Recovery of 177Lu from Irradiated HfO2 Targets for Nuclear Medicine Purposes

A new method of production of one of the most widely used isotopes in nuclear medicine, 177Lu, with high chemical purity was developed; this method includes irradiation of the HfO2 target with bremsstrahlung photons. The irradiated target was dissolved in HF and then diluted and placed onto a column filled with LN resin. Quantitative sorption of 177Lu could be observed during this process. The column later was rinsed with the mixture of 0.1 M HF and 1 M HNO3 and then 2 M HNO3 to remove impurities. Quantitative desorption of 177Lu was achieved by using 6 M HNO3. The developed method of 177Lu production ensures high purification of this isotope from macroquantities of hafnium and zirconium and radioactive impurities of carrier-free yttrium. The content of 177mLu in 177Lu in photonuclear production was determined. Due to high chemical and radionuclide purity, 177Lu obtained by the developed method can be used in nuclear medicine

A unified understanding of (γ, n) and (n, γ) reactions and direct neutron-multiplicity sorting

We discuss the γ-ray strength function toward a unified understanding of (γ,n) and (n,γ) reactions and propose a novel technique of direct neutron-multiplicity sorting to resolve the long-standing discrepancy between the Livermore and Scalya data of partial photoneutron cross sections.SCOPUS: cp.pinfo:eu-repo/semantics/publishe

New 209Bi photodisintegration data and physical criteria of data reliability

The well-known problem of noticeable disagreements between photoneutron cross sections from various experiments was discussed in detail for 209Bi. Data for partial photoneutron reactions cross sections obtained at Livermore (USA) using quasimonoenergetic annihilation photons and the method of neutron multiplicity sorting were analyzed using the objective physical criteria and the experimental-theoretical method for evaluation. Because of significant systematic uncertainties involved in the method for determining the neutron multiplicity, experimental data do not satisfy the criteria of reliability and differ noticeably from the evaluated data. The new experimental data for 209Bi (γ, in) reactions with i = 1–4 were obtained using quasimonochromatic laser Compton-scattering (LCS) γ-ray beams at the NewSUBARU synchrotron radiation facility and the novel technique of direct neutron-multiplicity sorting with a flat-efficiency detector. It was found that new σ(γ, 1n), σ (γ, 2n), and σ (γ, 3n) contradict noticeably to the Livermore data. It was shown that at the same time the new 209Bi photoneutron cross-sections are in good agreement with data evaluated using experimental-theoretical method and assuring the reliability of those

A unified understanding of (γ, n) and (n, γ) reactions and direct neutron-multiplicity sorting

We discuss the γ-ray strength function toward a unified understanding of (γ,n) and (n,γ) reactions and propose a novel technique of direct neutron-multiplicity sorting to resolve the long-standing discrepancy between the Livermore and Scalya data of partial photoneutron cross sections

Yields of Photo-Proton Reactions on Nuclei of Nickel and Separation of Cobalt Isotopes from Irradiated Targets

Nowadays, cobalt isotopes 55Co, 57Co, and 58mCo are considered to be promising radionuclides in nuclear medicine, with 55Co receiving the most attention as an isotope for diagnostics by positron emission tomography. One of the current research directions is dedicated to its production using electron accelerators (via photonuclear method). In our work, the yields of nuclear reactions occurring during the irradiation of natNi and 60Ni by bremsstrahlung photons with energy up to 55 MeV were determined. A method of fast and simple cobalt isotopes separation from irradiated targets using extraction chromatography was developed

New

The well-known problem of noticeable disagreements between photoneutron cross sections from various experiments was discussed in detail for 209Bi. Data for partial photoneutron reactions cross sections obtained at Livermore (USA) using quasimonoenergetic annihilation photons and the method of neutron multiplicity sorting were analyzed using the objective physical criteria and the experimental-theoretical method for evaluation. Because of significant systematic uncertainties involved in the method for determining the neutron multiplicity, experimental data do not satisfy the criteria of reliability and differ noticeably from the evaluated data. The new experimental data for 209Bi (γ, in) reactions with i = 1–4 were obtained using quasimonochromatic laser Compton-scattering (LCS) γ-ray beams at the NewSUBARU synchrotron radiation facility and the novel technique of direct neutron-multiplicity sorting with a flat-efficiency detector. It was found that new σ(γ, 1n), σ (γ, 2n), and σ (γ, 3n) contradict noticeably to the Livermore data. It was shown that at the same time the new 209Bi photoneutron cross-sections are in good agreement with data evaluated using experimental-theoretical method and assuring the reliability of those

Partial photoneutron cross section measurements on

New data of total and partial (γ,xn) cross sections with x = 1–3 are proposed to be measured by direct neutron multiplicity sorting using Laser Compton scattering (LCS) gamma ray beams at the ELI-NP to solve long standing discrepancies between existing Lawrence Livermore National Laboratory (USA) and France Centre d'Etudes Nucleaires de Saclay photonuclear data. Pioneering experiments are currently performed at the NewSUBARU facility. We present here preliminary results on 209Bi(g,xn) cross section measurements

Partial photoneutron cross section measurements on 209Bi

New data of total and partial (γ,xn) cross sections with x = 1–3 are proposed to be measured by direct neutron multiplicity sorting using Laser Compton scattering (LCS) gamma ray beams at the ELI-NP to solve long standing discrepancies between existing Lawrence Livermore National Laboratory (USA) and France Centre d'Etudes Nucleaires de Saclay photonuclear data. Pioneering experiments are currently performed at the NewSUBARU facility. We present here preliminary results on 209Bi(g,xn) cross section measurements

Photonuclear Alchemy: Obtaining Medical Isotopes of Gold from Mercury Irradiated on Electron Accelerators

In our work, the photonuclear production of 198,199Au isotopes for nuclear medicine purposes was studied, and a method for their recovery from irradiated mercury was developed. The yields of the corresponding nuclear reactions were determined, and a comparison of various methods of obtaining gold radioisotopes was provided. New sorbents based on benzo-15-crown-5, which selectively binds gold, were studied, and the optimal conditions for Au recovery with a high degree of purification from mercury were found. It was established that, for the fast and quantitative recovery of Au isotopes, it was necessary to add at least 0.1 mg of the carrier. As a result, the developed method can be regularly used to obtain 198,199Au for the research of radiopharmaceuticals based on them

GDR cross sections updated in the IAEA-CRP

The Coordinated Research Project (CRP) with the code F41032 has been launched by the International Atomic Energy Agency (IAEA) in 2016 as a 5-year project with the scientific goal being two-fold: 1) updating the 2000 photonuclear data library and 2) constructing a reference database of photon strength functions. We report the experimental technique and methodology used for the former goal and selected giant-dipole resonance (GDR) data updated in the IAEA-CRP