Dark-field transmission electron microscopy and the Debye-Waller factor of graphene

Graphene's structure bears on both the material's electronic properties and fundamental questions about long range order in two-dimensional crystals. We present an analytic calculation of selected area electron diffraction from multi-layer graphene and compare it with data from samples prepared by chemical vapor deposition and mechanical exfoliation. A single layer scatters only 0.5% of the incident electrons, so this kinematical calculation can be considered reliable for five or fewer layers. Dark-field transmission electron micrographs of multi-layer graphene illustrate how knowledge of the diffraction peak intensities can be applied for rapid mapping of thickness, stacking, and grain boundaries. The diffraction peak intensities also depend on the mean-square displacement of atoms from their ideal lattice locations, which is parameterized by a Debye-Waller factor. We measure the Debye-Waller factor of a suspended monolayer of exfoliated graphene and find a result consistent with an estimate based on the Debye model. For laboratory-scale graphene samples, finite size effects are sufficient to stabilize the graphene lattice against melting, indicating that ripples in the third dimension are not necessary.Comment: 10 pages, 4 figure

Alternative derivation of the Feigel effect and call for its experimental verification

A recent theory by Feigel [Phys. Rev. Lett. {\bf 92}, 020404 (2004)] predicts the finite transfer of momentum from the quantum vacuum to a fluid placed in strong perpendicular electric and magnetic fields. The momentum transfer arises because of the optically anisotropic magnetoelectric response induced in the fluid by the fields. After summarising Feigel's original assumptions and derivation (corrected of trivial mistakes), we rederive the same result by a simpler route, validating Feigel's semi-classical approach. We then derive the stress exerted by the vacuum on the fluid which, if the Feigel hypothesis is correct, should induce a Poiseuille flow in a tube with maximum speed $\approx 100\mu$m/s (2000 times larger than Feigel's original prediction). An experiment is suggested to test this prediction for an organometallic fluid in a tube passing through the bore of a high strength magnet. The predicted flow can be measured directly by tracking microscopy or indirectly by measuring the flow rate ($\approx 1$ml/min) corresponding to the Poiseuille flow. A second experiment is also proposed whereby a `vacuum radiometer' is used to test a recent prediction that the net force on a magnetoelectric slab in the vacuum should be zero.Comment: 20 pages, 1 figures. revised and improved versio

Spin-Peierls Quantum Phase Transitions in Coulomb Crystals

The spin-Peierls instability describes a structural transition of a crystal due to strong magnetic interactions. Here we demonstrate that cold Coulomb crystals of trapped ions provide an experimental testbed in which to study this complex many-body problem and to access extreme regimes where the instability is triggered by quantum fluctuations alone. We present a consistent analysis based on different analytical and numerical methods, and provide a detailed discussion of its feasibility on the basis of ion-trap experiments. Moreover, we identify regimes where this quantum simulation may exceed the power of classical computers.Comment: slightly longer than the published versio

NMR evidence for Friedel-like oscillations in the CuO chains of ortho-II YBa2_2Cu3_3O6.5_{6.5}

Nuclear magnetic resonance (NMR) measurements of CuO chains of detwinned Ortho-II YBa$_2$Cu$_3$O$_{6.5}$ (YBCO6.5) single crystals reveal unusual and remarkable properties. The chain Cu resonance broadens significantly, but gradually, on cooling from room temperature. The lineshape and its temperature dependence are substantially different from that of a conventional spin/charge density wave (S/CDW) phase transition. Instead, the line broadening is attributed to small amplitude static spin and charge density oscillations with spatially varying amplitudes connected with the ends of the finite length chains. The influence of this CuO chain phenomenon is also clearly manifested in the plane Cu NMR.Comment: 4 pages, 3 figures, refereed articl

Quasi-long-range ordering in a finite-size 2D Heisenberg model

We analyse the low-temperature behaviour of the Heisenberg model on a two-dimensional lattice of finite size. Presence of a residual magnetisation in a finite-size system enables us to use the spin wave approximation, which is known to give reliable results for the XY model at low temperatures T. For the system considered, we find that the spin-spin correlation function decays as 1/r^eta(T) for large separations r bringing about presence of a quasi-long-range ordering. We give analytic estimates for the exponent eta(T) in different regimes and support our findings by Monte Carlo simulations of the model on lattices of different sizes at different temperatures.Comment: 9 pages, 3 postscript figs, style files include

