Making tracks in metals

Swift heavy ions lose energy primarily by inelastic electronic scattering and, above an energy threshold, electronic losses result in damage to the lattice. Such high energy radiation is beyond the range of validity of traditional cascade simulations, and predictive damage calculations are challenging. We use a novel methodology, which combines molecular dynamics with a consistent treatment of electronic energy transport and redistribution to the lattice, to model how swift heavy ions form damage tracks. We consider a range of material parameters (electron-phonon coupling strength, thermal conductivity and electronic specific heat) and show how these affect the maximum lattice temperature reached and the extent of residual damage. Our analysis also suggests that fission tracks may form in alloys of archaeological interest

Excitonic model of track registration of energetic heavy ions in insulators

The consequence of generation of dense electronic excitation along the paths of energetic heavy ions is discussed, emphasizing the fates of electron-hole pairs. It is pointed out that a substantial part of the energy imparted to electron-hole pairs in the materials in which excitons are self-trapped is converted directly to defect formation energy but do not contribute to heating. However, the thermal spike model can be an appropriate macroscopic model of the track registration of the materials in which excitons are self-trapped, because energy deposited to the material remains along the ion paths. The energy imparted to electron-hole pairs is diffused away from the ion paths in the materials in which excitons are not self-trapped. This explains the reason why the critical stopping power for track registration is higher in these materials. The difficulty for application of the thermal spike model to these materials is pointed out and it is suggested that nominal defects in densely excited region nucleate fragmental tracks. (C) 1998 Published by Elsevier Science B.V. All rights reserved

QUADRUPOLE SPLITTING OF MOSSBAUER LINES DUE TO DEFECTS IN CO0

The Fe3+ lines observed in CoO Mossbauer sources may arise from the decay of Co3+ ions associated with cation vacancies in the crystal. These defects produce an electric-field gradient that causes a quadrupole splitting of the resonance line and that can, in principle, distinguish between different types of defects. The calculation of the quadrupole splitting at Fe2+ and Fe3+ sites near various vacancy clusters includes the relaxation of the lattice about the defect. This lattice polarisation and distortion is shown to be extremely important, since simple calculations based on perfect ion positions give very different field gradients at neighbouring sites. The results compared with the experiments available and the quadrupole splittings observed are close to those predicted by a vacancy model

INITIAL PRODUCTION OF DEFECTS IN ALKALI-HALIDES - F AND H CENTER PRODUCTION BY NON-RADIATIVE DECAY OF SELF-TRAPPED EXCITON

Radiation damage in KCl can be produced by the decay of a self-trapped exciton into an F centre and an H centre. The authors present calculations of the energies of the states involved for various stages in the evolution of the damage. These lead to important conclusions about the very rapid damage process, and support strongly Itoh and Saidoh's suggestion (1973) that damage proceeds through an excited hole state. The results also help in understanding the prompt decay of F and H pairs at low temperatures, the thermal annihilation of F and H centres, the effects of optical excitation of the self-trapped exciton, and some of the trends within the alkali halides. The calculations use a self-consistent semi-empirical molecular-orbital method. A large cluster of ions is used (either 42 or 57 ions) plus long-range Madelung terms. The ion positions were obtained from separate lattice-relaxation calculations with the HADES code. The choice of CNDO parameters and the adequacy of the method were checked by a number of separate predictions

The dielectric constant of UO2 below the Néel point

We report measurements of the frequency-dependent dielectric constant of UO2 from 4.2 K to above the phase transition at 30 K. The static dielectric constant of 23.6 at 4.2 K is comparable with accepted values at higher temperatures: it is essentially identical in both phases. The effects of undergoing the transition on the dielectric constant are marginal (about 1%) and take place in the temperature range 29 K to 37 K. The displacement of the oxygen sublattice, which occurs at the Ne´el point, should produce only a 0.05% change on the dielectric constant and of the opposite sense to that measured. Hence the structural changes at the transition are not the primary source of the observed small difference between the dielectric constant in the two phases which probably accrues from the influence of the displacements on a defect-related contribution

