62 research outputs found

    Magnetoresistance of Pr1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12}: Disentangling local crystalline-electric-field physics and lattice effects

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    Resistivity measurements were performed on Pr1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12} single crystals at temperatures down to 20 mK and in fields up to 18 T. The results for dilute-Pr samples (x=0.3x=0.3 and 0.67) are consistent with model calculations performed assuming a singlet crystalline-electric-field (CEF) ground state. The residual resistivity of these crystals features a smeared step centered around 9 T, the predicted crossing field for the lowest CEF levels. The CEF contribution to the magnetoresistance has a weaker-than-calculated dependence on the field direction, suggesting that interactions omitted from the CEF model lead to avoided crossing in the effective levels of the Pr3+^{3+} ion. The dome-shaped magnetoresistance observed for x=0x = 0 and 0.05 cannot be reproduced by the CEF model, and likely results from fluctuations in the field-induced antiferroquadrupolar phase

    First and second order magnetic and structural transitions in BaFe2(1βˆ’x)_{2(1-x)}Co2x_{2x}As2_{2}

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    We present here high resolution magnetization measurements on high-quality BaFe2(1βˆ’x)_{2(1-x)}Co2x_{2x}As2_{2}, 0≀\leqx≀\leq0.046 as-grown single crystals. The results confirm the existence of a magnetic tricritical point in the (xx,TT) plane at xtrm^{m}_{tr}β‰ˆ\approx0.022 and reveal the emergence of the heat capacity anomaly associated with the onset of the structural transition at xs^{s}β‰ˆ\approx0.0064. We show that the samples with doping near xtrm^{m}_{tr} do not show superconductivity, but rather superconductivity emerges at a slightly higher cobalt doping, xβ‰ˆ\approx0.0315Comment: 4 pages, 5 figure

    Exotic Kondo-hole band resistivity and magnetoresistance of Ce1βˆ’x_{1-x}Lax_{x}Os4_4Sb12_{12} alloys

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    Electrical resistivity measurements of non-magnetic single-crystalline Ce1βˆ’x_{1-x}Lax_xOs4_4Sb12_{12} alloys, x=0.02x=0.02 and 0.1, are reported for temperatures down to 20 mK and magnetic fields up to 18 T. At the lowest temperatures, the resistivity of Ce0.98_{0.98}La0.02_{0.02}Os4_4Sb12_{12} has a Fermi-liquid-like temperature variation ρ=ρ0+AT2\rho=\rho_0+A T^2, but with negative AA in small fields. The resistivity has an unusually strong magnetic field dependence for a paramagnetic metal. The 20 mK resistivity increases by 75% between H=0 and 4 T and then decreases by 65% between 4 T and 18 T. Similarly, the AA coefficient increases with the field from -77 to 29ΞΌΞ© \mu\OmegacmKβˆ’2^{-2} between H=0 and 7 T and then decreases to 18ΞΌΞ© \mu\OmegacmKβˆ’2^{-2} for 18 T. This nontrivial temperature and field variation is attributed to the existence of a very narrow Kondo-hole band in the hybridization gap, which pins the Fermi energy. Due to disorder the Kondo-hole band has localized states close to the band edges. The resistivity for x=0.1x=0.1 has a qualitatively similar behavior to that of x=0.02x=0.02, but with a larger Kondo-hole band

    Universal magnetic and structural behaviors in the iron arsenides

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    Commonalities among the order parameters of the ubiquitous antiferromagnetism present in the parent compounds of the iron arsenide high temperature superconductors are explored. Additionally, comparison is made between the well established two-dimensional Heisenberg-Ising magnet, K2_2NiF4_4 and iron arsenide systems residing at a critical point whose structural and magnetic phase transitions coincide. In particular, analysis is presented regarding two distinct classes of phase transition behavior reflected in the development of antiferromagnetic and structural order in the three main classes of iron arsenide superconductors. Two distinct universality classes are mirrored in their magnetic phase transitions which empirically are determined by the proximity of the coupled structural and magnetic phase transitions in these materials.Comment: 6 pages, 4 figure
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