882 research outputs found
Comment on "Magnetoelastic model for the relaxation of lanthanide ions in YBa2Cu3O7-d observed by neutron scattering"
Lovesey and Staub have argued [S.W. Lovesey and U. Staub, Phys. Rev. B 61,
9130 (2000)] that experimental data on the temperature dependence of the
paramagnetic relaxation of lanthanide ions doped into YBa2Cu3O6+x are in
agreement with the predictions of a model that describes the relaxation as due
to the scattering of phonons via a magnetoelastic interaction. By generalising
their model I show that the level of agreement is strongly dependent on the
number of intermediate lanthanide energy levels included in the calculation,
and that inclusion of a more complete set of levels leads to very different
results that do not necessarily support the phonon damping picture.Comment: 4 pages, 2 figures, to be published in Phys. Rev.
Approaching the quantum critical point in a highly-correlated all-in-all-out antiferromagnet
Continuous quantum phase transition involving all-in–all-out (AIAO) antiferromagnetic order in strongly spin-orbit-coupled 5d compounds could give rise to various exotic electronic phases and strongly-coupled quantum critical phenomena. Here we experimentally trace the AIAO spin order in Sm₂Ir₂O₇ using direct resonant x-ray magnetic diffraction techniques under high pressure. The magnetic order is suppressed at a critical pressure P_c=6.30GPa, while the lattice symmetry remains in the cubic Fd−3m space group across the quantum critical point. Comparing pressure tuning and the chemical series R₂Ir₂O₇ reveals that the approach to the AIAO quantum phase transition is characterized by contrasting evolutions of the pyrochlore lattice constant a and the trigonal distortion surrounding individual Ir moments, which affects the 5d bandwidth and the Ising anisotropy, respectively. We posit that the opposite effects of pressure and chemical tuning lead to spin fluctuations with different Ising and Heisenberg character in the quantum critical region. Finally, the observed low pressure scale of the AIAO quantum phase transition in Sm₂Ir₂O₇ identifies a circumscribed region of P-T space for investigating the putative magnetic Weyl semimetal state
Spin reorientation transition in the incommensurate stripe-ordered phase of La3/2Sr1/2NiO4
The spin ordering of La3/2Sr1/2NiO4 was investigated by magnetization
measurements, and by unpolarized- and polarized-neutron diffraction. Spin
ordering with an incommensurability epsilon ~ 0.445 is observed below T_so ~ 80
K. On cooling, a spin reorientation is observed at 57 +/- 1 K, with the spin
axes rotating from 52 +/- 4 degrees to 78 +/- 3 degrees. This is the first time
a spin reorientation has been observed in a La2-xSrxNiO4+delta compound having
incommensurate stripe order.Comment: REVTex 4. 4 pages including 4 figures. Minor changes to text.
Accepted to be published in Physical Review
Paramagnon dispersion in -FeSe observed by Fe -edge resonant inelastic x-ray scattering
We report an Fe -edge resonant inelastic x-ray scattering (RIXS) study of
the unusual superconductor -FeSe. The high energy resolution of this
RIXS experiment (55meV FWHM) made it possible to resolve
low-energy excitations of the Fe manifold. These include a broad peak
which shows dispersive trends between 100-200meV along the and
directions of the one-Fe square reciprocal lattice, and which can
be attributed to paramagnon excitations. The multi-band valence state of FeSe
is among the most metallic in which such excitations have been discerned by
soft x-ray RIXS
Magnetic spectrum of the two-dimensional antiferromagnet La2CoO4 studied by inelastic neutron scattering
We report measurements of the magnetic excitation spectrum of the layered
antiferromagnet La2CoO4 by time-of-flight neutron inelastic scattering. In the
energy range probed in our experiments (0-250 meV) the magnetic spectrum
consists of spin-wave modes with strong in-plane dispersion extending up to 60
meV, and a nearly dispersionless peak at 190 meV. The spin-wave modes exhibit a
small (~1 meV) dispersion along the magnetic zone boundary. We show that the
magnetic spectrum can be described very well by a model of a Heisenberg
antiferromagnet that includes the full spin and orbital degrees of freedom of
Co2+ in an axially-distorted crystal field. The collective magnetic dynamics
are found to be controlled by dominant nearest-neighbour exchange interactions,
strong XY-like single-ion anisotropy and a substantial unquenched orbital
angular momentum.Comment: 8 pages, 7 figure
The Temperature Evolution of the Out-of-Plane Correlation Lengths of Charge-Stripe Ordered La(1.725)Sr(0.275)NiO(4)
The temperature dependence of the magnetic order of stripe-ordered
La(1.725)Sr(0.275)NiO(4) is investigated by neutron diffraction. Upon cooling,
the widths if the magnetic Bragg peaks are observed to broaden. The degree of
broadening is found to be very different for l = odd-integer and l =
even-integer magnetic peaks. We argue that the observed behaviour is a result
of competition between magnetic and charge order.Comment: 3 figure
Absence of strong magnetic fluctuations in the iron phosphide superconductors LaFePO and Sr2ScO3FeP
We report neutron inelastic scattering measurements on polycrystalline LaFePO
and Sr2ScO3FeP, two members of the iron phosphide families of superconductors.
No evidence is found for any magnetic fluctuations in the spectrum of either
material in the energy and wavevector ranges probed. Special attention is paid
to the wavevector at which spin-density-wave-like fluctuations are seen in
other iron-based superconductors. We estimate that the magnetic signal, if
present, is at least a factor of four (Sr2ScO3FeP) or seven (LaFePO) smaller
than in the related iron arsenide and chalcogenide superconductors. These
results suggest that magnetic fluctuations are not as influential on the
electronic properties of the iron phosphide systems as they are in other
iron-based superconductors.Comment: 7 pages, 5 figure
Phonon Dispersion Relations in PrBa2Cu3O6+x (x ~ 0.2)
We report measurements of the phonon dispersion relations in
non-superconducting, oxygen-deficient PrBa2Cu3O6+x (x ~ 0.2) by inelastic
neutron scattering. The data are compared with a model of the lattice dynamics
based on a common interaction potential. Good agreement is achieved for all but
two phonon branches, which are significantly softer than predicted. These modes
are found to arise predominantly from motion of the oxygen ions in the CuO2
planes. Analogous modes in YBa2Cu3O6 are well described by the common
interaction potential model.Comment: 4 pages, 3 figures. Minor changes following referees' comment
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