1,228 research outputs found
{Rearrangement of the antiferromagnetic ordering at high magnetic fields in SmFeAsO and SmFeAsOF single crystals
The low-temperature antiferromagnetic state of the Sm-ions in both
nonsuperconducting SmFeAsO and superconducting SmFeAsOF single
crystals was studied by magnetic torque, magnetization, and magnetoresistance
measurements in magnetic fields up to 60~T and temperatures down to 0.6~K. We
uncover in both compounds a distinct rearrangement of the antiferromagnetically
ordered Sm-moments near ~T. This is seen in both, static and pulsed
magnetic fields, as a sharp change in the sign of the magnetic torque, which is
sensitive to the magnetic anisotropy and hence to the magnetic moment in the
-plane, ({\it i.e.} the FeAs-layers), and as a jump in the magnetization
for magnetic fields perpendicular to the conducting planes. This rearrangement
of magnetic ordering in ~T is essentially temperature independent and
points towards a canted or a partially polarized magnetic state in high
magnetic fields. However, the observed value for the saturation moment above
this rearrangement, suggests that the complete suppression of the
antiferromagnetism related to the Sm-moments would require fields in excess of
60~T. Such a large field value is particularly remarkable when compared to the
relatively small N\'{e}el temperature ~K, suggesting very
anisotropic magnetic exchange couplings. At the transition, magnetoresistivity
measurements show a crossover from positive to negative field-dependence,
indicating that the charge carriers in the FeAs planes are sensitive to the
magnetic configuration of the rare-earth elements. This is indicates a finite
magnetic/electronic coupling between the SmO and the FeAs layers which are
likely to mediate the exchange interactions leading to the long range
antiferromagnetic order of the Sm ions.Comment: 10 pages, 7 figures, accepted in Phys. Rev.
Microscopic Study of the Superconducting State of the Iron Pnictide RbFe_2As_2
A study of the temperature and field dependence of the penetration depth
\lambda of the superconductor RbFe_2As_2 (T_c=2.52 K) was carried out by means
of muon-spin rotation measurements. In addition to the zero temperature value
of the penetration depth \lambda(0)=267(5) nm, a determination of the upper
critical field B_c2(0)=2.6(2) T was obtained. The temperature dependence of the
superconducting carrier concentration is discussed within the framework of a
multi-gap scenario. Compared to the other "122" systems which exhibit much
higher Fermi level, a strong reduction of the large gap BCS ratio 2\Delta/k_B
T_c is observed. This is interpreted as a consequence of the absence of
interband processes. Indications of possible pair-breaking effect are also
discussed.Comment: 5 pages, 4 figure
Bulk electronic structure of superconducting LaRu2P2 single crystals measured by soft x-ray angle-resolved photoemission spectroscopy
We present a soft X-ray angle-resolved photoemission spectroscopy (SX-ARPES)
study of the stoichiometric pnictide superconductor LaRu2P2. The observed
electronic structure is in good agreement with density functional theory (DFT)
calculations. However, it is significantly different from its counterpart in
high-temperature superconducting Fe-pnictides. In particular the bandwidth
renormalization present in the Fe-pnictides (~2 - 3) is negligible in LaRu2P2
even though the mass enhancement is similar in both systems. Our results
suggest that the superconductivity in LaRu2P2 has a different origin with
respect to the iron pnictides. Finally we demonstrate that the increased
probing depth of SX-ARPES, compared to the widely used ultraviolet ARPES, is
essential in determining the bulk electronic structure in the experiment.Comment: 4 pages, 4 figures, 1 supplemental material. Accepted for publication
in Physical Review Letter
Charge and nematic orders in AFe2As2 (A = Rb, Cs) superconductors
We discuss the results of 75As nuclear quadrupole resonance (NQR) and muon spin relaxation measurements in AFe2As2 (A = Cs, Rb) iron-based superconductors. We point out that the crossover detected in the nuclear spin-lattice relaxation rate 1/T1 (around 150 K in RbFe2As2 and around 75 K in CsFe2As2), from a high temperature nearly localized to a low temperature delocalized behavior, is associated with the onset of an inhomogeneous local charge distribution causing the broadening or even the splitting of the NQR spectra as well as an increase in the muon spin relaxation rate. We argue that this crossover, occurring at temperatures well above the phase transition to the nematic long-range order, is due to a charge disproportionation at the Fe sites induced by competing Hund’s and Coulomb couplings. In RbFe2As2 around 35 K, far below that crossover temperature, we observe a peak in the NQR 1/T1 which is possibly associated with the critical slowing down of electronic nematic fluctuations on approaching the transition to the nematic long-range order
Interplay of composition, structure, magnetism, and superconductivity in SmFeAs1-xPxO1-y
Polycrystalline samples and single crystals of SmFeAs1-xPxO1-y were
synthesized and grown employing different synthesis methods and annealing
conditions. Depending on the phosphorus and oxygen content, the samples are
either magnetic or superconducting. In the fully oxygenated compounds the main
impact of phosphorus substitution is to suppress the N\'eel temperature TN of
the spin density wave (SDW) state, and to strongly reduce the local magnetic
field in the SDW state, as deduced from muon spin rotation measurements. On the
other hand the superconducting state is observed in the oxygen deficient
samples only after heat treatment under high pressure. Oxygen deficiency as a
result of synthesis at high pressure brings the Sm-O layer closer to the
superconducting As/P-Fe-As/P block and provides additional electron transfer.
Interestingly, the structural modifications in response to this variation of
the electron count are significantly different when phosphorus is partly
substituting arsenic. Point contact spectra are well described with two
superconducting gaps. Magnetic and resistance measurements on single crystals
indicate an in-plane magnetic penetration depth of 200 nm and an anisotropy of
the upper critical field slope of 4-5. PACS number(s): 74.70.Xa, 74.62.Bf,
74.25.-q, 81.20.-nComment: 36 pages, 13 figures, 2 table
Doniach diagram for ordered, disordered and underscreened Kondo lattices
The Doniach's diagram has been originally proposed to describe the
competition between the local Kondo effect and the intersite RKKY interactions
in cerium compounds. Here we discuss the extension of this diagram to different
variations of Kondo lattice model. We consider a) ordered cerium compounds
where the competition between magnetic order and Kondo effect plays an
important role, as , b) disordered cerium systems with competing
spin glass phase, magnetic ordered phases and a Kondo phase, as the heavy
fermion cerium alloy and, c) uranium compounds where a
coexistence between Kondo effect and ferromagnetic order has been observed, as
UTe. We show that all these cases can be described by a generalized Doniach
phase diagram.Comment: Presented in the Latin American Workshop on Magnetism and Magnetic
Materials (LAW3M) Rio de Janeiro, Brazil, August 12-16, 2007. Proceedings to
be published in JMM
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