81 research outputs found
Ultrafast quenching of ring closure in molecular switches, self-assembled on gold nanoparticles
Near-Resonant Nonlinear Optical Properties of Pseudoisocyanine J-Aggregates in Langmuir-Blodgett Layers
Compact cryogenic Kerr microscope for time-resolved studies of electron spin transport in microstructures
A compact cryogenic Kerr microscope for operation in the small volume of
high-field magnets is described. It is suited for measurements both in Voigt
and Faraday configuration. Coupled with a pulsed laser source, the microscope
is used to measure the time-resolved Kerr rotation response of semiconductor
microstructures with ~1 micron spatial resolution. The microscope was designed
to study spin transport, a critical issue in the field of spintronics. It is
thus possible to generate spin polarization at a given location on a
microstructure and probe it at a different location. The operation of the
microscope is demonstrated by time-resolved measurements of micrometer distance
diffusion of spin polarized electrons in a GaAs/AlGaAs heterojunction quantum
well at 4.2 K and 7 Tesla
Many-body effects in the stimulated Raman response of binary mixtures:A comparison between theory and experiment
The subpicosecond dynamics of binary mixtures of carbon disulfide and alkane have been studied using third-order time-resolved Raman techniques. Both the anisotropic and the isotropic responses were investigated. These depend differently on many-body contributions to the first-order susceptibility and probe different modes in the liquid. The anisotropic response is dominated by single molecule effects, whereas the isotropic response is completely determined by many-body contributions since the single molecule response vanishes. To interpret the experimental results, molecular dynamics simulations were performed on model mixtures. The effect of dilution on the subpicosecond response cannot be explained by many-body effects in the first-order susceptibility alone. Aggregation due to permanent quadrupole moments on the carbon disulfide molecules and density changes upon dilution are also inadequate explanations for the observed effect. Apparently the character of the many-body dynamics itself is modified by the change of the molecular force fields, when carbon disulfide molecules are replaced by alkanes.<br/
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