Measurement of energy and angular distributions of secondary ions in the sputtering of gold by swift Au-n clusters: Study of emission mechanisms

Energy and angular distributions of negative ions (Au–, Au2-, Au3-, and Au5-) emitted from gold target bombarded by Au, Au4, and Au9 projectiles at 200 keV/atom were measured with a multipixel position sensitive detector. The angular distributions are symmetrical with respect to the normal to the target surface and forward peaked. They depend on the type of emitted ions, on the emission energy, and on the projectile size. More forward directed emission is observed with Au9 projectiles. The secondary ion energy distributions obtained with Au and Au4 projectiles are well reproduced by a sum of linear collision cascades and thermal spike processes. However, in the case of Au9 projectiles the energy distributions are better described by using a simple spike model with two different average temperature regimes: the first one corresponds to high emission energy occurring in the early stage of the whole process, and the second to the low energy component

Simulation of MeV/atom cluster correlations in matter

We present an efficient algorithm able to predict the trajectories of individual cluster constituents as they penetrate relatively thick amorphous targets. Our algorithm properly treats both the intracluster Coulomb repulsion and the collisions between cluster constituents and target atoms. We have compared our simulation predictions to experimental measurements of the distribution of lateral exit velocities, and demonstrated that the in-target Coulomb explosion of 2MeV/atom carbon clusters in carbon foils must be shielded with a screening length of less than 2.5 Å. We also present a simple phenomenological model for the suppression of the exit-side charge of ions in clusters which depends on the enhanced ionization potential that an electron near an ion feels due to the ion’s charged comoving neighbors. By using our simulation algorithm we have predicted the exit correlations of the cluster constituents and verified that the charge suppression model fits the observed charge suppression of ions in clusters to within the experimental uncertainties

Heavy gold cluster beams production and identification

NIM ACCIt is shown that beams of very heavy gold clusters can be produced by a liquid metal ion source (LMIS). An experimental method is described for defining the LMIS source and the Wien filter parameters that must be set to extract and select large Aun clusters. This method is based on the acceleration of the clusters to high energy (MeV) and on the measurement, after their passage through a thin foil, of their number of constituents and velocity. Only an average mass over charge value is obtained for a given set of source and Wien filter parameters. These parameters can then be used to select heavy Aun cluster beams for applications at low energy (keV) in mass spectrometry

Energy loss and angular distributions of gold cluster constituents

Heavy gold cluster beams are accelerated to high energy (hundreds of keV/atom) and break up when going through a thin foil. The energy and angular distributions of the constituents are then measured and very well reproduced by a SRIM code calculation, which takes into account atomic interactions only. These distributions do not depend on the number of constituents in the cluster and are found to be the same as those of single gold atoms at the same velocity, in the studied energy range

Very large gold and silver sputtering yields induced by keV to MeV energy Aun_n clusters (n = 1-13)

CAS, BIA

Quadrupole deformations of neutron-drip-line nuclei studied within the Skyrme Hartree-Fock-Bogolyubov approach

We introduce a local-scaling point transformation to allow for modifying the asymptotic properties of the deformed three-dimensional Cartesian harmonic oscillator wave functions. The resulting single-particle bases are very well suited for solving the Hartree-Fock-Bogoliubov equations for deformed drip-line nuclei. We then present results of self-consistent calculations performed for the Mg isotopes and for light nuclei located near the two-neutron drip line. The results suggest that for all even-even elements with $Z$=10--18 the most weakly-bound nucleus has an oblate ground-state shape.Comment: 20 pages, 7 figure