The effects of nonlocality on the evolution of higher order fluxes in non-equilibrium thermodynamics

The role of gradient dependent constitutive spaces is investigated on the example of Extended Thermodynamics of rigid heat conductors. Different levels of nonlocality are developed and the different versions of extended thermodynamics are classified. The local form of the entropy density plays a crucial role in the investigations. The entropy inequality is solved under suitable constitutive assumptions. Balance form of evolution equations is obtained in special cases. Closure relations are derived on a phenomenological level.Comment: 16 pages, 1 figur

Counter-term charges generate bulk symmetries

We further explore the counter-term subtraction definition of charges (e.g., energy) for classical gravitating theories in spacetimes of relevance to gauge/gravity dualities; i.e., in asymptotically anti-de Sitter spaces and their kin. In particular, we show in general that charges defined via the counter-term subtraction method generate the desired asymptotic symmetries. As a result, they can differ from any other such charges, such as those defined by bulk spacetime-covariant techniques, only by a function of auxiliary non-dynamical structures such as a choice of conformal frame at infinity (i.e., a function of the boundary fields alone). Our argument is based on the Peierls bracket, and in the AdS context allows us to demonstrate the above result even for asymptotic symmetries which generate only conformal symmetries of the boundary (in the chosen conformal frame). We also generalize the counter-term subtraction construction of charges to the case in which additional non-vanishing boundary fields are present.Comment: 13 pages, Latex, no figures, v3: errors fixed, boundary terms carefully controlled, awkward assumption removed, references update

Classical evolution of fractal measures on the lattice

We consider the classical evolution of a lattice of non-linear coupled oscillators for a special case of initial conditions resembling the equilibrium state of a macroscopic thermal system at the critical point. The displacements of the oscillators define initially a fractal measure on the lattice associated with the scaling properties of the order parameter fluctuations in the corresponding critical system. Assuming a sudden symmetry breaking (quench), leading to a change in the equilibrium position of each oscillator, we investigate in some detail the deformation of the initial fractal geometry as time evolves. In particular we show that traces of the critical fractal measure can sustain for large times and we extract the properties of the chain which determine the associated time-scales. Our analysis applies generally to critical systems for which, after a slow developing phase where equilibrium conditions are justified, a rapid evolution, induced by a sudden symmetry breaking, emerges in time scales much shorter than the corresponding relaxation or observation time. In particular, it can be used in the fireball evolution in a heavy-ion collision experiment, where the QCD critical point emerges, or in the study of evolving fractals of astrophysical and cosmological scales, and may lead to determination of the initial critical properties of the Universe through observations in the symmetry broken phase.Comment: 15 pages, 15 figures, version publiced at Physical Review

Melting of Polydisperse Hard Disks

The melting of a polydisperse hard disk system is investigated by Monte Carlo simulations in the semigrand canonical ensemble. This is done in the context of possible continuous melting by a dislocation unbinding mechanism, as an extension of the 2D hard disk melting problem. We find that while there is pronounced fractionation in polydispersity, the apparent density-polydispersity gap does not increase in width, contrary to 3D polydisperse hard spheres. The point where the Young's modulus is low enough for the dislocation unbinding to occur moves with the apparent melting point, but stays within the density gap, just like for the monodisperse hard disk system. Additionally, we find that throughout the accessible polydispersity range, the bound dislocation-pair concentration is high enough to affect the dislocation unbinding melting as predicted by Kosterlitz, Thouless, Halperin, Nelson and Young.Comment: 6 pages, 6 figure

Representation of spectral functions and thermodynamics

In this paper we study the question of effective field assignment to measured or nonperturbatively calculated spectral functions. The straightforward procedure is to approximate it by a sum of independent Breit-Wigner resonances, and assign an independent field to each of these resonances. The problem with this idea is that it introduces new conserved quantities in the free model (the new particle numbers), therefore it changes the symmetry of the system. We avoid this inconsistency by representing each quantum channel with a single effective field, no matter how complicated the spectral function is. Thermodynamical characterization of the system will be computed with this representation method, and its relation to the independent resonance approximation will be discussed.Comment: 15 pages, 9 figures, revtex