Uniaxial anisotropy and enhanced magnetostriction of CoFe2_2O4_4 induced by reaction under uniaxial pressure with SPS

In this study, we have compared magnetic and magnetostrictive properties of polycrystalline CoFe$_2$O$_4$ pellets, produced by three different methods, focusing on the use of Spark Plasma Sintering (SPS). This technique allows a very short heat treatment stage while a uniaxial pressure is applied. SPS was utilized to sinter cobalt ferrite but also to make the reaction and the sintering (reactive sintering) of the same ceramic composition. Magnetic and magnetostrictive measurements show that the reactive sintering with SPS induces a uniaxial anisotropy, while it is not the case with a simple sintering process. The induced anisotropy is then expected to be a consequence of the reaction under uniaxial pressure. This anisotropy enhanced the magnetostrictive properties of the sample, where a maximum longitudinal magnetostriction of $-229$~ppm is obtained. This process can be a promising alternative to the magnetic-annealing because of the short processing time required (22 minutes)

Enhancement of the magnetoelectric effect in multiferroic CoFe2_2O4_4/PZT bilayer by induced uniaxial magnetic anisotropy

In this study we have compared magnetic, magnetostrictive and piezomagnetic properties of isotropic and anisotropic cobalt ferrite pellets. The isotropic sample was prepared by the ceramic method while the sample exhibiting uniaxial anisotropy was made by reactive sintering using Spark Plasma Sintering (SPS). This technique permits to induce a magnetic anisotropy in cobalt ferrite in the direction of the applied pressure during SPS process. Sample with uniaxial anisotropy revealed a higher longitudinal magnetostriction and piezomagnetism compared to the isotropic sample, but the transversal magnetostriction and piezomagnetism were dramatically reduced. In the case of magnetoelectric layered composite, the magnetoelectric coefficient is directly related to the sum of the longitudinal and transversal piezomagnetic coefficients. These two coefficients being opposite in sign, the use of material exhibiting high longitudinal and low transversal piezomagnetic coefficient (or vice versa) in ME devices is expected to improve the ME effect. Hence, ME bilayer devices were made using isotropic and anisotropic cobalt ferrite stuck with a PZT layer. ME measurements at low frequencies revealed that bilayer with anisotropic cobalt ferrite exhibits a ME coefficient three times higher than a bilayer with isotropic cobalt ferrite. We also investigated the behavior of such composites when excited at resonant frequency

A Method to Measure ϕ1\phi_1 Using Bˉ0→Dh0\bar{B}^0 \to D h^0 With Multibody DD Decay

We describe a new method to measure the angle $\phi_1$ of the CKM Unitarity Triangle using amplitude analysis of the multibody decay of the neutral $D$ meson produced via $\bar{B} \to D h^0$ colour-suppressed decays. The method employs the interference between $D^0$ and $\bar{D}^0$ to directly extract the value of $2\phi_1$, and thus resolve the ambiguity between $2\phi_1$ and $\pi-2\phi_1$ in the measurement of $\sin(2\phi_1)$ using \bar{B}^0 \to J/ \psi \ks. We present a feasibility study of this method using Monte Carlo simulation.Comment: 12 pages, 7 figures, 2 tables. See also talk presented by T.G. at CKM2005 (http://ckm2005.ucsd.edu/) Submitted to Physics Letters

Magnetic properties of Nd6Fe13Cu single crystals

The understanding of coercivity mechanism in high performance Nd-Fe-B permanent magnets relies on the analysis of the magnetic properties of all phases present in the magnets. By adding Cu in such compounds, a new Nd6Fe13Cu grain boundary phase is formed, however, the magnetic properties of this phase and its role in the magnetic decoupling of the matrix Nd2Fe14B grains are still insufficiently studied. In this work, we have grown Nd6Fe13Cu single crystals by the reactive flux method and studied their magnetic properties in detail. It is observed that below the N\'eel temperature (TN = 410 K), the Nd6Fe13Cu is antiferromagnetic in zero magnetic field; whereas when a magnetic field is applied along the a-axis, a spin-flop transition occurs at approx. 6 T, indicating a strong competition between antiferromagnetic and ferromagnetic interactions in two Nd layers below and above the Cu layers. Our atomistic spin dynamics simulation confirms that an increase in temperature and/or magnetic field can significantly change the antiferromagnetic coupling between the two Nd layers below and above the Cu layers, which, in turn, is the reason for the observed spin-flop transition. These results suggest that the role of antiferromagnetic Nd6Fe13Cu grain boundary phase in the coercivity enhancement of Nd-Fe-B-Cu magnets is more complex than previously thought, mainly due to the competition between its antiferro- and ferro-magnetic exchange interactions.Comment: 15 pages, 4 figure

Designing magnetocaloric materials for hydrogen liquefaction with light rare-earth Laves phases