Making tracks: electronic excitation roles in forming swift heavy ion tracks

Swift heavy ions cause material modification along their tracks, changes primarily due to their very dense electronic excitation. The available data for threshold stopping powers indicate two main classes of materials. Group I, with threshold stopping powers above about 10 keV nm(-1), includes some metals, crystalline semiconductors and a few insulators. Group II, with lower thresholds, comprises many insulators, amorphous materials and high T-c oxide superconductors. We show that the systematic differences in behaviour result from different coupling of the dense excited electrons, holes and excitons to atomic (ionic) motions, and the consequent lattice relaxation. The coupling strength of excitons and charge carriers with the lattice is crucial. For group II, the mechanism appears to be the self- trapped exciton model of Itoh and Stoneham ( 1998 Nucl. Instrum. Methods Phys. Res. B 146 362): the local structural changes occur roughly when the exciton concentration exceeds the number of lattice sites. In materials of group I, excitons are not self- trapped and structural change requires excitation of a substantial fraction of bonding electrons, which induces spontaneous lattice expansion within a few hundred femtoseconds, as recently observed by laser- induced time- resolved x- ray diffraction of semiconductors. Our analysis addresses a number of experimental results, such as track morphology, the efficiency of track registration and the ratios of the threshold stopping power of various materials

Data-efficient learning of feedback policies from image pixels using deep dynamical models

Data-efficient reinforcement learning (RL) in continuous state-action spaces using very high-dimensional observations remains a key challenge in developing fully autonomous systems. We consider a particularly important instance of this challenge, the pixels-to-torques problem, where an RL agent learns a closed-loop control policy ( torques ) from pixel information only. We introduce a data-efficient, model-based reinforcement learning algorithm that learns such a closed-loop policy directly from pixel information. The key ingredient is a deep dynamical model for learning a low-dimensional feature embedding of images jointly with a predictive model in this low-dimensional feature space. Joint learning is crucial for long-term predictions, which lie at the core of the adaptive nonlinear model predictive control strategy that we use for closed-loop control. Compared to state-of-the-art RL methods for continuous states and actions, our approach learns quickly, scales to high-dimensional state spaces, is lightweight and an important step toward fully autonomous end-to-end learning from pixels to torques

Status of reaction theory for studying rare isotopes

Reactions are an important tool to study nuclear structure and for extracting reactions relevant for astrophysics. In this paper we focus on deuteron induced reactions which can provide information on neutron shell evolution as well as neutron capture cross sections. We review recent work on the systematic comparison of the continuum discretized coupled channel method, the adiabatic wave approximation and the Faddeev momentum-space approach. We also explore other aspects of the reaction mechanism and discuss in detail difficulties encountered in the calculations.Comment: 7 pages, 5 figures, proceeding for HITES 201

Frequency dependence of electrical conductivity and dielectric constant of UO2

The dielectric constant and electrical conductivity of single crystal and polycrystalline UO2 are found to be frequency dependent. The dielectric constant measured at low frequencies is anomalously large at room temperature but decreases to a limiting value (~25) below about 130 K. A knee observed in the temperature dependence of the conductivity of polycrystalline UO2 corresponds to a process having an activation energy of 0.15 eV

NaNog: A pluripotency homeobox (master) molecule.

One of the most intriguing aspects of cell biology is the state of pluripotency, where the cell is capable of self-renewal for as many times as deemed necessary , then at a specified time can differentiate into any type of cell. This fundamental process is required during organogenesis in foetal life and importantly during tissue repair in health and disease. Pluripotency is very tightly regulated, as any dysregulation can result in congenital defects, inability to repair damage, or cancer. Fuelled by the relatively recent interest in stem cell biology and tissue regeneration, the molecules implicated in regulating pluripotency have been the subject of extensive research. One of the important molecules involved in pluripotency, is NaNog, the subject of this article