet magnon excitations, and the respective phases of
staggered magnetic order as linear combinations of dimer singlet and triplet
modes. We focus on the evolution with applied pressure and field of the
magnetic excitations in each phase, and in particular on the gapless
(Goldstone) modes in the ordered regimes which correspond to phase fluctuations
of the ordered moment. The bond-operator description yields a good account of
the magnetization curves and of magnon dispersion relations observed by
inelastic neutron scattering under applied fields, and a variety of
experimental predictions for pressure-dependent measurements.Comment: 20 pages, 17 figure
Frustration-Induced Two Dimensional Quantum Disordered Phase in Piperazinium Hexachlorodicuprate
Piperazinium Hexachlorodicuprate (PHCC) is shown to be a frustrated
quasi-two-dimensional quantum Heisenberg antiferromagnet with a gapped
spectrum. Zero-field inelastic neutron scattering and susceptibility and
specific heat measurements as a function of applied magnetic field are
presented. At T = 1.5 K, the magnetic excitation spectrum is dominated by a
single propagating mode with a gap, Delta = 1 meV, and bandwidth of
approximately 1.8 meV in the (h0l) plane. The mode has no dispersion along the
b* direction indicating that neighboring a-c planes of the triclinic structure
are magnetically decoupled. The heat capacity shows a reduction of the gap as a
function of applied magnetic field in agreement with a singlet-triplet
excitation spectrum. A field-induced ordered phase is observed in heat capacity
and magnetic susceptibility measurements for magnetic fields greater than H_c1
approximately equal to 7.5 Tesla. Analysis of the neutron scattering data
reveals the important exchange interactions and indicates that some of these
are highly frustrated.Comment: 13 pages with 14 figures, 7 pages of text, 6 pages of figures.
Submitted to Phys. Rev. B 4/7/2001. email comments to [email protected] or
[email protected]
Three-Dimensional Ordering in Weakly Coupled Antiferromagnetic Ladders and Chains
A theoretical description is presented for low-temperature magnetic-field
induced three-dimensional (3D) ordering transitions in strongly anisotropic
quantum antiferromagnets, consisting of weakly coupled antiferromagnetic
spin-1/2 chains and ladders. First, effective continuum field theories are
derived for the one-dimensional subsystems. Then the Luttinger parameters,
which determine the low-temperature susceptibilities of the chains and ladders,
are calculated from the Bethe ansatz solution for these effective models. The
3D ordering transition line is obtained using a random phase approximation for
the weak inter-chain (inter-ladder) coupling. Finally, considering a Ginzburg
criterion, the fluctuation corrections to this approach are shown to be small.
The nature of the 3D ordered phase resembles a Bose condensate of integer-spin
magnons. It is proposed that for systems with higher spin degrees of freedom,
e.g. N-leg spin-1/2 ladders, multi-component condensates can occur at high
magnetic fields.Comment: RevTex, 18 pages with 7 figure
Frustrated 3-Dimensional Quantum Spin Liquid in CuHpCl
Inelastic neutron scattering measurements are reported for the quantum
antiferromagnetic material Cu_2(C_5H_12N_2)_2Cl_4 (CuHpCl). The magnetic
excitation spectrum forms a band extending from 0.9 meV to 1.4 meV. The
spectrum contains two modes that disperse throughout the a-c plane of the
monoclinic unit cell with less dispersion along the unique b-axis. Simple
arguments based on the measured dispersion relations and the crystal structure
show that a spin ladder model is inappropriate for describing CuHpCl. Instead,
it is proposed that hydrogen bond mediated exchange interactions between the
bi-nuclear molecular units yield a three-dimensional interacting spin system
with a recurrent triangular motif similar to the Shastry-Sutherland Model
(SSM). Model independent analysis based on the first moment sum rule shows that
at least four distinct spin pairs are strongly correlated and that two of
these, including the dimer bond of the corresponding SSM, are magnetically
frustrated. These results show that CuHpCl should be classified as a
frustration induced three dimensional quantum spin liquid.Comment: 13 pages, 17 figures (Color) ReSubmitted to Phys. Rev. B 9/21/2001
resubmission has new content email comments to [email protected] or
[email protected]
Excitation Spectra of Structurally Dimerized and Spin-Peierls Chains in a Magnetic Field
The dynamical spin structure factor and the Raman response are calculated for
structurally dimerized and spin-Peierls chains in a magnetic field, using exact
diagonalization techniques. In both cases there is a spin liquid phase composed
of interacting singlet dimers at small fields h < h_c1, an incommensurate
regime (h_c1 < h < h_c2) in which the modulation of the triplet excitation
spectra adapts to the applied field, and a fully spin polarized phase above an
upper critical field h_c2. For structurally dimerized chains, the spin gap
closes in the incommensurate phase, whereas spin-Peierls chains remain gapped.
In the spin liquid regimes, the dominant feature of the triplet spectra is a
one-magnon bound state, separated from a continuum of states at higher
energies. There are also indications of a singlet bound state above the
one-magnon triplet.Comment: RevTex, 10 pages with 8 eps figure
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