1,038 research outputs found
Complete Exact Solution of Diffusion-Limited Coalescence, A + A -> A
Some models of diffusion-limited reaction processes in one dimension lend
themselves to exact analysis. The known approaches yield exact expressions for
a limited number of quantities of interest, such as the particle concentration,
or the distribution of distances between nearest particles. However, a full
characterization of a particle system is only provided by the infinite
hierarchy of multiple-point density correlation functions. We derive an exact
description of the full hierarchy of correlation functions for the
diffusion-limited irreversible coalescence process A + A -> A.Comment: 4 pages, 2 figures (postscript). Typeset with Revte
Stochastic Model and Equivalent Ferromagnetic Spin Chain with Alternation
We investigate a non-equilibrium reaction-diffusion model and equivalent
ferromagnetic spin 1/2 XY spin chain with alternating coupling constant. The
exact energy spectrum and the n-point hole correlations are considered with the
help of the Jordan-Wigner fermionization and the inter-particle distribution
function method. Although the Hamiltonian has no explicit translational
symmetry, the translational invariance is recovered after long time due to the
diffusion. We see the scaling relations for the concentration and the two-point
function in finite size analysis.Comment: 7 pages, LaTeX file, to appear in J. Phys. A: Math. and Ge
Two-Species Annihilation with Drift: A Model with Continuous Concentration-Decay Exponents
We propose a model for diffusion-limited annihilation of two species, or , where the motion of the particles is subject to a drift. For equal
initial concentrations of the two species, the density follows a power-law
decay for large times. However, the decay exponent varies continuously as a
function of the probability of which particle, the hopping one or the target,
survives in the reaction. These results suggest that diffusion-limited
reactions subject to drift do not fall into a limited number of universality
classes.Comment: 10 pages, tex, 3 figures, also available upon reques
Time evolution of the reaction front in a subdiffusive system
Using the quasistatic approximation, we show that in a subdiffusion--reaction
system the reaction front evolves in time according to the formula
, with being the subdiffusion parameter. The
result is derived for the system where the subdiffusion coefficients of
reactants differ from each other. It includes the case of one static reactant.
As an application of our results, we compare the time evolution of reaction
front extracted from experimental data with the theoretical formula and we find
that the transport process of organic acid particles in the tooth enamel is
subdiffusive.Comment: 18 pages, 3 figure
A Method of Intervals for the Study of Diffusion-Limited Annihilation, A + A --> 0
We introduce a method of intervals for the analysis of diffusion-limited
annihilation, A+A -> 0, on the line. The method leads to manageable diffusion
equations whose interpretation is intuitively clear. As an example, we treat
the following cases: (a) annihilation in the infinite line and in infinite
(discrete) chains; (b) annihilation with input of single particles, adjacent
particle pairs, and particle pairs separated by a given distance; (c)
annihilation, A+A -> 0, along with the birth reaction A -> 3A, on finite rings,
with and without diffusion.Comment: RevTeX, 13 pages, 4 figures, 1 table. References Added, and some
other minor changes, to conform with final for
Exactly solvable models through the empty interval method, for more-than-two-site interactions
Single-species reaction-diffusion systems on a one-dimensional lattice are
considered, in them more than two neighboring sites interact. Constraints on
the interaction rates are obtained, that guarantee the closedness of the time
evolution equation for 's, the probability that consecutive sites
are empty at time . The general method of solving the time evolution
equation is discussed. As an example, a system with next-nearest-neighbor
interaction is studied.Comment: 19 pages, LaTeX2
Diffusion-Limited Aggregation Processes with 3-Particle Elementary Reactions
A diffusion-limited aggregation process, in which clusters coalesce by means
of 3-particle reaction, A+A+A->A, is investigated. In one dimension we give a
heuristic argument that predicts logarithmic corrections to the mean-field
asymptotic behavior for the concentration of clusters of mass at time ,
, for . The total
concentration of clusters, , decays as at . We also investigate the problem with a localized steady source of
monomers and find that the steady-state concentration scales as
, , and , respectively,
for the spatial dimension equal to 1, 2, and 3. The total number of
clusters, , grows with time as , , and
for = 1, 2, and 3. Furthermore, in three dimensions we
obtain an asymptotic solution for the steady state cluster-mass distribution:
, with the scaling function
and the scaling variable .Comment: 12 pages, plain Te
Non-equilibrium Magnetization Dynamics in the Fe_8 Single-Molecule Magnet Induced by High-Intensity Microwave Radiation
Resonant microwave radiation applied to a single crystal of the molecular
magnet Fe_8 induces dramatic changes in the sample's magnetization. Transitions
between excited states are found even though at the nominal system temperature
these levels have negligible population. We find evidence that the sample heats
significantly when the resonance condition is met. In addition, heating is
observed after a short pulse of intense radiation has been turned off,
indicating that the spin system is out of equilibrium with the lattice.Comment: Version to appear in Europhysics Letters. Minor changes and updated
reference
Determining mean first-passage time on a class of treelike regular fractals
Relatively general techniques for computing mean first-passage time (MFPT) of
random walks on networks with a specific property are very useful, since a
universal method for calculating MFPT on general graphs is not available
because of their complexity and diversity. In this paper, we present techniques
for explicitly determining the partial mean first-passage time (PMFPT), i.e.,
the average of MFPTs to a given target averaged over all possible starting
positions, and the entire mean first-passage time (EMFPT), which is the average
of MFPTs over all pairs of nodes on regular treelike fractals. We describe the
processes with a family of regular fractals with treelike structure. The
proposed fractals include the fractal and the Peano basin fractal as their
special cases. We provide a formula for MFPT between two directly connected
nodes in general trees on the basis of which we derive an exact expression for
PMFPT to the central node in the fractals. Moreover, we give a technique for
calculating EMFPT, which is based on the relationship between characteristic
polynomials of the fractals at different generations and avoids the computation
of eigenvalues of the characteristic polynomials. Making use of the proposed
methods, we obtain analytically the closed-form solutions to PMFPT and EMFPT on
the fractals and show how they scale with the number of nodes. In addition, to
exhibit the generality of our methods, we also apply them to the Vicsek
fractals and the iterative scale-free fractal tree and recover the results
previously obtained.Comment: Definitive version published in Physical Review
Experimental Upper Bound on Superradiance Emission from Mn12 Acetate
We used a Josephson junction as a radiation detector to look for evidence of
the emission of electromagnetic radiation during magnetization avalanches in a
crystal assembly of Mn_12-Acetate. The crystal assembly exhibits avalanches at
several magnetic fields in the temperature range from 1.8 to 2.6 K with
durations of the order of 1 ms. Although a recent study shows evidence of
electromagnetic radiation bursts during these avalanches [J. Tejada, et al.,
Appl. Phys. Lett. {\bf 84}, 2373 (2004)], we were unable to detect any
significant radiation at well-defined frequencies. A control experiment with
external radiation pulses allows us to determine that the energy released as
radiation during an avalanche is less than 1 part in 10^4 of the total energy
released. In addition, our avalanche data indicates that the magnetization
reversal process does not occur uniformly throughout the sample.Comment: 4 RevTeX pages, 3 eps figure
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