Magnetocaloric hydrogen liquefaction could be a "game-changer" for liquid hydrogen industry. Although heavy rare-earth-based magnetocaloric materials show strong magnetocaloric effects in the temperature range required by hydrogen liquefaction (77 ~ 20 K), the high resource criticality of the heavy rare-earth elements is a major obstacle for upscaling this emerging liquefaction technology. In contrast, the higher abundances of the light rare-earth elements make their alloys highly appealing for magnetocaloric hydrogen liquefaction. Via a mean-field approach, it is demonstrated that tuning the Curie temperature ($T_C$) of an idealized light rare-earth-based magnetocaloric material towards lower cryogenic temperatures leads to larger maximum magnetic and adiabatic temperature changes ($\Delta S_T$ and $\Delta T_{ad}$). Especially in the vicinity of the condensation point of hydrogen (20 K), $\Delta S_T$ and $\Delta T_{ad}$ of the optimized light rare-earth-based material are predicted to show significantly large values. Following the mean-field approach and taking the chemical and physical similarities of the light rare-earth elements into consideration, a method of designing light rare-earth intermetallic compounds for hydrogen liquefaction is proposed: tunning $T_C$ of a rare-earth alloy to approach 20 K by mixing light rare-earth elements with different de Gennes factors. By mixing Nd and Pr in Laves phase $(Nd,Pr)Al_2$, and Pr and Ce in Laves phase $(Pr,Ce)Al_2$, a fully light rare-earth intermetallic series with large magnetocaloric effects covering the temperature range required by hydrogen liquefaction is developed, demonstrating a competitive maximum effect compared to the heavy rare-earth compound $DyAl_2$

Nitrogenation and sintering of (Nd-Zr)Fe10Si2 tetragonal compounds for permanent magnets applications

International audienceNd(1-x)Zr(x)Fe10Si2 alloys have been prepared in the tetragonal ThMn12-type structure by arc-melting and melt-spinning and then nitrogenated to improve their magnetic properties. For x = 0.4 and 0.6 the Curie temperature and magnetic anisotropy fields increase from 280-300 ºC to about 390 ºC and from 2.8-3 T to 4.5-5 T respectively. The saturation magnetization remains almost unchanged. The nitrogenated powders were processed by spark plasma sintering (SPS) leading to compact pellets, which retain the full nitrogen content and magnetic properties up to 600 ºC, but segregated Fe-Si at elevated temperatures. Nitrogenation and SPS processing are, therefore, appropriate for sintering metastable materials such as (Nd,Zr)Fe10Si2 into compact material without loosing functional properties. This opens a way towards a new family of permanent magnets, lean of critical raw materials

The Completed SDSS-IV Extended Baryon Oscillation Spectroscopic Survey: Growth rate of structure measurement from cosmic voids

We present a void clustering analysis in configuration-space using the completed Sloan Digital Sky Survey IV (SDSS-IV) extended Baryon Oscillation Spectroscopic Survey (eBOSS) DR16 samples. These samples consist of Luminous Red Galaxies (LRG) combined with the high redshift tail of the SDSS-III Baryon Oscillation Spectroscopic Survey (BOSS) DR12 CMASS galaxies (called as LRG+CMASS sample), Emission Line Galaxies (ELG) and quasars (QSO). We build void catalogues from the three eBOSS DR16 samples using a ZOBOV-based algorithm, providing 2,814 voids, 1,801 voids and 4,347 voids in the LRG+CMASS, ELG and QSO samples, respectively, spanning the redshift range $0.6<z<2.2$. We measure the redshift space distortions (RSD) around voids using the anisotropic void-galaxy cross-correlation function and we extract the distortion parameter $\beta$. We test the methodology on realistic simulations before applying it to the data, and we investigate all our systematic errors on these mocks. We find $\beta^{\rm LRG}(z=0.74)=0.415\pm0.087$, $\beta^{\rm ELG}(z=0.85)=0.665\pm0.125$ and $\beta^{\rm QSO}(z=1.48)=0.313\pm0.134$, for the LRG+CMASS, ELG and QSO sample, respectively. The quoted errors include systematic and statistical contributions. In order to convert our measurements in terms of the growth rate $f\sigma_8$, we use consensus values of linear bias from the eBOSS DR16 companion papers~\citep{eBOSScosmo}, resulting in the following constraints: $f\sigma_8(z=0.74)=0.50\pm0.11$, $f\sigma_8(z=0.85)=0.52\pm0.10$ and $f\sigma_8(z=1.48)=0.30\pm0.13$. Our measurements are consistent with other measurements from eBOSS DR16 using conventional clustering techniques.Comment: 17 pages, 8 figure

Probing Charge-Symmetry-Violating Quark Distributions in Semi-Inclusive Leptoproduction of Hadrons

Recent experiments by the HERMES group at HERA are measuring semi-inclusive electroproduction of pions from deuterium. We point out that by comparing the production of $\pi^+$ and $\pi^-$ from an isoscalar target, it is possible, in principle, to measure charge symmetry violation in the valence quark distributions of the nucleons. It is also possible in the same experiments to obtain an independent measurement of the quark fragmentation functions. We review the information which can be deduced from such experiments and show the ``signature'' for charge symmetry violation in such experiments. Finally, we predict the magnitude of the charge symmetry violation, from both the valence quark distributions and the pion fragmentation function, which might be expected in these experiments.Comment: 19 pages plus 5 figures, used eps