2,415 research outputs found
Can the jamming transition be described using equilibrium statistical mechanics?
When materials such as foams or emulsions are compressed, they display solid
behaviour above the so-called `jamming' transition. Because compression is done
out-of-equilibrium in the absence of thermal fluctuations, jamming appears as a
new kind of a nonequilibrium phase transition. In this proceeding paper, we
suggest that tools from equilibrium statistical mechanics can in fact be used
to describe many specific features of the jamming transition. Our strategy is
to introduce thermal fluctuations and use statistical mechanics to describe the
complex phase behaviour of systems of soft repulsive particles, before sending
temperature to zero at the end of the calculation. We show that currently
available implementations of standard tools such as integral equations,
mode-coupling theory, or replica calculations all break down at low temperature
and large density, but we suggest that new analytical schemes can be developed
to provide a fully microscopic, quantitative description of the jamming
transition.Comment: 8 pages, 6 figs. Talk presented at Statphys24 (July 2010, Cairns,
Australia
Comment on "Constant stress and pressure rheology of colloidal suspensions"
This is a comment on the recent letter by Wang and Brady on "Constant stress
and pressure rheology of colloidal suspensions", Phys. Rev. Lett. 115, 158301
(2015).Comment: 1 page; under review -> v2: publishe
Static and dynamic lengthscales in a simple glassy plaquette model
We study static and dynamic spatial correlations in a two-dimensional spin
model with four-body plaquette interactions and standard Glauber dynamics by
means of analytic arguments and Monte Carlo simulations. We study in detail the
dynamical behaviour which becomes glassy at low temperatures due to the
emergence of effective kinetic constraints in a dual representation where spins
are mapped to plaquette variables. We study the interplay between non-trivial
static correlations of the spins and the dynamic `four-point' correlations
usually studied in the context of supercooled liquids. We show that slow
dynamics is spatially heterogeneous due to the presence of diverging
lengthscales and scaling, as is also found in kinetically constrained models.
This analogy is illustrated by a comparative study of a froth model where the
kinetic constraints are imposed.Comment: 12 pages, 13 figs; published versio
A critical test of the mode-coupling theory of the glass transition
The mode-coupling theory of the glass transition predicts the time evolution
of the intermediate scattering functions in viscous liquids on the sole basis
of the structural information encoded in two-point density correlations. We
provide a critical test of this property and show that the theory fails to
describe the qualitatively distinct dynamical behavior obtained in two model
liquids characterized by very similar pair correlation functions. Because we
use `exact' static information provided by numerical simulations, our results
are a direct proof that some important information about the dynamics of
viscous liquids is not captured by pair correlations, and is thus not described
by the mode-coupling theory, even in the temperature regime where the theory is
usually applied.Comment: 7 pages, 5 figures
The role of attractive forces in viscous liquids
We present evidence from computer simulation that the slowdown of relaxation
of a standard Lennard-Jones glass-forming liquid and that of its reduction to a
model with truncated pair potentials without attractive tails is quantitatively
and qualitatively different in the viscous regime. The pair structure of the
two models is however very similar. This finding, which appears to contradict
the common view that the physics of dense liquids is dominated by the steep
repulsive forces between atoms, is characterized in detail, and its
consequences are explored. Beyond the role of attractive forces themselves, a
key aspect in explaining the differences in the dynamical behavior of the two
models is the truncation of the interaction potentials beyond a cutoff at
typical interatomic distance. This leads us to question the ability of the
jamming scenario to describe the physics of glass-forming liquids and polymers.Comment: 13 pages, 12 figure
Surfing on a critical line: Rejuvenation without chaos, Memory without a hierarchical phase space
The dynamic behaviour of glassy materials displays strong nonequilibrium
effects, such as ageing in simple protocols, memory, rejuvenation and Kovacs
effects in more elaborated experiments. We show that this phenomenology may be
easily understood in the context of the nonequilibrium critical dynamics of
non-disordered systems, the main ingredient being the existence of an infinite
equilibrium correlation length. As an example, we analytically investigate the
behaviour of the 2D XY model submitted to temperature protocols similar to
experiments. This shows that typical glassy effects may be obtained by `surfing
on a critical line' without invoking the concept of temperature chaos nor the
existence of a hierarchical phase space, as opposed to previous theoretical
approaches. The relevance of this phenomenological approach to glassy dynamics
is finally discussed.Comment: Version to be published in Europhysics Letters. Slight modifs + ref
to "surfing" adde
- …