78 research outputs found
Development of Trivalent Ytterbium Doped Fluorapatites for Diode-Pumped Laser Applications
One of the major motivators of this work is the Mercury Project, which is a 1 kW scalable diode-pumped solid-state laser system under development at Lawrence Livermore National Laboratory (LLNL). Major goals include 100 J pulses, 10% wallplug efficiency, 10 Hz repetition rate, and a 5 times diffraction limited beam. To achieve these goals the Mercury laser incorporates ytterbium doped Sr{sub 5}(PO{sub 4}){sub 3}F (S-FAP) as the amplifier gain medium. The primary focus of this thesis is a full understanding of the properties of this material which are necessary for proper design and modeling of the system. Ytterbium doped fluorapatites, which were previously investigated at LLNL, were found to be ideal candidate materials for a high power amplifier systems providing high absorption and emission cross sections, long radiative lifetimes, and high efficiency. A family of barium substituted S-FAP crystals were grown in an effort to modify the pump and emission bandwidths for application to broadband diode pumping and short pulse generation. Crystals of Yb{sup 3+}:Sr{sub 5-x}Ba{sub x}(PO{sub 4}){sub 3}F where x < 1 showed homogeneous lines offering 8.4 nm (1.8 times enhancement) of absorption bandwidth and 6.9 nm (1.4 times enhancement) of emission bandwidth. The gain saturation fluence of Yb:S-FAP was measured to be 3.2 J/cm{sup 2} using a pump-probe experiment where the probe laser was a high intensity Q-switched master oscillator power amplifier system. The extraction data was successfully fit to a homogeneous extraction model. The crystal quality of Czochralski grown Yb:S-FAP crystals, which have been plagued by many defects such as cracking, cloudiness, bubble core, slip dislocations, and anomalous absorption, was investigated interferometrically and quantified by means of Power Spectral Density (PSD) plots. The very best crystals grown to date were found to have adequate crystal quality for use in the Mercury laser system. In addition to phase distortions which are fixed by material growth, thermal loading of the S-FAP media also leads to distortions due to thermal expansion, {alpha}, temperature dependent refractive index, {partial_derivative}n/{partial_derivative}T, and stress optic effects. The stress optic coefficients necessary for modeling thermal distortions in Yb:S-FAP slab amplifiers were measured giving q{sub 33} = 0.308 x 10{sup -12} Pa{sup -1}, and q{sub 31} = 0.936 x 10{sup -12} Pa{sup -1}. Nonlinear optical losses due to high intensity laser interaction with S-FAP were evaluated including Stimulated Raman Scattering (SRS) and Stimulated Brillouin Scattering. The SRS gain coefficient was measured to be 1.3 cm/GW. The SRS losses in the Mercury amplifier system were successfully modeled and shown to be an issue for high-energy short pulse operation. Countermeasures including the addition of bandwidth to the extraction beam and wedging of amplifier surfaces would allow operation of the Mercury laser at 100 J and 2 ns output below SRS threshold. A simple model of SBS losses in the Mercury laser system shows SBS will also be a problem, however suppression is possible with the introduction of moderate bandwidth (relative to the SRS case). Finally, a Q-switched Yb:S-FAP oscillator was developed which operates three-level at 985 nm with a 21% slope efficiency. Frequency conversion of the 985 nm light to the 2nd harmonic at 492.5 nm was achieved with a 31% conversion efficiency. A diode pumped, doubled Yb:S-FAP laser at 492.5 nm would make a compact efficient blue laser source
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Development of Trivalent Ytterbium Doped Fluorapatites for Diode-Pumped Laser Applications
One of the major motivators of this work is the Mercury Project, which is a 1 kW scalable diode-pumped solid-state laser system under development at Lawrence Livermore National Laboratory (LLNL). Major goals include 100 J pulses, 10% wallplug efficiency, 10 Hz repetition rate, and a 5 times diffraction limited beam. To achieve these goals the Mercury laser incorporates ytterbium doped Sr{sub 5}(PO{sub 4}){sub 3}F (S-FAP) as the amplifier gain medium. The primary focus of this thesis is a full understanding of the properties of this material which are necessary for proper design and modeling of the system. Ytterbium doped fluorapatites, which were previously investigated at LLNL, were found to be ideal candidate materials for a high power amplifier systems providing high absorption and emission cross sections, long radiative lifetimes, and high efficiency. A family of barium substituted S-FAP crystals were grown in an effort to modify the pump and emission bandwidths for application to broadband diode pumping and short pulse generation. Crystals of Yb{sup 3+}:Sr{sub 5-x}Ba{sub x}(PO{sub 4}){sub 3}F where x < 1 showed homogeneous lines offering 8.4 nm (1.8 times enhancement) of absorption bandwidth and 6.9 nm (1.4 times enhancement) of emission bandwidth. The gain saturation fluence of Yb:S-FAP was measured to be 3.2 J/cm{sup 2} using a pump-probe experiment where the probe laser was a high intensity Q-switched master oscillator power amplifier system. The extraction data was successfully fit to a homogeneous extraction model. The crystal quality of Czochralski grown Yb:S-FAP crystals, which have been plagued by many defects such as cracking, cloudiness, bubble core, slip dislocations, and anomalous absorption, was investigated interferometrically and quantified by means of Power Spectral Density (PSD) plots. The very best crystals grown to date were found to have adequate crystal quality for use in the Mercury laser system. In addition to phase distortions which are fixed by material growth, thermal loading of the S-FAP media also leads to distortions due to thermal expansion, {alpha}, temperature dependent refractive index, {partial_derivative}n/{partial_derivative}T, and stress optic effects. The stress optic coefficients necessary for modeling thermal distortions in Yb:S-FAP slab amplifiers were measured giving q{sub 33} = 0.308 x 10{sup -12} Pa{sup -1}, and q{sub 31} = 0.936 x 10{sup -12} Pa{sup -1}. Nonlinear optical losses due to high intensity laser interaction with S-FAP were evaluated including Stimulated Raman Scattering (SRS) and Stimulated Brillouin Scattering. The SRS gain coefficient was measured to be 1.3 cm/GW. The SRS losses in the Mercury amplifier system were successfully modeled and shown to be an issue for high-energy short pulse operation. Countermeasures including the addition of bandwidth to the extraction beam and wedging of amplifier surfaces would allow operation of the Mercury laser at 100 J and 2 ns output below SRS threshold. A simple model of SBS losses in the Mercury laser system shows SBS will also be a problem, however suppression is possible with the introduction of moderate bandwidth (relative to the SRS case). Finally, a Q-switched Yb:S-FAP oscillator was developed which operates three-level at 985 nm with a 21% slope efficiency. Frequency conversion of the 985 nm light to the 2nd harmonic at 492.5 nm was achieved with a 31% conversion efficiency. A diode pumped, doubled Yb:S-FAP laser at 492.5 nm would make a compact efficient blue laser source
