6 research outputs found
Beyond the Point Ps Approximation
In application to positron annihilation spectroscopy, Ps atom is considered
not as a point particle, but as a finite size e+ e- pair localized in a
bubble-state in a medium. Variation of the internal Coulombic e+ -e- attraction
vs. the bubble radius is estimated
Formation of quasi-free and bubble positronium states in water and aqueous solutions
It is shown that in aqueous solutions a positronium atom is first formed in
the quasi-free state, and, after 50-100 ps, becomes localized in a nanobubble.
Analysis of the annihilation spectra of NaNO3 aqueous solutions shows that the
hydrated electron is not involved in the positronium (Ps) formation
Positronium in a liquid phase: formation, bubble state and chemical reactions
This chapter reviews the following items: 1. Energy deposition and track
structure of fast positrons: ionization slowing down, number of ion-electron
pairs, typical sizes, thermalization, electrostatic interaction between e+ and
its blob, effect of local heating; 2. Positronium formation in condensed media:
the Ore model, quasifree Ps state, intratrack mechanism of Ps formation; 3.
Fast intratrack diffusion-controlled reactions: Ps oxidation and ortho-para
conversion by radiolytic products, reaction rate constants, interpretation of
the PAL spectra in water at different temperatures; 4. Ps bubble models.
"Non-point" positronium: wave function, energy contributions, relationship
between the pick-off annihilation rate and the bubble radius