15 research outputs found
Ultrafast Acousto-Plasmonics in Gold Nanoparticles Superlattice
We report the investigation of the generation and detection of GHz coherent
acoustic phonons in plasmonic gold nanoparticles superlattices (NPS). The
experiments have been performed from an optical femtosecond pump-probe scheme
across the optical plasmon resonance of the superlattice. Our experiments allow
to estimate the collective elastic response (sound velocity) of the NPS as well
as an estimate of the nano-contact elastic stiffness. It appears that the
light-induced coherent acoustic phonon pulse has a typical in-depth spatial
extension of about 45 nm which is roughly 4 times the optical skin depth in
gold. The modeling of the transient optical reflectivity indicates that the
mechanism of phonon generation is achieved through ultrafast heating of the NPS
assisted by light excitation of the volume plasmon. These results demonstrate
how it is possible to map the photon-electron-phonon interaction in
subwavelength nanostructures