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Properties of a new average power Nd-doped phosphate laser glass
The Nd-doped phosphate laser glass described herein can withstand 2.3 times greater thermal loading without fracture, compared to APG-1 (commercially-available average-power glass from Schott Glass Technologies). The enhanced thermal loading capability is established on the basis of the intrinsic thermomechanical properties and by direct thermally-induced fracture experiments using Ar-ion laser heating of the samples. This Nd-doped phosphate glass (referred to as APG-t) is found to be characterized by a 29% lower gain cross section and a 25% longer low-concentration emission lifetime
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New tunable lasers for potential use in LIDAR systems
We discuss the optical and laser properties of two new tunable laser crystals, Ce:LiSrAlF{sub 6} and Cr:ZnSe. These crystals are unique in that they provide a practical alternative to optical parametric oscillators as a means of generating tunable radiation in the near ultraviolet and mid-infrared regions (their tuning ranges are at least 285-315 nm and 2.2-2.8 microns, respectively). While these crystals are relatively untested in field deployment, they are promising and likely to be useful in the near future
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Removal of Lattice Imperfections that Impact the Optical Quality of Ti:Sapphire using Advanced Magnetorheological Finishing Techniques
Advanced magnetorheological finishing (MRF) techniques have been applied to Ti:sapphire crystals to compensate for sub-millimeter lattice distortions that occur during the crystal growing process. Precise optical corrections are made by imprinting topographical structure onto the crystal surfaces to cancel out the effects of the lattice distortion in the transmitted wavefront. This novel technique significantly improves the optical quality for crystals of this type and sets the stage for increasing the availability of high-quality large-aperture sapphire and Ti:sapphire optics in critical applications
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Mercury: A High Repetition Rate Laser for High Energy Density Physics
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Removal of Lattice Imperfections that Impact the Optical Quality of Ti:Sapphire using Advanced Magnetorheological Finishing Techniques
Ti:sapphire has become the premier lasing medium material for use in solid-state femtosecond high-peak power laser systems because of its wide wavelength tuning range. With a tuneable range from 680 to 1100 nm, peaking at 800 nm, Ti:sapphire lasing crystals can easily be tuned to the required pump wavelength and provide very high pump brightness due to their good beam quality and high output power of typically several watts. Femtosecond lasers are used for precision cutting and machining of materials ranging from steel to tooth enamel to delicate heart tissue and high explosives. These ultra-short pulses are too brief to transfer heat or shock to the material being cut, which means that cutting, drilling, and machining occur with virtually no damage to surrounding material. Furthermore, these lasers can cut with high precision, making hairline cuts of less than 100 microns in thick materials along a computer-generated path. Extension of laser output to higher energies is limited by the size of the amplification medium. Yields of high quality large diameter crystals have been constrained by lattice distortions that may appear in the boule limiting the usable area from which high quality optics can be harvested. Lattice distortions affect the transmitted wavefront of these optics which ultimately limits the high-end power output and efficiency of the laser system, particularly when operated in multi-pass mode. To make matters even more complicated, Ti:sapphire is extremely hard (Mohs hardness of 9 with diamond being 10) which makes it extremely difficult to accurately polish using conventional methods without subsurface damage or significant wavefront error. In this presentation, we demonstrate for the first time that Magnetorheological finishing (MRF) can be used to compensate for the lattice distortions in Ti:sapphire by perturbing the transmitted wavefront. The advanced MRF techniques developed allow for precise polishing of the optical inverse of lattice distortions with magnitudes of about 70 nm in optical path difference onto one or both of the optical surfaces to produce high quality optics from otherwise unusable Ti:sapphire crystals. The techniques include interferometric, software, and machine modifications to precisely locate and polish sub-millimeter sites onto the optical surfaces that can not be polished into the optics conventionally. This work may allow extension of Ti:sapphire based systems to peak powers well beyond one petawatt
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New Concepts for Reducing Costs and Increasing Efficiency of Solid-State Laser Drivers for IFE
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Full System Operations of Mercury; A Diode-Pumped Solid-State Laser
Operation of the Mercury laser with two amplifiers activated has yielded 30 Joules at 1 Hz and 12 Joules at 10 Hz and over 8 x 10{sup 4} shots on the system. Static distortions in the Yb:S-FAP amplifiers were corrected by magneto rheological finishing technique
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