Non-Markovian generalization of the Lindblad theory of open quantum systems

A systematic approach to the non-Markovian quantum dynamics of open systems is given by the projection operator techniques of nonequilibrium statistical mechanics. Combining these methods with concepts from quantum information theory and from the theory of positive maps, we derive a class of correlated projection superoperators that take into account in an efficient way statistical correlations between the open system and its environment. The result is used to develop a generalization of the Lindblad theory to the regime of highly non-Markovian quantum processes in structured environments.Comment: 10 pages, 1 figure, replaced by published versio

Witness for initial system-environment correlations in open system dynamics

We study the evolution of a general open quantum system when the system and its environment are initially correlated. We show that the trace distance between two states of the open system can increase above its initial value, and derive tight upper bounds for the growth of the distinguishability of open system states. This represents a generalization of the contraction property of quantum dynamical maps. The obtained inequalities can be interpreted in terms of the exchange of information between the system and the environment, and lead to a witness for system-environment correlations which can be determined through measurements on the open system alone.Comment: 4 pages, 1 figur

New method to simulate quantum interference using deterministic processes and application to event-based simulation of quantum computation

We demonstrate that networks of locally connected processing units with a primitive learning capability exhibit behavior that is usually only attributed to quantum systems. We describe networks that simulate single-photon beam-splitter and Mach-Zehnder interferometer experiments on a causal, event-by-event basis and demonstrate that the simulation results are in excellent agreement with quantum theory. We also show that this approach can be generalized to simulate universal quantum computers.Comment: J. Phys. Soc. Jpn. (in press) http://www.compphys.net/dl

Stochastic wave function method for non-Markovian quantum master equations

A generalization of the stochastic wave function method to quantum master equations which are not in Lindblad form is developed. The proposed stochastic unravelling is based on a description of the reduced system in a doubled Hilbert space and it is shown, that this method is capable of simulating quantum master equations with negative transition rates. Non-Markovian effects in the reduced systems dynamics can be treated within this approach by employing the time-convolutionless projection operator technique. This ansatz yields a systematic perturbative expansion of the reduced systems dynamics in the coupling strength. Several examples such as the damped Jaynes Cummings model and the spontaneous decay of a two-level system into a photonic band gap are discussed. The power as well as the limitations of the method are demonstrated.Comment: RevTex, 14 pages, 9 figures, uses multico

Time-convolutionless master equation for quantum dots: Perturbative expansion to arbitrary order

The master equation describing the non-equilibrium dynamics of a quantum dot coupled to metallic leads is considered. Employing a superoperator approach, we derive an exact time-convolutionless master equation for the probabilities of dot states, i.e., a time-convolutionless Pauli master equation. The generator of this master equation is derived order by order in the hybridization between dot and leads. Although the generator turns out to be closely related to the T-matrix expressions for the transition rates, which are plagued by divergences, in the time-convolutionless generator all divergences cancel order by order. The time-convolutionless and T-matrix master equations are contrasted to the Nakajima-Zwanzig version. The absence of divergences in the Nakajima-Zwanzig master equation due to the nonexistence of secular reducible contributions becomes rather transparent in our approach, which explicitly projects out these contributions. We also show that the time-convolutionless generator contains the generator of the Nakajima-Zwanzig master equation in the Markov approximation plus corrections, which we make explicit. Furthermore, it is shown that the stationary solutions of the time-convolutionless and the Nakajima-Zwanzig master equations are identical. However, this identity neither extends to perturbative expansions truncated at finite order nor to dynamical solutions. We discuss the conditions under which the Nakajima-Zwanzig-Markov master equation nevertheless yields good results.Comment: 13 pages + appendice

Phonon-induced dephasing of singlet-triplet superpositions in double quantum dots without spin-orbit coupling

We show that singlet-triplet superpositions of two-electron spin states in a double quantum dot undergo a phonon-induced pure dephasing which relies only on the tunnel coupling between the dots and on the Pauli exclusion principle. As such, this dephasing process is independent of spin-orbit coupling or hyperfine interactions. The physical mechanism behind the dephasing is elastic phonon scattering, which persists to much lower temperatures than real phonon-induced transitions. Quantitative calculations performed for a lateral GaAs/AlGaAs gate-defined double quantum dot yield micro-second dephasing times at sub-Kelvin temperatures, which is consistent with experimental observations.Comment: Extended versio

Quantum Transport through Nanostructures with Orbital Degeneracies

Geometric symmetries cause orbital degeneracies in a molecule's spectrum. In a single-molecule junction, these degeneracies are lifted by various symmetry-breaking effects. We study quantum transport through such nanostructures with an almost degenerate spectrum. We show that the master equation for the reduced density matrix must be derived within the singular-coupling limit as opposed to the conventional weak-coupling limit. This results in signatures of the density matrix's off-diagonal elements in the transport characteristics

On the Contractivity of Hilbert-Schmidt distance under open system dynamics

We show that the Hilbert-Schmidt distance, unlike the trace distance, between quantum states is generally not monotonic for open quantum systems subject to Lindblad semigroup dynamics. Sufficient conditions for contractivity of the Hilbert-Schmidt norm in terms of the dissipation generators are given. Although these conditions are not necessary, simulations suggest that non-contractivity is the typical case, i.e., that systems for which the Hilbert-Schmidt distance between quantum states is monotonically decreasing form only a small set of all possible dissipative systems for N>2, in contrast to the case N=2 where the Hilbert-Schmidt distance is always monotonically decreasing.Comment: Major revision. We would particularly like to thank D Perez-Garcia for constructive feedbac

Optimal entanglement criterion for mixed quantum states

We develop a strong and computationally simple entanglement criterion. The criterion is based on an elementary positive map Phi which operates on state spaces with even dimension N >= 4. It is shown that Phi detects many entangled states with positive partial transposition (PPT) and that it leads to a class of optimal entanglement witnesses. This implies that there are no other witnesses which can detect more entangled PPT states. The map Phi yields a systematic method for the explicit construction of high-dimensional manifolds of bound entangled states.Comment: 4 pages, no figures, replaced by published version (minor changes), Journal-reference adde